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内源反硝化过程中N_2O的产生特征 被引量:6

Nitrous Oxide Production Characteristic During Endogenous Denitrification
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摘要 为了控制污水处理过程温室气体氧化亚氮(N2O)的排放量和提高污水处理厂产能,提出了强化反硝化过程中N2O积累,而后用N2O氧化甲烷提高燃烧产能同时减少N2O排放的方法.通过研究内源反硝化过程中N2O的产生特征得出,以硝酸盐(NO-3)作为电子受体的内源反硝化过程会出现亚硝酸盐(NO-2)和N2O的积累,且二者同时出现;当以不同质量浓度的NO-2-N(13~90 mg/L)作为电子受体进行内碳源反硝化时得出,高籽(NO-2-N)会同时抑制NO-2和N2O的还原过程,从而使得内源反硝化过程中出现N2O的积累.基于此结果提出通过调控籽(NO-2-N)来强化反硝化过程中N2O的积累,从而为N2O氧化甲烷提供基础. In order to control greenhouse gas emission and improve energy production in wastewater treatment plants, a new method based on nitrous oxide ( N2 O) oxidizing methane was proposed with anincrease in energy production from methane oxidation and a decrease in N2 O emission. This studyinvestigated N2 O production characteristic during endogenous denitrification. The results showed that nitrite and N2 O were accumulated simultaneously when nitrate was used as electron acceptor. Nitrite and N2 O reduction wereinhibited when nitrite concentrationincreasedin the range of 13-90 mg/L, resultingin N2 O accumulation during endogenous denitrification process. Based on these results, to enhance N2 O accumulation by adjusting nitrite concentration was proposed, which could provide the basis of methane oxidation using N2 O sequentially.
出处 《北京工业大学学报》 CAS CSCD 北大核心 2015年第8期1253-1258,共6页 Journal of Beijing University of Technology
基金 国家自然科学基金资助项目(51478013) 北京市自然科学基金资助项目(8154041) 北京市优秀人才培养资助项目(2014000020124G043)
关键词 污水处理 温室气体 氧化亚氮 内源反硝化 watewater treatment greenhouse gas endogenous denitrification
作者简介 汪传新(1963-),男,博士研究生,主要从事水污染控制方面的研究,E-mail:mabin@bjut.edu.cn
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