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Atomically Precise Cu Nanoclusters:Recent Advances,Challenges,and Perspectives in Synthesis and Catalytic Applications
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作者 Mengyao Chen Chengyu Guo +4 位作者 Lubing Qin Lei Wang Liang Qiao Kebin Chi Zhenghua Tang 《Nano-Micro Letters》 2025年第4期130-165,共36页
Atomically precise metal nanoclusters are an emerging type of nanomaterial which has diverse interfacial metal-ligand coordination motifs that can significantly affect their physicochemical properties and functionalit... Atomically precise metal nanoclusters are an emerging type of nanomaterial which has diverse interfacial metal-ligand coordination motifs that can significantly affect their physicochemical properties and functionalities.Among that,Cu nanoclusters have been gaining continuous increasing research attentions,thanks to the low cost,diversified structures,and superior catalytic performance for various reactions.In this review,we first summarize the recent progress regarding the synthetic methods of atomically precise Cu nanoclusters and the coordination modes between Cu and several typical ligands and then discuss the catalytic applications of these Cu nanoclusters with some explicit examples to explain the atomical-level structure-performance relationship.Finally,the current challenges and future research perspectives with some critical thoughts are elaborated.We hope this review can not only provide a whole picture of the current advances regarding the synthesis and catalytic applications of atomically precise Cu nanoclusters,but also points out some future research visions in this rapidly booming field. 展开更多
关键词 Atomically precise Cu nanoclusters Controllable synthesis Catalytic applications Structure-performance relationship Challenges and perspectives
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Adsorption behavior of CO_(2)/H_(2)S mixtures in calcite slit nanopores for CO_(2) storage:An insight from molecular perspective
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作者 Cheng Qian Zhen-Hua Rui +4 位作者 Yue-Liang Liu Kai Du Chen Liu Yang Zhao Xiao-Min Ma 《Petroleum Science》 SCIE EI CAS CSCD 2024年第4期2444-2456,共13页
It is acknowledged that injecting CO_(2) into oil reservoirs and saline aquifers for storage is a practical and affordable method for CO_(2) sequestration.Most CO_(2) produced from industrial exhaust contains impurity... It is acknowledged that injecting CO_(2) into oil reservoirs and saline aquifers for storage is a practical and affordable method for CO_(2) sequestration.Most CO_(2) produced from industrial exhaust contains impurity gases such as H_(2)S that might impact CO_(2) sequestration due to competitive adsorption.This study makes a commendable effort to explore the adsorption behavior of CO_(2)/H_(2)S mixtures in calcite slit nanopores.Grand Canonical Monte Carlo(GCMC)simulation is employed to reveal the adsorption of CO_(2),H_(2)S as well as their binary mixtures in calcite nanopores.Results show that the increase in pressure and temperature can promote and inhibit the adsorption capacity of CO_(2) and H_(2)S in calcite nanopores,respectively.CO_(2)exhibits stronger adsorption on calcite surface than H_(2)S.Electrostatic energy plays the dominating role in the adsorption behavior.Electrostatic energy accounts for 97.11%of the CO_(2)-calcite interaction energy and 56.33%of the H_(2)S-calcite interaction energy at 10 MPa and 323.15 K.The presence of H_(2)S inhibits the CO_(2) adsorption in calcite nanopores due to competitive adsorption,and a higher mole fraction of H_(2)S leads to less CO_(2) adsorption.The quantity of CO_(2) adsorbed is lessened by approximately 33%when the mole fraction of H_(2)S reaches 0.25.CO_(2) molecules preferentially occupy the regions near the po re wall and H_(2)S molecules tend to reside at the center of nanopore even when the molar ratio of CO_(2) is low,indicating that CO_(2) has an adsorption priority on the calcite surface over H_(2)S.In addition,moisture can weaken the adsorption of both CO_(2) and H_(2)S,while CO_(2) is more affected.More interestingly,we find that pure CO_(2) is more suitable to be sequestrated in the shallower formations,i.e.,500-1500 m,whereas CO_(2)with H_(2)S impurity should be settled in the deeper reservoirs. 展开更多
关键词 Adsorption behavior CO_(2)/H_(2)S binary mixtures Molecular perspective Calcite slit nanopores CO_(2)sequestration
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DETERMINATION OF UNKNOWN CAMERA PARAMETERS FOR THE PERSPECTIVE IMAGES
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作者 昂海松 《Transactions of Nanjing University of Aeronautics and Astronautics》 EI 1996年第2期95+91-94,共5页
To obtain an accurate 3 D object configuration from images,the essential perspective characteristics must be considered. Several new inverse transformation relations of the perspective image lines are given. Utiliz... To obtain an accurate 3 D object configuration from images,the essential perspective characteristics must be considered. Several new inverse transformation relations of the perspective image lines are given. Utilizing the analytic transformation relations, an optimization procedure for obtaining the unknown camera parameters of images is presented in this paper. A 3 D reproduction method and examples are introduced. 展开更多
关键词 perspective projection optimization perspective image 3 D reproduction
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An Analysis of Love Metaphor LOVE IS A JOURNEY from the Perspective of Cognition
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作者 周玉亮 《海外英语》 2011年第8X期364-365,共2页
The working mechanism and experiential basis of love metaphor are deeply elaborated, and on the base of it, an analysis of love metaphor LOVE IS A JOURNEY from the perspective of cognition is carried out, which furthe... The working mechanism and experiential basis of love metaphor are deeply elaborated, and on the base of it, an analysis of love metaphor LOVE IS A JOURNEY from the perspective of cognition is carried out, which further illustrates the contemporary conceptual metaphor theory. 展开更多
关键词 LOVE METAPHOR working mechanism EXPERIENTIAL basis perspective of COGNITION
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A Naturalistic Perspective to the Kite Runner and Its Enlightenments to the Contemporary
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作者 钟伟轩 《海外英语》 2010年第9X期242-243,共2页
By analyzing the basic naturalistic features,namely the controlling power of environment and heredity,it is expected that the naturalistic tendency,at least naturalistic features of the novel can be revealed and some ... By analyzing the basic naturalistic features,namely the controlling power of environment and heredity,it is expected that the naturalistic tendency,at least naturalistic features of the novel can be revealed and some enlightenments on the world view of the contemporary can be gained.The early part of the thesis provides a frame by giving the research background and synopsis,while the later sections aim at approaching the conclusion at the efforts of unveiling the naturalistic features in the novel. 展开更多
关键词 NATURALISTIC perspective NATURALISTIC TENDENCY Enlightenments on world VIEW
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A Pragmatic Approach to Idiom Translation from a Cultural Perspective
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作者 马姝 《海外英语》 2011年第15期172-177,共6页
Idioms are gems of a language which have been refined through ages of use. Idioms are thus always rich in cultural connotation and national flavor. Lots of cultural information is embedded in idioms. Language is a par... Idioms are gems of a language which have been refined through ages of use. Idioms are thus always rich in cultural connotation and national flavor. Lots of cultural information is embedded in idioms. Language is a part of culture. Language is the important carrier of culture. Language and culture have close relationship with each other. The study of the relationship between language and culture has been considered a subject of great value. Owing to this, translation theorists and translators have put more attention to the cultural barriers that exist in translation. Therefore, translators have to better understand the relationship between language and culture and the relationship between culture and translation so as to render idioms from the SL into the TL faithfully and effectively. 展开更多
关键词 PRAGMATIC APPROACH IDIOM TRANSLATION CULTURAL perspective
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Literary Text Translation from Functional Perspective
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作者 李菁菁 《海外英语》 2012年第19期150-152,共3页
Functional linguistics has become the most influential linguistic theory in the field of translation study since the last de cade of 20th century.However,for the complexity of the context,it is uncommon and insufficie... Functional linguistics has become the most influential linguistic theory in the field of translation study since the last de cade of 20th century.However,for the complexity of the context,it is uncommon and insufficient to explore literary texts.Draw ing a general picture of literary text translation from functional perspectives aims to probe into the functional modes of translation. 展开更多
关键词 LITERARY TEXT TRANSLATION FUNCTIONAL perspective F
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Analysis of Ambiguity in Newspaper Headlines from a Cognitive Perspective
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作者 刘启迪 《海外英语》 2011年第15期310-312,共3页
Ambiguity in newspaper headlines have been studied by many people, which mostly focuses upon the traditional linguistics perspective: lexical, grammatical and syntactical. In this paper, the author intends to study th... Ambiguity in newspaper headlines have been studied by many people, which mostly focuses upon the traditional linguistics perspective: lexical, grammatical and syntactical. In this paper, the author intends to study the ambiguity in newspaper headlines from the cognitive perspective in order to find how people perceive the ambiguous headlines. To support the analysis, many examples of ambiguous headlines are collected to investigate into way people perceive them. Finally, the author concluded that in the cognitive perspective, people are prone to accept one of the two or more interpretations about the ambiguous headlines according to the following factors: their back ground knowledge, the common sense, the social-cultural environment as well as their personal altitudes, which are drawn upon from the image schema theory. 展开更多
关键词 AMBIGUITY NEWSPAPER HEADLINE COGNITIVE perspective
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A Warm Death Trip——An Interpretation of The Great Blue Yonder from the Dead Children Narrative Perspective
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作者 黄洁 《海外英语》 2015年第21期195-197,共3页
When it comes to the death,it can be gruesome or be dolente.However,the death also can be warm and be a new start of life.It is because we regard the death from different perspective that we show different attitude to... When it comes to the death,it can be gruesome or be dolente.However,the death also can be warm and be a new start of life.It is because we regard the death from different perspective that we show different attitude to the death.The novel The Great Blue Yonder which described the experience of the little protagonist died as a ghost wandering in the mortal world interpreted the death by fairy tale.In his wandering trip,he experience not only tears but also laughter.The more important experience he realized was that he took a new look at love and comprehended the significance of life.Because of the dislocation between narrative perspective and narrative contents,the abnormal narrative perspective owns the unique artistic charm.This thesis aims to interpret the Great Blue Yonder by taking the abnormal narrative perspective as the point of view from the dual narrative perspective of the ghosts and the children.The abnormal narrative perspective is endowed with the unique aesthetic effect because of its own aesthetic properties.It will make a great fresh aesthetic feast to readers. 展开更多
关键词 the dead ghost narrative perspective the children narrative perspective DEATH The great blue yonder
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Challenges of gaming disorder: suggestions from a public health perspective 被引量:3
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作者 Min Zhao Wei Hao 《General Psychiatry》 CSCD 2019年第3期105-106,共2页
Based on the results from numerous studies and discussions by expert groups organised by the WHO, gaming disorder is recognised as a mental disorder and is listed in the chapter of mental, behavioural and neurodevelop... Based on the results from numerous studies and discussions by expert groups organised by the WHO, gaming disorder is recognised as a mental disorder and is listed in the chapter of mental, behavioural and neurodevelopmental disorders in the recently released International Classification of Diseases, 11th Version (ICD-11). 展开更多
关键词 CHALLENGES gaming DISORDER a PUBLIC HEALTH perspective
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Second Harmonic Generation of Lamb Wave in Numerical Perspective 被引量:2
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作者 朱武军 邓明晰 +2 位作者 项延训 轩福贞 刘长军 《Chinese Physics Letters》 SCIE CAS CSCD 2016年第10期71-74,共4页
The influences of phase and group velocity matching on cumulative second harmonic generation of Lamb waves are investigated in numerical perspective. Finite element simulations of nonlinear Lamb wave propagation are p... The influences of phase and group velocity matching on cumulative second harmonic generation of Lamb waves are investigated in numerical perspective. Finite element simulations of nonlinear Lamb wave propagation are performed for Lamb wave mode pairs with exact and approximate phase velocity matching, with and without group velocity matching, respectively. The evolution of time-domain second harmonic Lamb waves is analyzed with the propagation distance. The amplitudes of primary and second harmonic waves are calculated to characterize the acoustic nonlinearity. The results verify that phase velocity matching is necessary for generation of the cumulative second harmonic Lamb wave in numerical perspective, while group velocity matching is demonstrated to not be a necessary condition. 展开更多
关键词 of on MODE Second Harmonic Generation of Lamb Wave in Numerical perspective in IS for PAIR
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Numerical Perspective of Second-Harmonic Generation of Circumferential Guided Wave Propagation in a Circular Tube 被引量:2
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作者 李明亮 邓明晰 +2 位作者 朱武军 高广健 项延训 《Chinese Physics Letters》 SCIE CAS CSCD 2016年第12期81-85,共5页
The effect of second-harmonic generation (SHG) by primary (fundamental) circumferential guided wave (CGW) propagation is investigated from a numerical standpoint. To enable that the second harmonic of the primar... The effect of second-harmonic generation (SHG) by primary (fundamental) circumferential guided wave (CGW) propagation is investigated from a numerical standpoint. To enable that the second harmonic of the primary CGW mode can accumulate along the circumferential direction, an appropriate mode pair of primary and double frequency CGWs is chosen. Finite element simulations and evaluations of nonlinear CGW propagation are analyzed for the selected CGW mode pair. The numerical simulations performed directly demonstrate that the response of SHG is completely generated by the desired primary CGW mode that satisfies the condition of phase velocity matching at a specific driving frequency, and that the second harmonic of the primary CGW mode does have a cumulative effect with circumferential angles. The numerical perspective obtained yields an insight into the complicated physical process of SHG of primary CGW propagation unavailable previously. 展开更多
关键词 of on MODE Numerical perspective of Second-Harmonic Generation of Circumferential Guided Wave Propagation in a Circular Tube in SHG is for that
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PERSPECTIVE OF COAL DEVELOPMENT OF CHINA IN THE EARLY 2000'S 被引量:1
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作者 王玉浚 《Journal of China University of Mining and Technology》 1996年第1期1-8,共8页
According to the Researches on Coal Development Strategies in China (1991 ~ 2020),the production scale of coal in China will increase to 2100 Mt in the year 2020 and the district layout of coal development and product... According to the Researches on Coal Development Strategies in China (1991 ~ 2020),the production scale of coal in China will increase to 2100 Mt in the year 2020 and the district layout of coal development and production will be diverted from the east to the central-west step by step. In addit1on, the multi-ply runnning struc ture-mines of the nation,the local and the village and town combined with produc tion scales of the large, the middle,and the small-will be kept. However,the tech nique of mining will be improved greatly. 展开更多
关键词 COAL DEVELOPMENT perspective
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On Sister Carrie from Feminist Perspective and its Influence on Chinese Modern Women
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作者 毛武毅 叶青 《海外英语》 2013年第1X期187-189,共3页
Sister Carrie is a famous naturalistic novelist-Theodore Dreiser's first novel in the first 20th century.It tells a story of a young rural woman Carrie how to become the red Broadway actress from the bottom of soc... Sister Carrie is a famous naturalistic novelist-Theodore Dreiser's first novel in the first 20th century.It tells a story of a young rural woman Carrie how to become the red Broadway actress from the bottom of society,and the story vividly depicts the survival state and psychological and ideological process of Carrie.When it was published,it attracted attentions of critics from domestic and abroad at large,and they researched it from different perspectives.But most of their researches discussed from the materialism angle to concern with the expression of Determinism and Darwinism.So far,few people made the research from the topic of Carrie's pursuit of self-achievement and perspective of feminist.Actually,not only did Carrie restrict on the material pursuit,but also boldly in pursuit of the self-achievement of new women.This paper aims at Carrie how to pursue the selfachievement of new women,and the influence of feminist to Chinese modern women. 展开更多
关键词 SISTER CARRIE FEMINIST perspective CHINESE MODERN
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An Analysis of Passing from the Psychological Perspective
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作者 马莲 胡笑瑛 《海外英语》 2012年第21期174-176,共3页
The short novel Passing,written by Nella Larsen,who is an American novelist and short story writer.Larsen was best known for her contributions to the literary development in Harlem renaissance.This paper aims at analy... The short novel Passing,written by Nella Larsen,who is an American novelist and short story writer.Larsen was best known for her contributions to the literary development in Harlem renaissance.This paper aims at analyzing the short novel from the psychological perspective. 展开更多
关键词 ANALYSIS PASSING PSYCHOLOGICAL perspective
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Reasons for Chinese Crave for Civil-Service Jobs:A Cross-Cultural Perspective
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作者 张梦 张严心 《海外英语》 2021年第14期295-296,共2页
This paper is aimed at exploring the cultural reasons underlying the civil service examinations,which can be concludedas"Tri-Cs",namely the well-established agricultural civilization,cadre culture and family... This paper is aimed at exploring the cultural reasons underlying the civil service examinations,which can be concludedas"Tri-Cs",namely the well-established agricultural civilization,cadre culture and family-oriented concept.Through in-depthanalyses,the author strives to clarify the possible reasons for this exam fever and help delineate a clearer picture of the essentials ofChinese culture. 展开更多
关键词 civil service exam cross-cultural perspective agricultural civilization cadre culture family-oriented concept
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On the Defamiliarization Effect of Benjy's Idiot Perspective in The Sound and the Fury
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作者 庞悦 《海外英语》 2017年第7期181-183,共3页
As the core conception in Russian Formalism,the defamiliarization is fully manifested in The Sound and the Fury.The employ-ments of two defamiliarization devices—the uniqueness of narrative perspective and the diffic... As the core conception in Russian Formalism,the defamiliarization is fully manifested in The Sound and the Fury.The employ-ments of two defamiliarization devices—the uniqueness of narrative perspective and the difficulty of the language are much prominent inthe narration of the idiot Benji,through which the work possesses a strong aesthetic effect.Through exploring the much objective descrip-tion of the stream of consciousness and the defamiliarization effect which are created by the idiot perspective,this thesis will highlightthe various conflicts of the Compson family and the time they lived in,thus revealing the theme of a great family's decline.The authorwill also analyze the sensory stimulation and emotional shock brought by the unique narrative perspective. 展开更多
关键词 idiot perspective DEFAMILIARIZATION LANGUAGE stream of consciousness The Sound and the Fury
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Construction scheme comparison with comprehensive evaluation of independent perspectives
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作者 阎西康 王磊 CHEN Pei 《Journal of Chongqing University》 CAS 2013年第3期131-135,共5页
Considering both the characteristics of construction scheme evaluation and the lack of consideration of index proportionality after introducing comprehensive evaluation of independent perspectives into construction sc... Considering both the characteristics of construction scheme evaluation and the lack of consideration of index proportionality after introducing comprehensive evaluation of independent perspectives into construction scheme evaluation, a construction scheme evaluation model of independent perspectives was put forward through the study and optimization of comprehensive evaluation of independent perspectives. The feasibility and rationality of the optimized method were illustrated through a case study and the evaluation results were compared between the optimized method and non-optimized method. The optimized method has the practical value in construction scheme comparison. 展开更多
关键词 construction scheme evaluation model independent perspective comprehensive evaluation
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Clinical perspective on C-reactive protein in prognostication of major adverse cardiac events in the elderly with established coronary heart disease
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作者 Olabode Oladeinde 《Journal of Geriatric Cardiology》 SCIE CAS CSCD 2006年第2期82-84,共3页
  The systemic response to tissue injury, regardless of cause is characterized by a cytokine-mediated alteration in the hepatic synthesis of a number of different plasma proteins,known collectively as 'acute pha...   The systemic response to tissue injury, regardless of cause is characterized by a cytokine-mediated alteration in the hepatic synthesis of a number of different plasma proteins,known collectively as 'acute phase reactants'. These proteins include C-reactive protein, serum amyloid A protein, alphal glycoprotein, ceruloplasmin, alpha macroglobulins, complement components (C1-C4, factor B, C9, C11), alpha1antitrypsin, alpha1 antichymotrypsin, fibrinogen, prothrombin,factor Ⅷ, plasminogen, haptoglobin, ferritin, immunoglobulins and lipoproteins. The initiation of the acute phase response is linked to the production of hormone-like polypeptide mediators now called cytokines, namedly, interleukin 1(IL-1),tumor necrosis factor, interferon gamma, interleukin 6 (IL-6),leukemia inhibitory factor, ciliary neurotropic factor, oncostatin M, and interleukin 11 (IL- 11).…… 展开更多
关键词 CRP Clinical perspective on C-reactive protein in prognostication of major adverse cardiac events in the elderly with established coronary heart disease CHD MACE
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Perspective on NGN Commercial Deployment in China
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作者 Liu Yinghe (Telecom Weekly,China Electronics News,Bejing 100044,China) 《ZTE Communications》 2004年第2期2-4,共3页
NGN not only means the renewal of network technology,but also marks an important milestone of telecom industry development.Carriers,equipment manufacturers,various members on the industrial chain and the government sh... NGN not only means the renewal of network technology,but also marks an important milestone of telecom industry development.Carriers,equipment manufacturers,various members on the industrial chain and the government should keep pace with time and make innovation together to implement large-scale NGN commercialization. 展开更多
关键词 NGN perspective on NGN Commercial Deployment in China ZTE
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