With the rapid advancement of quantum computing,hybrid quantum–classical machine learning has shown numerous potential applications at the current stage,with expectations of being achievable in the noisy intermediate...With the rapid advancement of quantum computing,hybrid quantum–classical machine learning has shown numerous potential applications at the current stage,with expectations of being achievable in the noisy intermediate-scale quantum(NISQ)era.Quantum reinforcement learning,as an indispensable study,has recently demonstrated its ability to solve standard benchmark environments with formally provable theoretical advantages over classical counterparts.However,despite the progress of quantum processors and the emergence of quantum computing clouds,implementing quantum reinforcement learning algorithms utilizing parameterized quantum circuits(PQCs)on NISQ devices remains infrequent.In this work,we take the first step towards executing benchmark quantum reinforcement problems on real devices equipped with at most 136 qubits on the BAQIS Quafu quantum computing cloud.The experimental results demonstrate that the policy agents can successfully accomplish objectives under modified conditions in both the training and inference phases.Moreover,we design hardware-efficient PQC architectures in the quantum model using a multi-objective evolutionary algorithm and develop a learning algorithm that is adaptable to quantum devices.We hope that the Quafu-RL can be a guiding example to show how to realize machine learning tasks by taking advantage of quantum computers on the quantum cloud platform.展开更多
We introduce Quafu-Qcover,an open-source cloud-based software package developed for solving combinatorial optimization problems using quantum simulators and hardware backends.Quafu-Qcover provides a standardized and c...We introduce Quafu-Qcover,an open-source cloud-based software package developed for solving combinatorial optimization problems using quantum simulators and hardware backends.Quafu-Qcover provides a standardized and comprehensive workflow that utilizes the quantum approximate optimization algorithm(QAOA).It facilitates the automatic conversion of the original problem into a quadratic unconstrained binary optimization(QUBO)model and its corresponding Ising model,which can be subsequently transformed into a weight graph.The core of Qcover relies on a graph decomposition-based classical algorithm,which efficiently derives the optimal parameters for the shallow QAOA circuit.Quafu-Qcover incorporates a dedicated compiler capable of translating QAOA circuits into physical quantum circuits that can be executed on Quafu cloud quantum computers.Compared to a general-purpose compiler,our compiler demonstrates the ability to generate shorter circuit depths,while also exhibiting superior speed performance.Additionally,the Qcover compiler has the capability to dynamically create a library of qubits coupling substructures in real-time,utilizing the most recent calibration data from the superconducting quantum devices.This ensures that computational tasks can be assigned to connected physical qubits with the highest fidelity.The Quafu-Qcover allows us to retrieve quantum computing sampling results using a task ID at any time,enabling asynchronous processing.Moreover,it incorporates modules for results preprocessing and visualization,facilitating an intuitive display of solutions for combinatorial optimization problems.We hope that Quafu-Qcover can serve as an instructive illustration for how to explore application problems on the Quafu cloud quantum computers.展开更多
Semiconductor quantum dots have been intensively investigated because of their fundamental role in solid-state quan- tum information processing. The energy levels of quantum dots are quantized and can be tuned by exte...Semiconductor quantum dots have been intensively investigated because of their fundamental role in solid-state quan- tum information processing. The energy levels of quantum dots are quantized and can be tuned by external field such as optical, electric, and magnetic field. In this review, we focus on the development of magneto-optical properties of single InAs quantum dots embedded in GaAs matrix, including charge injection, relaxation, tunneling, wavefunction distribution, and coupling between different dimensional materials. Finally, the perspective of coherent manipulation of quantum state of single self-assembled quantum dots by photocurrent spectroscopy with an applied magnetic field is discussed.展开更多
We demonstrate the in situ growth of ultra-thin InA s nanowires with an epitaxial Al film by molecular-beam epitaxy.Our InAs nanowire diameter(~30 nm)is much thinner than before(~100 nm).The ultra-thin InAs nanowires ...We demonstrate the in situ growth of ultra-thin InA s nanowires with an epitaxial Al film by molecular-beam epitaxy.Our InAs nanowire diameter(~30 nm)is much thinner than before(~100 nm).The ultra-thin InAs nanowires are pure phase crystals for various different growth directions.Transmission electron microscopy confirms an atomically abrupt and uniform interface between the Al shell and the InAs wire.Quantum transport study on these devices resolves a hard induced superconducting gap and 2 e-periodic Coulomb blockade at zero magnetic field,a necessary step for future Majorana experiments.By reducing wire diameter,our work presents a promising route for reaching fewer sub-band regime in Major ana nanowire devices.展开更多
This review summarizes the requirement of low temperature conditions in existing experimental approaches to quantum computation and quantum simulation.
We propose a new method to construct low-dimensional quantum devices consisting of the magnetic topological insulators.Unlike previous systems based on locally depleting two-dimensional electron gas in semiconductor h...We propose a new method to construct low-dimensional quantum devices consisting of the magnetic topological insulators.Unlike previous systems based on locally depleting two-dimensional electron gas in semiconductor heterojunctions,magnetization provides a simpler and rewriteable fabrication way.The motion of electrons can be manipulated through the domain wall formed by the boundary between different magnetic domains.Here,three devices designed by local magnetization are presented.For the quantum point contact,conductance exhibits quantized plateaus with the increasing silt width between two magnetic domains.For the quantum dot,conductance shows pronounced peaks as the change of gate voltage.Finally,for the Aharonov–Bohm ring,conductance oscillates periodically with the external magnetic field.Numerical results show that the transport of these local magnetization systems is identical to that of the previous systems based on depleting two-dimensional electron gas,and the only difference is the approach of construction.These findings may pave the way for realization of low-power-consumption devices based on magnetic domain walls.展开更多
The past few decades have witnessed a great endeavor in the search for quantum spin liquids(QSLs).;This phase of matter,which features long-ranged quantum entanglement and fractionalized spin excitations,is beyond Lan...The past few decades have witnessed a great endeavor in the search for quantum spin liquids(QSLs).;This phase of matter,which features long-ranged quantum entanglement and fractionalized spin excitations,is beyond Landau’s symmetrybreaking paradigm and is naturally associated with the celebrated idea of resonating valence bond(RVB).;What is more,high-temperature superconductivity was proposed to emerge from doping such an RVB state.展开更多
We report the magnetoresistance(MR),de Haas-van Alphen(dHvA) oscillations and the electronic structures of single-crystal PtGa.The large unsaturated MR is observed with the magnetic field B ‖ [111].Evident dHvA oscil...We report the magnetoresistance(MR),de Haas-van Alphen(dHvA) oscillations and the electronic structures of single-crystal PtGa.The large unsaturated MR is observed with the magnetic field B ‖ [111].Evident dHvA oscillations with the B ‖ [001] configuration are observed,from which twelve fundamental frequencies are extracted and the spin-orbit coupling(SOC) induced band splitting is revealed.The light cyclotron effective masses are extracted from the fitting by the thermal damping term of the Lifshitz-Kosevich formula.Combining with the calculated frequencies from the first-principles calculations,the dHvA frequencies F1/F3 and F11/F12are confirmed to originate from the electron pockets at F and R,respectively.The first-principles calculations also reveal the existence of spin-3/2 Rarita-Schwinger-Weyl fermions and time-reversal doubling of the spin-1 excitation at Γ and R with large Chern numbers of ±4 when SOC is included.展开更多
Angle-resolved photoemission spectroscopy(ARPES)and torque magnetometry(TM)measurements have been carried out to study the electronic structures of a correlated topological insulator(TI)candidate Yb B6.We observed cle...Angle-resolved photoemission spectroscopy(ARPES)and torque magnetometry(TM)measurements have been carried out to study the electronic structures of a correlated topological insulator(TI)candidate Yb B6.We observed clear surface states on the[001]surface centered at theГ^- and М^- points of the surface Brillouin zone.Interestingly,the fermiology revealed by the quantum oscillation of TM measurements agrees excellently with ARPES measurements.Moreover,the band structures we observed suggest that the band inversion in Yb B6 happens between the Yb5 dand B2bands,instead of the Yb5dand Yb4fbands as suggested by previous theoretical investigation,which will help settle the heavy debate regarding the topological nature of samarium/ytterbium hexaborides.展开更多
We studied the dynamic correlations of non-integrable systems with quantum many-body scar(QMBS)states generated by a ladder operator.The ladder operator's spectral function has an exact δ-function peak induced by...We studied the dynamic correlations of non-integrable systems with quantum many-body scar(QMBS)states generated by a ladder operator.The ladder operator's spectral function has an exact δ-function peak induced by the QMBS states.As a concrete example,we show that in the one-dimensional(1D)spin-1 Affleck-Kennedy-Lieb-Tasaki model,the spectral function of two-magnon excitations exhibits a characteristic bowtie shape composed of aδ-function resonance peak at momentum k=π and a continuum spectrum elsewhere.The two-magnon excitations can be observed via resonant inelastic X-ray scattering spectroscopy on quasi-1D nickelates and other spin-1 antiferromagnetic materials.Therefore,the findings of this study pave the way for detecting(approximate)QMBS states in realistic materials.展开更多
Harnessing the potential of graphite is key to fast charging at 4C(fully charged within 15 minutes)for electric vehicles.However,graphite is subject to lithium dendrite growth during charging,leading to short circuits...Harnessing the potential of graphite is key to fast charging at 4C(fully charged within 15 minutes)for electric vehicles.However,graphite is subject to lithium dendrite growth during charging,leading to short circuits and battery failures,which is one of the biggest problems for batteries[1-4].Therefore,quickly identifying the lithium dendrites and different types of dendrites on the graphite surface can quickly help analyze the state of graphite and design good charging protocols.展开更多
We report a fabrication process and characterization of the Josephson parametric amplifier(JPA) for the single-shot quantum state measurement of superconducting multiqubit system. The device is prepared using Nb film ...We report a fabrication process and characterization of the Josephson parametric amplifier(JPA) for the single-shot quantum state measurement of superconducting multiqubit system. The device is prepared using Nb film as its base layer,which is convenient in the sample patterning process like e-beam lithography and film etching. Our results show that the JPA has a bandwidth up to 600 MHz with gain above 15 dB and noise temperature approaching the quantum limit. The qubit state differentiation measurements demonstrate the signal-to-noise ratio around 3 and the readout fidelity above 97%and 91% for the ground and first-excited states, respectively.展开更多
Recently,intrinsic antiferromagnetic topological insulator MnBi_(2)Te_(4) has drawn intense research interest and leads to plenty of significant progress in physics and materials science by hosting quantum anomalous H...Recently,intrinsic antiferromagnetic topological insulator MnBi_(2)Te_(4) has drawn intense research interest and leads to plenty of significant progress in physics and materials science by hosting quantum anomalous Hall effect,axion insulator state,and other quantum phases.An essential ingredient to realize these quantum states is the magnetic gap in the topological surface states induced by the out-of-plane ferromagnetism on the surface of MnBi_(2)Te_(4).However,the experimental observations of the surface gap remain controversial.Here,we report the observation of the surface gap via the point contact tunneling spectroscopy.In agreement with theoretical calculations,the gap size is around 50 me V,which vanishes as the sample becomes paramagnetic with increasing temperature.The magnetoresistance hysteresis is detected through the point contact junction on the sample surface with an out-of-plane magnetic field,substantiating the surface ferromagnetism.Furthermore,the non-zero transport spin polarization coming from the ferromagnetism is determined by the point contact Andreev reflection spectroscopy.Combining these results,the magnetism-induced gap in topological surface states of MnBi_(2)Te_(4) is revealed.展开更多
We report the experimental investigation of the superconductor-metal quantum phase transition of the Eu O/KTa O3 interface.Around the transition,a divergence of the dynamical critical exponent is observed,which suppor...We report the experimental investigation of the superconductor-metal quantum phase transition of the Eu O/KTa O3 interface.Around the transition,a divergence of the dynamical critical exponent is observed,which supports the quantum Griffiths singularity in the Eu O/KTa O3 interface.The quantum Griffiths singularity could be attributed to large rare superconducting regions and quenched disorders at the interface.Our results could pave the way for studying the exotic superconducting properties at the Eu O/KTa O3 interface.展开更多
Two-dimensional(2D)transition metal dichalcogenides(TMDs)have attracted considerable attention because of their unique properties and great potential in nano-technology applications.Great efforts have been devoted to ...Two-dimensional(2D)transition metal dichalcogenides(TMDs)have attracted considerable attention because of their unique properties and great potential in nano-technology applications.Great efforts have been devoted to fabrication of novel structured TMD monolayers by modifying their pristine structures at the atomic level.Here we propose an intriguing structured 1T-PtTe2 monolayer as hydrogen evolution reaction(HER)catalyst,namely,Pt4Te7,using first-principles calculations.It is found that Pt4Te7 is a stable monolayer material verified by the calculation of formation energy,phonon dispersion,and ab initio molecular dynamics simulations.Remarkably,the novel structured void-containing monolayer exhibits superior catalytic activity toward HER compared with the pristine one,with a Gibbs free energy very close to zero(less than 0.07 eV).These features indicate that Pt4Te7 monolayer is a high-performance HER catalyst with a high platinum utilization.These findings open new perspectives for the functionalization of 2D TMD materials at an atomic level and its application in HER catalysis.展开更多
Recently,a contact-resistance-measurement method was developed to detect the minigap,hence the Andreev bound states(ABSs),in Josephson junctions constructed on the surface of three-dimensional topological insulators(3...Recently,a contact-resistance-measurement method was developed to detect the minigap,hence the Andreev bound states(ABSs),in Josephson junctions constructed on the surface of three-dimensional topological insulators(3D TIs).In this work,we further generalize that method to the circumstance with radio frequency(rf)irradiation.We find that with the increase of the rf power,the measured minigap becomes broadened and extends to higher energies in a way similar to the rf power dependence of the outer border of the Shapiro step region.We show that the corresponding data of contact resistance under rf irradiation can be well interpreted by using the resistively shunted Josephson junction(RSJ)model and the Blonder–Tinkham–Klapwijk(BTK)theory.Our findings could be useful when using the contact-resistancemeasurement method to study the Majorana-related physics in topological insulator-based Josephson junctions under rf irradiation.展开更多
We investigate nonlocal advantage of quantum coherence(NAQC)in a correlated dephasing channel modeled by themultimode bosonic reservoir.We obtain analytically the dephasing and memory factors of this channel for the r...We investigate nonlocal advantage of quantum coherence(NAQC)in a correlated dephasing channel modeled by themultimode bosonic reservoir.We obtain analytically the dephasing and memory factors of this channel for the reservoirhaving a Lorentzian spectral density,and analyze how they affect the NAQC defined by the l1 norm and relative entropy.It is shown that the memory effects of this channel on NAQC are state-dependent,and they suppress noticeably the rapiddecay of NAQC for the family of input Bell-like states with one excitation.For the given transmission time of each qubit,we also obtain the regions of the dephasing and memory factors during which there is NAQC in the output states.展开更多
Superlattice potentials are theoretically predicted to modify the single-particle electronic structures. The resulting Coulomb-interaction-dominated low-energy physics would generate highly novel many-body phenomena. ...Superlattice potentials are theoretically predicted to modify the single-particle electronic structures. The resulting Coulomb-interaction-dominated low-energy physics would generate highly novel many-body phenomena. Here,by in situ tunneling spectroscopy, we show the signatures of superstructure-modulated correlated electron states in epitaxial bilayer graphene(BLG) on 6H-Si C(0001). As the carrier density is locally quasi-‘tuned’ by the superlattice potentials of a 6 × 6 interface reconstruction phase, the spectral-weight transfer occurs between the two broad peaks flanking the charge-neutral point. Such a detected non-rigid band shift beyond the single-particle band description implies the existence of correlation effects, probably attributed to the modified interlayer coupling in epitaxial BLG by the 6×6 reconstruction as in magic-angle BLG by the moiré potentials. Quantitative analysis suggests that the intrinsic interface reconstruction shows a high carrier tunability of ~1/2 filling range, equivalent to the back gating by a voltage of ~70 V in a typical gated BLG/SiO_(2)/Si device. The finding in interfacemodulated epitaxial BLG with reconstruction phase extends the BLG platform with electron correlations beyond the magic-angle situation, and may stimulate further investigations on correlated states in graphene systems and other van der Waals materials.展开更多
We theoretically study the Josephson effect in a quantum anomalous Hall insulator(QAHI)nanoribbon with a domain wall structure and covered by the superconductor.The anomalous Josephson current,the nonzero supercurrent...We theoretically study the Josephson effect in a quantum anomalous Hall insulator(QAHI)nanoribbon with a domain wall structure and covered by the superconductor.The anomalous Josephson current,the nonzero supercurrent at the zero superconducting phase difference,appears with the nonzero magnetization and the suitable azimuth angle of the domain wall.Dependent on the configuration of the domain wall,the anomalous current peaks in the Bloch type but disappears in the Néel type because the y-component of magnetization is necessary to break symmetry to arouse the anomalous current.The phase shift of the anomalous current is tunable by the magnetization,the azimuth angle,or the thickness of the domain wall.By introducing a bare QAHI region in the middle of the junction which is not covered by the superconductor,the anomalous Josephson effect is enhanced such that the phase shift can exceedπ.Thus,a continuous change between 0 andπjunctions is realized via regulating the configuration of the domain wall or the magnetization strength.As long as an s-wave superconductor is placed on the top of the QAHI with a domain wall structure,this proposal can be experimentally fabricated and useful for the phase battery or superconducting quantum bit.展开更多
Fractional quantum Hall systems are often described by model wave functions,which are the ground states of pure systems with short-range interaction.A primary example is the Laughlin wave function,which supports Abeli...Fractional quantum Hall systems are often described by model wave functions,which are the ground states of pure systems with short-range interaction.A primary example is the Laughlin wave function,which supports Abelian quasiparticles with fractionalized charge.In the presence of disorder,the wave function of the ground state is expected to deviate from the Laughlin form.We study the disorder-driven colla.pse of the quantum Hall state by analyzing the evolution of the ground state and the single-quasihole state.In particular,we demonstrate that the quasihole tunneling amplitude can signal the fractional quantum Hall phase to insulator transition.展开更多
基金supported by the Beijing Academy of Quantum Information Sciencessupported by the National Natural Science Foundation of China(Grant No.92365206)+2 种基金the support of the China Postdoctoral Science Foundation(Certificate Number:2023M740272)supported by the National Natural Science Foundation of China(Grant No.12247168)China Postdoctoral Science Foundation(Certificate Number:2022TQ0036)。
文摘With the rapid advancement of quantum computing,hybrid quantum–classical machine learning has shown numerous potential applications at the current stage,with expectations of being achievable in the noisy intermediate-scale quantum(NISQ)era.Quantum reinforcement learning,as an indispensable study,has recently demonstrated its ability to solve standard benchmark environments with formally provable theoretical advantages over classical counterparts.However,despite the progress of quantum processors and the emergence of quantum computing clouds,implementing quantum reinforcement learning algorithms utilizing parameterized quantum circuits(PQCs)on NISQ devices remains infrequent.In this work,we take the first step towards executing benchmark quantum reinforcement problems on real devices equipped with at most 136 qubits on the BAQIS Quafu quantum computing cloud.The experimental results demonstrate that the policy agents can successfully accomplish objectives under modified conditions in both the training and inference phases.Moreover,we design hardware-efficient PQC architectures in the quantum model using a multi-objective evolutionary algorithm and develop a learning algorithm that is adaptable to quantum devices.We hope that the Quafu-RL can be a guiding example to show how to realize machine learning tasks by taking advantage of quantum computers on the quantum cloud platform.
基金supported by the National Natural Science Foundation of China(Grant No.92365206)the support of the China Postdoctoral Science Foundation(Certificate Number:2023M740272)+1 种基金supported by the National Natural Science Foundation of China(Grant No.12247168)China Postdoctoral Science Foundation(Certificate Number:2022TQ0036)。
文摘We introduce Quafu-Qcover,an open-source cloud-based software package developed for solving combinatorial optimization problems using quantum simulators and hardware backends.Quafu-Qcover provides a standardized and comprehensive workflow that utilizes the quantum approximate optimization algorithm(QAOA).It facilitates the automatic conversion of the original problem into a quadratic unconstrained binary optimization(QUBO)model and its corresponding Ising model,which can be subsequently transformed into a weight graph.The core of Qcover relies on a graph decomposition-based classical algorithm,which efficiently derives the optimal parameters for the shallow QAOA circuit.Quafu-Qcover incorporates a dedicated compiler capable of translating QAOA circuits into physical quantum circuits that can be executed on Quafu cloud quantum computers.Compared to a general-purpose compiler,our compiler demonstrates the ability to generate shorter circuit depths,while also exhibiting superior speed performance.Additionally,the Qcover compiler has the capability to dynamically create a library of qubits coupling substructures in real-time,utilizing the most recent calibration data from the superconducting quantum devices.This ensures that computational tasks can be assigned to connected physical qubits with the highest fidelity.The Quafu-Qcover allows us to retrieve quantum computing sampling results using a task ID at any time,enabling asynchronous processing.Moreover,it incorporates modules for results preprocessing and visualization,facilitating an intuitive display of solutions for combinatorial optimization problems.We hope that Quafu-Qcover can serve as an instructive illustration for how to explore application problems on the Quafu cloud quantum computers.
基金Project supported by the National Basic Research Program of China(Grant No.2014CB921003)the National Natural Science Foundation of China(Grant Nos.11721404,51761145104,and 61675228)+1 种基金the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant Nos.XDB07030200 and XDPB0803)the CAS Interdisciplinary Innovation Team
文摘Semiconductor quantum dots have been intensively investigated because of their fundamental role in solid-state quan- tum information processing. The energy levels of quantum dots are quantized and can be tuned by external field such as optical, electric, and magnetic field. In this review, we focus on the development of magneto-optical properties of single InAs quantum dots embedded in GaAs matrix, including charge injection, relaxation, tunneling, wavefunction distribution, and coupling between different dimensional materials. Finally, the perspective of coherent manipulation of quantum state of single self-assembled quantum dots by photocurrent spectroscopy with an applied magnetic field is discussed.
基金supported by the National Natural Science Foundation of China(Grant Nos.92065106,61974138,12104053,and 11704364)the Beijing Natural Science Foundation(Grant No.1192017)+2 种基金Tsinghua University Initiative Scientifc Research Programthe support from Youth Innovation Promotion Association,Chinese Academy of Sciences(Grant No.Y2021043)China Postdoctoral Science Foundation(Grant Nos.2020M670173 and 2020T130058)。
文摘We demonstrate the in situ growth of ultra-thin InA s nanowires with an epitaxial Al film by molecular-beam epitaxy.Our InAs nanowire diameter(~30 nm)is much thinner than before(~100 nm).The ultra-thin InAs nanowires are pure phase crystals for various different growth directions.Transmission electron microscopy confirms an atomically abrupt and uniform interface between the Al shell and the InAs wire.Quantum transport study on these devices resolves a hard induced superconducting gap and 2 e-periodic Coulomb blockade at zero magnetic field,a necessary step for future Majorana experiments.By reducing wire diameter,our work presents a promising route for reaching fewer sub-band regime in Major ana nanowire devices.
基金Project supported by the National Key Research and Development Program of China(Grant No.2017YFA0303301)the National Natural Science Foundation of China(Grant Nos.11674009 and 11921005)+1 种基金the Beijing Natural Science Foundation,China(Grant No.JQ18002)the Strategic Priority Research Program of Chinese Academy of Sciences(Grant No.XDB28000000)。
文摘This review summarizes the requirement of low temperature conditions in existing experimental approaches to quantum computation and quantum simulation.
基金Supported by the National Key R&D Program of China(Grant No.2017YFA0303301)the National Natural Science Foundation of China(Grant Nos.11921005 and 11574007)+1 种基金the Strategic Priority Research Program of Chinese Academy of Sciences(Grant No.XDB28000000)Beijing Municipal Science and Technology Commission,China(Grant No.Z191100007219013).
文摘We propose a new method to construct low-dimensional quantum devices consisting of the magnetic topological insulators.Unlike previous systems based on locally depleting two-dimensional electron gas in semiconductor heterojunctions,magnetization provides a simpler and rewriteable fabrication way.The motion of electrons can be manipulated through the domain wall formed by the boundary between different magnetic domains.Here,three devices designed by local magnetization are presented.For the quantum point contact,conductance exhibits quantized plateaus with the increasing silt width between two magnetic domains.For the quantum dot,conductance shows pronounced peaks as the change of gate voltage.Finally,for the Aharonov–Bohm ring,conductance oscillates periodically with the external magnetic field.Numerical results show that the transport of these local magnetization systems is identical to that of the previous systems based on depleting two-dimensional electron gas,and the only difference is the approach of construction.These findings may pave the way for realization of low-power-consumption devices based on magnetic domain walls.
文摘The past few decades have witnessed a great endeavor in the search for quantum spin liquids(QSLs).;This phase of matter,which features long-ranged quantum entanglement and fractionalized spin excitations,is beyond Landau’s symmetrybreaking paradigm and is naturally associated with the celebrated idea of resonating valence bond(RVB).;What is more,high-temperature superconductivity was proposed to emerge from doping such an RVB state.
基金Supported by the National Key Research and Development Program of China(Grant Nos.2019YFA0308602, 2018YFA0305700 and 2016YFA0300600)the National Natural Science Foundation of China(Grant Nos.11874422 and 11574391)+6 种基金the Fundamental Research Funds for the Central Universitiesthe Research Funds of Renmin University of China(Grant Nos.19XNLG18 and 18 XNLG14)the Chinese Academy of Sciences(Grant No.XDB28000000)the Science Challenge Project(Grant No.TZ2016004)the K.C.Wong Education Foundation(Grant No.GJTD-2018-01)the Beijing Municipal Science&Technology Commission(Grant No.Z181100004218001)the Beijing Natural Science Foundation(Grant No.Z180008)
文摘We report the magnetoresistance(MR),de Haas-van Alphen(dHvA) oscillations and the electronic structures of single-crystal PtGa.The large unsaturated MR is observed with the magnetic field B ‖ [111].Evident dHvA oscillations with the B ‖ [001] configuration are observed,from which twelve fundamental frequencies are extracted and the spin-orbit coupling(SOC) induced band splitting is revealed.The light cyclotron effective masses are extracted from the fitting by the thermal damping term of the Lifshitz-Kosevich formula.Combining with the calculated frequencies from the first-principles calculations,the dHvA frequencies F1/F3 and F11/F12are confirmed to originate from the electron pockets at F and R,respectively.The first-principles calculations also reveal the existence of spin-3/2 Rarita-Schwinger-Weyl fermions and time-reversal doubling of the spin-1 excitation at Γ and R with large Chern numbers of ±4 when SOC is included.
基金supported by the National Natural Science Foundation of China (Grant Nos. 11774190, 11674229, 11634009, and 11774427)the National Key R&D Program of China (Grant Nos. 2017YFA0304600 and 2017YFA0305400)+5 种基金support from the EPSRC (UK) grant EP/K04074X/1 and a DARPA (US) MESO project (No. N66001-11-1-4105)supported by the Office of Naval Research through the National Science Foundation under Award No. DMR-1707620 (magnetization measurement)supported by the Office of Basic Energy Sciences of the U.S. Department of Energy (DE-AC0205CH11231)SIMES and SLAC National Accelerator Laboratory is supported by the Office of Basic Energy Sciences of the U.S. Department of Energy (DE-AC0276SF00515)Nanjing University is supported by the National Basic Research Program of China (Grant No. 51002074)the National Basic Research of China (Grant Nos. 2012CB921503 and 2012CB632702)
文摘Angle-resolved photoemission spectroscopy(ARPES)and torque magnetometry(TM)measurements have been carried out to study the electronic structures of a correlated topological insulator(TI)candidate Yb B6.We observed clear surface states on the[001]surface centered at theГ^- and М^- points of the surface Brillouin zone.Interestingly,the fermiology revealed by the quantum oscillation of TM measurements agrees excellently with ARPES measurements.Moreover,the band structures we observed suggest that the band inversion in Yb B6 happens between the Yb5 dand B2bands,instead of the Yb5dand Yb4fbands as suggested by previous theoretical investigation,which will help settle the heavy debate regarding the topological nature of samarium/ytterbium hexaborides.
基金supported by the National Natural Science Foundation of China(Grant No.12174387)the Chinese Academy of Sciences(Grant Nos.YSBR-057 and JZHKYPT-2021-08)the Innovative Program for Quantum Science and Technology(Grant No.2021ZD0302600)。
文摘We studied the dynamic correlations of non-integrable systems with quantum many-body scar(QMBS)states generated by a ladder operator.The ladder operator's spectral function has an exact δ-function peak induced by the QMBS states.As a concrete example,we show that in the one-dimensional(1D)spin-1 Affleck-Kennedy-Lieb-Tasaki model,the spectral function of two-magnon excitations exhibits a characteristic bowtie shape composed of aδ-function resonance peak at momentum k=π and a continuum spectrum elsewhere.The two-magnon excitations can be observed via resonant inelastic X-ray scattering spectroscopy on quasi-1D nickelates and other spin-1 antiferromagnetic materials.Therefore,the findings of this study pave the way for detecting(approximate)QMBS states in realistic materials.
文摘Harnessing the potential of graphite is key to fast charging at 4C(fully charged within 15 minutes)for electric vehicles.However,graphite is subject to lithium dendrite growth during charging,leading to short circuits and battery failures,which is one of the biggest problems for batteries[1-4].Therefore,quickly identifying the lithium dendrites and different types of dendrites on the graphite surface can quickly help analyze the state of graphite and design good charging protocols.
基金Project supported by the Science Funds from the Ministry of Science and Technology of China(Grant Nos.2015CB921104 and 2016YFA0300601)the National Natural Science Foundation of China(Grant Nos.11674380 and 11874063)+1 种基金the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant Nos.XDB07010300 and XDB28000000)the Key Research and Development Program of Guangdong Province,China(Grant No.2018B030326001)
文摘We report a fabrication process and characterization of the Josephson parametric amplifier(JPA) for the single-shot quantum state measurement of superconducting multiqubit system. The device is prepared using Nb film as its base layer,which is convenient in the sample patterning process like e-beam lithography and film etching. Our results show that the JPA has a bandwidth up to 600 MHz with gain above 15 dB and noise temperature approaching the quantum limit. The qubit state differentiation measurements demonstrate the signal-to-noise ratio around 3 and the readout fidelity above 97%and 91% for the ground and first-excited states, respectively.
基金Supported by the National Key Research and Development Program of China (Grant Nos. 2017YFA0303302,2018YFA0305604,2018YFA0307100)the National Natural Science Foundation of China (Grant Nos. 11888101,11774008,11704279,11874035,51788104)+2 种基金the Strategic Priority Research Program of Chinese Academy of Sciences (Grant No. XDB28000000)the Beijing Natural Science Foundation (Grant Nos. Z180010 and 1202005)the Open Research Fund Program of the State Key Laboratory of Low-Dimensional Quantum Physics,Tsinghua University (Grant No. KF202001)
文摘Recently,intrinsic antiferromagnetic topological insulator MnBi_(2)Te_(4) has drawn intense research interest and leads to plenty of significant progress in physics and materials science by hosting quantum anomalous Hall effect,axion insulator state,and other quantum phases.An essential ingredient to realize these quantum states is the magnetic gap in the topological surface states induced by the out-of-plane ferromagnetism on the surface of MnBi_(2)Te_(4).However,the experimental observations of the surface gap remain controversial.Here,we report the observation of the surface gap via the point contact tunneling spectroscopy.In agreement with theoretical calculations,the gap size is around 50 me V,which vanishes as the sample becomes paramagnetic with increasing temperature.The magnetoresistance hysteresis is detected through the point contact junction on the sample surface with an out-of-plane magnetic field,substantiating the surface ferromagnetism.Furthermore,the non-zero transport spin polarization coming from the ferromagnetism is determined by the point contact Andreev reflection spectroscopy.Combining these results,the magnetism-induced gap in topological surface states of MnBi_(2)Te_(4) is revealed.
基金Supported by the National Key R&D Program of China(Grant Nos.2019YFA0308401 and 2017YFA0303301)the National Natural Science Foundation of China(Grant Nos.11974025,11674009,and 11934016)+1 种基金the Beijing Natural Science Foundation(Grant No.1192009)the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB28000000)。
文摘We report the experimental investigation of the superconductor-metal quantum phase transition of the Eu O/KTa O3 interface.Around the transition,a divergence of the dynamical critical exponent is observed,which supports the quantum Griffiths singularity in the Eu O/KTa O3 interface.The quantum Griffiths singularity could be attributed to large rare superconducting regions and quenched disorders at the interface.Our results could pave the way for studying the exotic superconducting properties at the Eu O/KTa O3 interface.
基金Project supported by the National Key R&D Program of China(Grant Nos.2016YFA0202300,2018YFA0305800,and 2019YFA0308500)the National Natural Science Foundation of China(Grant Nos.61888102,51872284,and 51922011)the Strategic Priority Research Program of Chinese Academy of Sciences(Grant No.XDB30000000).
文摘Two-dimensional(2D)transition metal dichalcogenides(TMDs)have attracted considerable attention because of their unique properties and great potential in nano-technology applications.Great efforts have been devoted to fabrication of novel structured TMD monolayers by modifying their pristine structures at the atomic level.Here we propose an intriguing structured 1T-PtTe2 monolayer as hydrogen evolution reaction(HER)catalyst,namely,Pt4Te7,using first-principles calculations.It is found that Pt4Te7 is a stable monolayer material verified by the calculation of formation energy,phonon dispersion,and ab initio molecular dynamics simulations.Remarkably,the novel structured void-containing monolayer exhibits superior catalytic activity toward HER compared with the pristine one,with a Gibbs free energy very close to zero(less than 0.07 eV).These features indicate that Pt4Te7 monolayer is a high-performance HER catalyst with a high platinum utilization.These findings open new perspectives for the functionalization of 2D TMD materials at an atomic level and its application in HER catalysis.
基金Project supported by the National Basic Research Program of China(Grant Nos.2016YFA0300601,2017YFA0304700,and 2015CB921402)the National Natural Science Foundation China(Grant Nos.11527806,91221203,11174357,91421303,and 11774405)+1 种基金the Strategic Priority Research Program B of the Chinese Academy of Sciences(Grant Nos.XDB07010100 and XDB28000000)the Beijing Municipal Science&Technology Commission,China(Grant No.Z191100007219008)
文摘Recently,a contact-resistance-measurement method was developed to detect the minigap,hence the Andreev bound states(ABSs),in Josephson junctions constructed on the surface of three-dimensional topological insulators(3D TIs).In this work,we further generalize that method to the circumstance with radio frequency(rf)irradiation.We find that with the increase of the rf power,the measured minigap becomes broadened and extends to higher energies in a way similar to the rf power dependence of the outer border of the Shapiro step region.We show that the corresponding data of contact resistance under rf irradiation can be well interpreted by using the resistively shunted Josephson junction(RSJ)model and the Blonder–Tinkham–Klapwijk(BTK)theory.Our findings could be useful when using the contact-resistancemeasurement method to study the Majorana-related physics in topological insulator-based Josephson junctions under rf irradiation.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11675129,11774406,and 11934018)the National Key R&D Program of China(Grant Nos.2016YFA0302104 and 2016YFA0300600)+1 种基金the Strategic Priority Research Program of Chinese Academy of Sciences(Grant No.XDB28000000)the Research Program of Beijing Academy of Quantum Information Sciences(Grant No.Y18G07).
文摘We investigate nonlocal advantage of quantum coherence(NAQC)in a correlated dephasing channel modeled by themultimode bosonic reservoir.We obtain analytically the dephasing and memory factors of this channel for the reservoirhaving a Lorentzian spectral density,and analyze how they affect the NAQC defined by the l1 norm and relative entropy.It is shown that the memory effects of this channel on NAQC are state-dependent,and they suppress noticeably the rapiddecay of NAQC for the family of input Bell-like states with one excitation.For the given transmission time of each qubit,we also obtain the regions of the dephasing and memory factors during which there is NAQC in the output states.
基金supported by the National Natural Science Foundation of China (Grant Nos. 11888101 and 11774008)the National Key R&D Program of China (Grant Nos. 2018YFA0305604 and 2017YFA0303302)+1 种基金the Beijing Natural Science Foundation (Grant No. Z180010)the Strategic Priority Research Program of Chinese Academy of Sciences (Grant No. XDB28000000)。
文摘Superlattice potentials are theoretically predicted to modify the single-particle electronic structures. The resulting Coulomb-interaction-dominated low-energy physics would generate highly novel many-body phenomena. Here,by in situ tunneling spectroscopy, we show the signatures of superstructure-modulated correlated electron states in epitaxial bilayer graphene(BLG) on 6H-Si C(0001). As the carrier density is locally quasi-‘tuned’ by the superlattice potentials of a 6 × 6 interface reconstruction phase, the spectral-weight transfer occurs between the two broad peaks flanking the charge-neutral point. Such a detected non-rigid band shift beyond the single-particle band description implies the existence of correlation effects, probably attributed to the modified interlayer coupling in epitaxial BLG by the 6×6 reconstruction as in magic-angle BLG by the moiré potentials. Quantitative analysis suggests that the intrinsic interface reconstruction shows a high carrier tunability of ~1/2 filling range, equivalent to the back gating by a voltage of ~70 V in a typical gated BLG/SiO_(2)/Si device. The finding in interfacemodulated epitaxial BLG with reconstruction phase extends the BLG platform with electron correlations beyond the magic-angle situation, and may stimulate further investigations on correlated states in graphene systems and other van der Waals materials.
基金Project supported by the National Key R&D Program of China(Grant No.2017YFA0303301)the National Natural Science Foundation of China(Grant Nos.11921005 and 11574007)+1 种基金the Strategic Priority Research Program of Chinese Academy of Sciences(Grant No.XDB28000000)Beijing Municipal Science&Technology Commission,China(Grant No.Z191100007219013).
文摘We theoretically study the Josephson effect in a quantum anomalous Hall insulator(QAHI)nanoribbon with a domain wall structure and covered by the superconductor.The anomalous Josephson current,the nonzero supercurrent at the zero superconducting phase difference,appears with the nonzero magnetization and the suitable azimuth angle of the domain wall.Dependent on the configuration of the domain wall,the anomalous current peaks in the Bloch type but disappears in the Néel type because the y-component of magnetization is necessary to break symmetry to arouse the anomalous current.The phase shift of the anomalous current is tunable by the magnetization,the azimuth angle,or the thickness of the domain wall.By introducing a bare QAHI region in the middle of the junction which is not covered by the superconductor,the anomalous Josephson effect is enhanced such that the phase shift can exceedπ.Thus,a continuous change between 0 andπjunctions is realized via regulating the configuration of the domain wall or the magnetization strength.As long as an s-wave superconductor is placed on the top of the QAHI with a domain wall structure,this proposal can be experimentally fabricated and useful for the phase battery or superconducting quantum bit.
基金Supported by the National Natural Science Foundation of China under Grant No 11674282the Strategic Priority Research Program of Chinese Academy of Sciences under Grant No XDB28000000the National Basic Research Program of China under Grant No 2015CB921101
文摘Fractional quantum Hall systems are often described by model wave functions,which are the ground states of pure systems with short-range interaction.A primary example is the Laughlin wave function,which supports Abelian quasiparticles with fractionalized charge.In the presence of disorder,the wave function of the ground state is expected to deviate from the Laughlin form.We study the disorder-driven colla.pse of the quantum Hall state by analyzing the evolution of the ground state and the single-quasihole state.In particular,we demonstrate that the quasihole tunneling amplitude can signal the fractional quantum Hall phase to insulator transition.
