We show that the volume of the projection bodyΠ(Z)of an n-dimensional zonotope Z with n+1 generators and of volume 1 is always exactly 2^(n).Moroever,we point out that an upper bound on the volume ofΠ(K)of a central...We show that the volume of the projection bodyΠ(Z)of an n-dimensional zonotope Z with n+1 generators and of volume 1 is always exactly 2^(n).Moroever,we point out that an upper bound on the volume ofΠ(K)of a centrally symmetric n-dimensional convex body of volume 1 is at least 2^(n)(9/8)^([n/3]).展开更多
Non-precious metal cobalt-based oxide inevitably dissolves for acid oxygen evolution reaction(OER).Designing an efficient deposition channel for leaching cobalt species is a promising approach.The dissolution-depositi...Non-precious metal cobalt-based oxide inevitably dissolves for acid oxygen evolution reaction(OER).Designing an efficient deposition channel for leaching cobalt species is a promising approach.The dissolution-deposition equilibrium of Co is achieved by doping Mn in the lattice of LaCo_(1-x)Mn_(x)O_(3),prolonging the lifespan in acidic conditions by 14 times.The lattice doping of Mn produces a strain that enhances the adsorption capacity of OH^(-).The self-catalysis of Mn causes the leaching Co to be deposited in the form of CoO_(2),which ensures that the long-term stability of LaCo_(1-x)Mn_(x)O_(3)is 70 h instead of 5 h for LaCoO_(3).Mn doping enhances the deprotonation of^(*)OOH→O_(2)in acidic environments.Notably,the over-potential of optimized LaCo_(1-x)Mn_(x)O_(3)is 345 mV at 10 mA cm^(-2)for acidic OER.This work presents a promising method for developing noble metal-free catalysts that enhance the acidic OER activity and stability.展开更多
Peanut allergy is majorly related to severe food induced allergic reactions.Several food including cow's milk,hen's eggs,soy,wheat,peanuts,tree nuts(walnuts,hazelnuts,almonds,cashews,pecans and pistachios),fis...Peanut allergy is majorly related to severe food induced allergic reactions.Several food including cow's milk,hen's eggs,soy,wheat,peanuts,tree nuts(walnuts,hazelnuts,almonds,cashews,pecans and pistachios),fish and shellfish are responsible for more than 90%of food allergies.Here,we provide promising insights using a large-scale data-driven analysis,comparing the mechanistic feature and biological relevance of different ingredients presents in peanuts,tree nuts(walnuts,almonds,cashews,pecans and pistachios)and soybean.Additionally,we have analysed the chemical compositions of peanuts in different processed form raw,boiled and dry-roasted.Using the data-driven approach we are able to generate new hypotheses to explain why nuclear receptors like the peroxisome proliferator-activated receptors(PPARs)and its isoform and their interaction with dietary lipids may have significant effect on allergic response.The results obtained from this study will direct future experimeantal and clinical studies to understand the role of dietary lipids and PPARisoforms to exert pro-inflammatory or anti-inflammatory functions on cells of the innate immunity and influence antigen presentation to the cells of the adaptive immunity.展开更多
The behavior of a chemical tanker(CT)in extreme waves was discussed in detail,that is,in terms of rigid body heave and pitch motions,vertical bending moments(VBMs)amidships,green water,and slamming impacts through the...The behavior of a chemical tanker(CT)in extreme waves was discussed in detail,that is,in terms of rigid body heave and pitch motions,vertical bending moments(VBMs)amidships,green water,and slamming impacts through the analysis of the experimental data from model tests.Regular wave tests conducted for two wave steepness showed that the increase in wave steepness caused the increase in the asymmetry between hogging and sagging moments and the contribution of green water on deck to the decrease in vertical wave bending moments.Random uncertainty analysis of statistical values in irregular wave tests with various seeds revealed slight experimental uncertainties on motions and VBMs and slightly higher errors in slamming pressure peaks.With the increase in forward speed,experimental uncertainty on slamming pressures at the bow increased.Breather solutions of the nonlinear Schrödinger equation applied to generate tailored extreme waves of certain critical wavelengths showed a good performance in terms of ship response,and it was further verified for the CT.展开更多
Seawater photoelectrolysis is showing huge potential in green energy conversion field,yet it is still a formidable challenge to develop one catalyst that can drive the electrolysis reaction stably,economically and eff...Seawater photoelectrolysis is showing huge potential in green energy conversion field,yet it is still a formidable challenge to develop one catalyst that can drive the electrolysis reaction stably,economically and efficiently.Motivated by this point,the inorganic–organic hybridization strategy is proposed to insitu construct one hierarchical electrode via concurrent electroless plating and polymerization,which assures the growth of boron-modulated nickel–cobalt oxyhydroxide nanoballs and photosensitive polyaniline nanochains on the self-supporting Ti-based foil(B-Co Ni OOH/PANI@TiO_(2)/Ti).Upon inducing photoelectric effect(PEE),the designed target electrode delivers overpotentials as low as 196 and 398 mV at 100 mA cm^(-2)for hydrogen evolution reaction(HER)and oxygen evolution reaction(OER),respectively,corresponding to an activity enhancement by about 15%as compared to those without PEE.Inspiringly,when served as bifunctional electrocatalysts for overall seawater electrolysis,it can stably maintain at 200 mA cm^(-2)with negligible decay over 72 h.Further analysis reveals that the exceptional catalytic performance can be credit to the B-CoNiOOH,polyaniline(PANI)and TiO_(2)subunit coupling-induced physically and chemically synergistic catalysis effect such as admirable composition stability,photoelectric function and adhesion capability.The finding in this contribution may trigger much more broad interest to the novel hybrid catalysts consisting of photosensitive polymer and transition metal-based electrocatalysts.展开更多
The size of hysteresis loops and interior loops in pseudoelasticity were investigated with CuZnAl memory single crystal.The results show that the width of the hysteresis loop does not change significantly with tempera...The size of hysteresis loops and interior loops in pseudoelasticity were investigated with CuZnAl memory single crystal.The results show that the width of the hysteresis loop does not change significantly with temperature;while the size of the interior loops of hysteresis strongly depends on the martensitic phase fraction induced from austenit.展开更多
This paper presents a comprehensive experimental study on the effect of extreme waves on a LNG carrier.The LNG carrier model was equipped with a variety of sensors to measure motions,green water height on deck as well...This paper presents a comprehensive experimental study on the effect of extreme waves on a LNG carrier.The LNG carrier model was equipped with a variety of sensors to measure motions,green water height on deck as well as local and global loads.Experiments in transient wave packets provided the general performance in waves in terms of response amplitude operators and were accompanied by tests in regular waves with two different wave steepness.These tests allowed detailed insights into the nonlinear behavior of the vertical wave bending moment in steep waves showing that green water on deck can contribute to a decrease of vertical wave bending moment.Afterwards,systematic model tests in irregular waves were performed to provide the basis for statistical analysis.It is shown that the generalized extreme value distribution model is suitable for the estimation of the extreme peak values of motions and loads.Finally,model tests in tailored extreme wave sequences were conducted comparing the results with the statistical analysis.For this purpose,analytical breather solutions of the nonlinear Schrödinger equation were applied to generate tailored extreme waves of certain critical wave lengths in terms of ship response.Besides these design extreme waves,the LGN carrier was also investigated in the model scale reproduction of the real-world Draupner wave.By comparing the motions,vertical wave bending moment,green water column and slamming pressures it is concluded that the breather solutions are a powerful and efficient tool for the generation of design extreme waves of certain critical wave lengths for wave/structure investigations on different subjects.展开更多
文摘We show that the volume of the projection bodyΠ(Z)of an n-dimensional zonotope Z with n+1 generators and of volume 1 is always exactly 2^(n).Moroever,we point out that an upper bound on the volume ofΠ(K)of a centrally symmetric n-dimensional convex body of volume 1 is at least 2^(n)(9/8)^([n/3]).
基金financially supported by the Shandong Provincial Natural Science Foundation(ZR2023LFG005)the National Natural Science Foundation of China(Nos.22479161,52274308 and U22B20144)the Fundamental Research Funds for the Central Universities(No.24CX03012A)。
文摘Non-precious metal cobalt-based oxide inevitably dissolves for acid oxygen evolution reaction(OER).Designing an efficient deposition channel for leaching cobalt species is a promising approach.The dissolution-deposition equilibrium of Co is achieved by doping Mn in the lattice of LaCo_(1-x)Mn_(x)O_(3),prolonging the lifespan in acidic conditions by 14 times.The lattice doping of Mn produces a strain that enhances the adsorption capacity of OH^(-).The self-catalysis of Mn causes the leaching Co to be deposited in the form of CoO_(2),which ensures that the long-term stability of LaCo_(1-x)Mn_(x)O_(3)is 70 h instead of 5 h for LaCoO_(3).Mn doping enhances the deprotonation of^(*)OOH→O_(2)in acidic environments.Notably,the over-potential of optimized LaCo_(1-x)Mn_(x)O_(3)is 345 mV at 10 mA cm^(-2)for acidic OER.This work presents a promising method for developing noble metal-free catalysts that enhance the acidic OER activity and stability.
文摘Peanut allergy is majorly related to severe food induced allergic reactions.Several food including cow's milk,hen's eggs,soy,wheat,peanuts,tree nuts(walnuts,hazelnuts,almonds,cashews,pecans and pistachios),fish and shellfish are responsible for more than 90%of food allergies.Here,we provide promising insights using a large-scale data-driven analysis,comparing the mechanistic feature and biological relevance of different ingredients presents in peanuts,tree nuts(walnuts,almonds,cashews,pecans and pistachios)and soybean.Additionally,we have analysed the chemical compositions of peanuts in different processed form raw,boiled and dry-roasted.Using the data-driven approach we are able to generate new hypotheses to explain why nuclear receptors like the peroxisome proliferator-activated receptors(PPARs)and its isoform and their interaction with dietary lipids may have significant effect on allergic response.The results obtained from this study will direct future experimeantal and clinical studies to understand the role of dietary lipids and PPARisoforms to exert pro-inflammatory or anti-inflammatory functions on cells of the innate immunity and influence antigen presentation to the cells of the adaptive immunity.
文摘The behavior of a chemical tanker(CT)in extreme waves was discussed in detail,that is,in terms of rigid body heave and pitch motions,vertical bending moments(VBMs)amidships,green water,and slamming impacts through the analysis of the experimental data from model tests.Regular wave tests conducted for two wave steepness showed that the increase in wave steepness caused the increase in the asymmetry between hogging and sagging moments and the contribution of green water on deck to the decrease in vertical wave bending moments.Random uncertainty analysis of statistical values in irregular wave tests with various seeds revealed slight experimental uncertainties on motions and VBMs and slightly higher errors in slamming pressure peaks.With the increase in forward speed,experimental uncertainty on slamming pressures at the bow increased.Breather solutions of the nonlinear Schrödinger equation applied to generate tailored extreme waves of certain critical wavelengths showed a good performance in terms of ship response,and it was further verified for the CT.
基金supported by the National Natural Science Foundation of China(22109098)the Shanghai Sailing Program(20YF1432300)+4 种基金the Shanghai Engineering Research Center for Food Rapid Detection(19DZ2251300)the Natural Science Foundation of Jiangsu Province(BK20210735)the Natural Science Foundation of the Higher Education Institutions of Jiangsu Province(21KJB430043)the Collaborative Innovation Center of Suzhou Nano Science&Technology,the 111 Projectthe Suzhou Key Laboratory of Functional Nano&Soft Materials。
文摘Seawater photoelectrolysis is showing huge potential in green energy conversion field,yet it is still a formidable challenge to develop one catalyst that can drive the electrolysis reaction stably,economically and efficiently.Motivated by this point,the inorganic–organic hybridization strategy is proposed to insitu construct one hierarchical electrode via concurrent electroless plating and polymerization,which assures the growth of boron-modulated nickel–cobalt oxyhydroxide nanoballs and photosensitive polyaniline nanochains on the self-supporting Ti-based foil(B-Co Ni OOH/PANI@TiO_(2)/Ti).Upon inducing photoelectric effect(PEE),the designed target electrode delivers overpotentials as low as 196 and 398 mV at 100 mA cm^(-2)for hydrogen evolution reaction(HER)and oxygen evolution reaction(OER),respectively,corresponding to an activity enhancement by about 15%as compared to those without PEE.Inspiringly,when served as bifunctional electrocatalysts for overall seawater electrolysis,it can stably maintain at 200 mA cm^(-2)with negligible decay over 72 h.Further analysis reveals that the exceptional catalytic performance can be credit to the B-CoNiOOH,polyaniline(PANI)and TiO_(2)subunit coupling-induced physically and chemically synergistic catalysis effect such as admirable composition stability,photoelectric function and adhesion capability.The finding in this contribution may trigger much more broad interest to the novel hybrid catalysts consisting of photosensitive polymer and transition metal-based electrocatalysts.
文摘The size of hysteresis loops and interior loops in pseudoelasticity were investigated with CuZnAl memory single crystal.The results show that the width of the hysteresis loop does not change significantly with temperature;while the size of the interior loops of hysteresis strongly depends on the martensitic phase fraction induced from austenit.
基金the experimental work performed during the project EXTREME SEASwhich was funded by the European Commissionunder the Grant agreement No. 234175
文摘This paper presents a comprehensive experimental study on the effect of extreme waves on a LNG carrier.The LNG carrier model was equipped with a variety of sensors to measure motions,green water height on deck as well as local and global loads.Experiments in transient wave packets provided the general performance in waves in terms of response amplitude operators and were accompanied by tests in regular waves with two different wave steepness.These tests allowed detailed insights into the nonlinear behavior of the vertical wave bending moment in steep waves showing that green water on deck can contribute to a decrease of vertical wave bending moment.Afterwards,systematic model tests in irregular waves were performed to provide the basis for statistical analysis.It is shown that the generalized extreme value distribution model is suitable for the estimation of the extreme peak values of motions and loads.Finally,model tests in tailored extreme wave sequences were conducted comparing the results with the statistical analysis.For this purpose,analytical breather solutions of the nonlinear Schrödinger equation were applied to generate tailored extreme waves of certain critical wave lengths in terms of ship response.Besides these design extreme waves,the LGN carrier was also investigated in the model scale reproduction of the real-world Draupner wave.By comparing the motions,vertical wave bending moment,green water column and slamming pressures it is concluded that the breather solutions are a powerful and efficient tool for the generation of design extreme waves of certain critical wave lengths for wave/structure investigations on different subjects.
