An atmospheric pressure argon plasma brush with air addition is employed to treat polyethylene terephthalate(PET)surface in order to improve its hydrophilicity.Results indicate that the plasma plume generated by the p...An atmospheric pressure argon plasma brush with air addition is employed to treat polyethylene terephthalate(PET)surface in order to improve its hydrophilicity.Results indicate that the plasma plume generated by the plasma brush presents periodically pulsed current despite a direct current voltage is applied.Voltage-current curve reveals that there is a transition from a Townsend discharge regime to a glow one during one discharge period.Optical emission spectrum indicates that more oxygen atoms are produced in the plume with increasing air content,which leads to the better hydrophilicity of PET surface after plasma treatment.Besides,an aging behavior is also observed.The hydrophilicity improvement is attributed to the production of oxygen functional groups,which increase in number with increasing air content.Moreover,some grain-like structures are observed on the treated PET surface,and its mean roughness increases with increasing air content.These results are of great importance for the hydrophilicity improvement of PET surface with a large scale.展开更多
基金supported by National Natural Science Foundation of China(Nos.11875121,11575050 and51977057)the Midwest Universities Comprehensive Strength Promotion Project+4 种基金the Natural Science Foundation of Hebei Province,China(Nos.A2019201100,A2020201025)College Hundred Outstanding Innovative Talent Support Program of Hebei Education Bureau(No.SLRC2017021)Post-graduate’s Innovation Fund Project of Hebei Province(Nos.CXZZBS2019023,CXZZBS2019029)the Natural Science Interdisciplinary Research Program of Hebei University(No.DXK201908)Post-graduate’s Innovation Fund Project of Hebei University(No.HBU2021bs011)。
文摘An atmospheric pressure argon plasma brush with air addition is employed to treat polyethylene terephthalate(PET)surface in order to improve its hydrophilicity.Results indicate that the plasma plume generated by the plasma brush presents periodically pulsed current despite a direct current voltage is applied.Voltage-current curve reveals that there is a transition from a Townsend discharge regime to a glow one during one discharge period.Optical emission spectrum indicates that more oxygen atoms are produced in the plume with increasing air content,which leads to the better hydrophilicity of PET surface after plasma treatment.Besides,an aging behavior is also observed.The hydrophilicity improvement is attributed to the production of oxygen functional groups,which increase in number with increasing air content.Moreover,some grain-like structures are observed on the treated PET surface,and its mean roughness increases with increasing air content.These results are of great importance for the hydrophilicity improvement of PET surface with a large scale.