摘要
利用计算化学工程方法,针对甲烷催化燃烧和甲烷水蒸气重整的模型反应体系,研究了一种结构较复杂的金属基整体式催化反应器用于吸/放热反应耦合时的性能.模拟结果表明,这种金属基整体式催化反应器应用于吸/放热反应耦合具有很大的研发潜力.初步分析了操作参数的影响,重整侧与燃烧侧入口气体速度的比值、气体入口温度以及燃烧部分和重整部分的甲烷体积流量比都是影响反应器性能的重要因素.
A metal monolith reactor with complicated structure, used in coupled methane steam reforming-combustion, was investigated by using a heterogeneous model based on the whole reactor in this work. Preliminary results showed that the application was considerably attractive, and the significant effects on the reactor performance of the operating parameters, such as inlet gas velocity ratio of reforming side and combustion side, inlet gas temperature and volumetric flux ratio of combustion side and reforming side were presented.
出处
《化工学报》
EI
CAS
CSCD
北大核心
2006年第8期1904-1910,共7页
CIESC Journal
关键词
金属基整体式催化反应器
吸/放热反应耦合
操作参数
metal monolith reactor
coupled endothermic and exothermic reactions
operating parameters
作者简介
梅红（1981-）,女,博士研究生.
李成岳. 联系人：E-mail：licy@mail.buct.edu.cn
