This paper presents the behavior simulation of high level radioactive waste repository in Beishan granite site which is the most potential one in China.Based on the results from site characterization in Beishan granit...This paper presents the behavior simulation of high level radioactive waste repository in Beishan granite site which is the most potential one in China.Based on the results from site characterization in Beishan granite site,the conceptual model of repository in this site is proposed and its calculation model is developed with software GoldSim.After verification,this calculation model is applied to simulate the展开更多
High level waste is nuclear energy generated during the application process ,which is the greatest and the most difficult to management the waste. Proper treatment and disposal of it has already become a worldwide pro...High level waste is nuclear energy generated during the application process ,which is the greatest and the most difficult to management the waste. Proper treatment and disposal of it has already become a worldwide problem, and has become one of the key factors of restricting nuclear energy for sustainable development. Zirconolite (CaZrTi2O7) is one of the most stable mineral on the Earth and actinide major parasitic phase, therefore, it is widely used to solidify actinides separated from high level radioactive waste. In this paper, the zirconolite solid solution was synthesized by high temperature solid-stated method using a particular composition of simulated Np/Pu radioactive incineration ash (SRIA). The phase composition has been investigated by X-ray diffraction (XRD), the calcined temperature gained according to thermogravimetry scanning calorimeter (TG-DSC) analysis. Anti-leaching performance has also been researched with MCC-1 method. Results show that CaZrTi2O7 can load 40% SRIA, the accumulated leaching fraction of Ca is only about 10-4 cm in 28 days at 90 ℃, the concentrations of Zr , Ti and other noble metal ions were all less than detectability of ICP-MS, the leaching rate , normalization leaching rate, and accumulated leaching fraction of all Zr , Ti and other noble ions were 10-8 cm/d, 10-8 g/cm2·d and 10-7 cm, the results indicate that the zirconolite solidification has excellent chemical durability.展开更多
Low radioactive rare earth waste (containing 232 Th,specific activity 5 000 8 000 Bq·kg -1 ) were diluted 20 times by cement,sand and carbide ash and were made into special cement.The radioactivity of...Low radioactive rare earth waste (containing 232 Th,specific activity 5 000 8 000 Bq·kg -1 ) were diluted 20 times by cement,sand and carbide ash and were made into special cement.The radioactivity of this special cement complied with the healthy protect standard for radioactive materials (GB6566 86).Test results showed that this special cement could lower COD,the degradation rate increased as the time went on.In acidic medium,this special cement could remove E Coli effectively.Applying aeration and adding lumps of cement,the degradation of COD versus time complied with Logistic model through fitting by computer.The two “S” curves indicated that aeration and adding lumps of cement had synergistic action on sewage treatment.展开更多
高放废物地质处置特别是地下实验室研发过程中的多源数据融合挖掘研究具有重要意义(Wang Ju et al.,2018)。然而,目前阶段尚未实现对研发过程中多源数据的融合挖掘与二次应用。针对上述问题,从地下实验室多源监测数据特点出发,在确定地...高放废物地质处置特别是地下实验室研发过程中的多源数据融合挖掘研究具有重要意义(Wang Ju et al.,2018)。然而,目前阶段尚未实现对研发过程中多源数据的融合挖掘与二次应用。针对上述问题,从地下实验室多源监测数据特点出发,在确定地下实验室多源监测数据模型构建的基础上,结合深度学习技术,初步构建了地下实验室多源监测数据融合技术方法,并初步开展了数据融合设计,为处置库场址评价和安全评价等综合评价工作提供了新的研究思路。展开更多
文摘This paper presents the behavior simulation of high level radioactive waste repository in Beishan granite site which is the most potential one in China.Based on the results from site characterization in Beishan granite site,the conceptual model of repository in this site is proposed and its calculation model is developed with software GoldSim.After verification,this calculation model is applied to simulate the
文摘High level waste is nuclear energy generated during the application process ,which is the greatest and the most difficult to management the waste. Proper treatment and disposal of it has already become a worldwide problem, and has become one of the key factors of restricting nuclear energy for sustainable development. Zirconolite (CaZrTi2O7) is one of the most stable mineral on the Earth and actinide major parasitic phase, therefore, it is widely used to solidify actinides separated from high level radioactive waste. In this paper, the zirconolite solid solution was synthesized by high temperature solid-stated method using a particular composition of simulated Np/Pu radioactive incineration ash (SRIA). The phase composition has been investigated by X-ray diffraction (XRD), the calcined temperature gained according to thermogravimetry scanning calorimeter (TG-DSC) analysis. Anti-leaching performance has also been researched with MCC-1 method. Results show that CaZrTi2O7 can load 40% SRIA, the accumulated leaching fraction of Ca is only about 10-4 cm in 28 days at 90 ℃, the concentrations of Zr , Ti and other noble metal ions were all less than detectability of ICP-MS, the leaching rate , normalization leaching rate, and accumulated leaching fraction of all Zr , Ti and other noble ions were 10-8 cm/d, 10-8 g/cm2·d and 10-7 cm, the results indicate that the zirconolite solidification has excellent chemical durability.
文摘Low radioactive rare earth waste (containing 232 Th,specific activity 5 000 8 000 Bq·kg -1 ) were diluted 20 times by cement,sand and carbide ash and were made into special cement.The radioactivity of this special cement complied with the healthy protect standard for radioactive materials (GB6566 86).Test results showed that this special cement could lower COD,the degradation rate increased as the time went on.In acidic medium,this special cement could remove E Coli effectively.Applying aeration and adding lumps of cement,the degradation of COD versus time complied with Logistic model through fitting by computer.The two “S” curves indicated that aeration and adding lumps of cement had synergistic action on sewage treatment.
文摘高放废物地质处置特别是地下实验室研发过程中的多源数据融合挖掘研究具有重要意义(Wang Ju et al.,2018)。然而,目前阶段尚未实现对研发过程中多源数据的融合挖掘与二次应用。针对上述问题,从地下实验室多源监测数据特点出发,在确定地下实验室多源监测数据模型构建的基础上,结合深度学习技术,初步构建了地下实验室多源监测数据融合技术方法,并初步开展了数据融合设计,为处置库场址评价和安全评价等综合评价工作提供了新的研究思路。