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多光子过程光强指数的新应用——激发截面估计 被引量:5

A New Application of Laser Power Index in Multiphoton Processer:estimation of excitation cross sections
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摘要 本文针对多光子过程产物信号随激光强度变化的特征,提出了一个利用测得的产物信号的激光强度依赖关系来估算多步多光子过程的激发截面的简单方法.该估算方法是从两步多光子吸收过程的动力学模型中导出的,并可以合理地推广到任意多步的多光子过程.我们用一些数值模拟计算和实验的结果进一步验证了该方法的合理性. In this paper, the general characteristics of laser power index of product signal in multphoton processes were discussed and a new method to estimate excitation process by analyzing the variation of power indew with laser intensity were proposed. The validity of this method is theoretically demonstrated by means of the rate equations based upon a two-step kinetic model and some numerical and experimental results. This method could, in principle, be extended to the multiphoton process with steps more than two.
出处 《Chinese Journal of Chemical Physics》 SCIE CAS CSCD 1996年第2期104-112,共9页 化学物理学报(英文)
基金 国家自然科学基金资助课题
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参考文献1

  • 1Chen C X,Chem Phys Lett,1993年,203卷,307页

同被引文献29

  • 1李海洋,白吉玲.多光子电离伴随的碎片化过程的速率方程分析[J].物理化学学报,1995,11(2):107-112. 被引量:1
  • 2柳晓军,张冰,方黎,郭文跃,周金刚,蔡继业,路轶群,周士康.甲胺分子多光子电离质谱研究[J].物理化学学报,1996,12(11):981-985. 被引量:17
  • 3郭文跃,魏杰,张冰,方黎,蔡继业.多光子过程的光强指数研究[J].量子电子学报,1997,14(2):130-136. 被引量:6
  • 4Boesl U,Weinkauf R,Walter K,et al.Tandem time of flight techniques and multiphoton mass spectrometry:the ladder switching in benzene[J].J.Phys.Chem.,1990,94(23):8 567—8 573.
  • 5Kiihlewind H,Neusser H J,Schlag E W.Laser multiphoton dissociation of alkyl cations: I.Fragmentation mechanism of homologous alkyl cationsproduced from their iodides[J].J.Phys.Chem.1985,89(26):5 593-5 599.
  • 6Silberstein J,Ohmichi N。Levine R D.The dominant fragmentation pathways in multiphoton ionization of alkyl iodides[J],Phys.Chem.,1985,85(26):5 606—5613.
  • 7Xing X,McDiarmid R,Philis J G,et al.Vibrational assignments in the 3p Rydberg states of acetone[J].J.Chem.Phys.1993,99(10):7 565—7 573.
  • 8Brint P,O’Toole L.Muhiphoton ionization spectroscopy of the 3s(2+2,1)and 4s(3+1)Rydberg states of acetone:evidence for a molecular valence state at 153 nm[J].J.Chem.Soc.Faraday Tram.,1990,87(18):2891—2 895.
  • 9Decanken A,McDiarmid R.Experimental one and two photon absorption properties of acetone[J].J.Chem.Phvs..1990.92(5):3 237—3 238.
  • 10Liu H,Li S,Han J,et al.Multiphoton ionization and fragmentation study of acetone at XeCl excimer laser radiation[J].Chem.Phys.,1987,118:285-287.

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