摘要
Developing high-performance energy storage and conversion(ESC)device relies on both the utilization of good constituent materials and rational design of assembly structure.Graphene-based materials,due to their superior properties like high electrical/thermal conductivity,large surface area,and unique optical properties,have been extensively reported for ESC applications.The emerging three-dimensional(3D)printing techniques,especially extrusion-based direct ink writing technique,have brought a revolutionary improvement in structure control accuracy and designing capability to graphene-based macro-assemblies,triggering a boost in functionalities and performances of graphene-based ESC devices.In these circumstances,understanding the very recent progress of 3Dprinted graphene materials and their design philosophy to bring new concepts for material designs and address the requirements for high-performance ESC devices are urgently important.In this review,we aim to outline recent developments in 3D printing of graphene-based materials and their applications in ESC applications.Basic requirements and theoretical analysis for preparation printable inks are discussed,as well as feasible GO ink preparation strategies in existing literatures.The representative explorations of 3D-printed graphenematerials in ESC applications like batteries,supercapacitors,solar steam generators,and electro-thermal conversion are also reviewed.This study attempts to provide a comprehensive overview of the progresses and limitations of present 3D printed graphenematerials,and seeks to enlighten the opportunities and orientations of future research in this field.
出处
《SusMat》
2021年第3期304-323,共20页
可持续发展材料（英文）
基金
NationalNatural Science Foundation of China,Grant/Award Numbers:52090030,51533008,51973191,51703194,51803177
China Postdoctoral Science Foundation,Grant/Award Number:2021M692772
National Key R&D Program of China,Grant/Award Number:2016YFA0200200
FundamentalResearch Funds for the CentralUniversities,Grant/Award Numbers:30920041106,K20200060,30919011271
Hundred Talents Programof Zhejiang University,Grant/Award Number:188020*194231701/113
Key Research and Development Plan of Zhejiang Province,Grant/Award Number:2018C01049
KeyLaboratory of Novel Adsorption and Separation Materialsand Application Technology of Zhejiang Province,Grant/AwardNumber:512301-I21502。
作者简介
Zhen Xu,Email:zhenxu@zju.edu.cn;Correspondence:Chao Gao,Email:chaogao@zju.edu.cn。
