The poor interfacial stability not only deteriorates fibre lithium-ion batteries(FLBs)performance but also impacts their scalable applications.To efficiently address these challenges,Prof.Huisheng Peng team proposed a...The poor interfacial stability not only deteriorates fibre lithium-ion batteries(FLBs)performance but also impacts their scalable applications.To efficiently address these challenges,Prof.Huisheng Peng team proposed a generalized channel structures strategy with optimized in situ polymerization technology in their recent study.The resultant FLBs can be woven into different-sized powering textiles,providing a high energy density output of 128 Wh kg^(-1) and simultaneously demonstrating good durability even under harsh conditions.Such a promising strategy expands the horizon in developing FLB with particular polymer gel electrolytes,and significantly ever-deepening understanding of the scaled wearable energy textile system toward a sustainable future.展开更多
Over the last decade,remarkable progress has been made in metal halide perovskite solar cells(PSCs),which have been a focus of emerging photovoltaic techniques and show great potential for commercialization.However,th...Over the last decade,remarkable progress has been made in metal halide perovskite solar cells(PSCs),which have been a focus of emerging photovoltaic techniques and show great potential for commercialization.However,the upscaling of small-area PSCs to large-area solar modules to meet the demands of practical applications remains a significant challenge.The scalable production of high-quality perovskite films by a simple,reproducible process is crucial for resolving this issue.Furthermore,the crystallization behavior in the solution-processed fabrication of perovskite films can be strongly influenced by the physicochemical properties of the precursor inks,which are significantly affected by the employed solvents and their interactions with the solutes.Thus,a comprehensive understanding of solvent engineering for fabricating perovskite films over large areas is urgently required.In this paper,we first analyze the role of solvents in the solution-processed fabrication of large-area perovskite films based on the classical crystal nucleation and growth mechanism.Recent efforts in solvent engineering to improve the quality of perovskite films for solar modules are discussed.Finally,the basic principles and future challenges of solvent system design for scalable fabrication of high-quality perovskite films for efficient solar modules are proposed.展开更多
Perovskite solar cells have reached a power-conversion efficiency(PCE) of 25.6%,showing great potential with reliable moisture and heat stability.Most results are achieved on small-area devices,using conventional thin...Perovskite solar cells have reached a power-conversion efficiency(PCE) of 25.6%,showing great potential with reliable moisture and heat stability.Most results are achieved on small-area devices,using conventional thin-film processing technologies like spin-coating method.However,such approaches may not be upscaled for large-area substrates.Thus,strategies and materials need to be developed for manufacturing processing routes to realize future commercial photovoltaic fabrications.Notable results have been achieved on large-area perovskite solar cells.In this review,similarities and differences of large-area perovskite fabrication mechanisms between the various pathways are investigated,especially on the parameters affecting the nucleation and crystal growth kinetics.Moreover,the methods for large-area transporting layers and electrodes are discussed,and some key issues from cells to modules.Challenges and opportunities are proposed to pave the way of high-efficiency perovskite solar modules.展开更多
Scalable video coding(SVC)has been widely used in video-on-demand(VOD)service,to efficiently satisfy users’different video quality requirements and dynamically adjust video stream to timevariant wireless channels.Und...Scalable video coding(SVC)has been widely used in video-on-demand(VOD)service,to efficiently satisfy users’different video quality requirements and dynamically adjust video stream to timevariant wireless channels.Under the 5G network structure,we consider a cooperative caching scheme inside each cluster with SVC to economically utilize the limited caching storage.A novel multi-agent deep reinforcement learning(MADRL)framework is proposed to jointly optimize the video access delay and users’satisfaction,where an aggregation node is introduced helping individual agents to achieve global observations and overall system rewards.Moreover,to cope with the large action space caused by the large number of videos and users,a dimension decomposition method is embedded into the neural network in each agent,which greatly reduce the computational complexity and memory cost of the reinforcement learning.Experimental results show that:1)the proposed value-decomposed dimensional network(VDDN)algorithm achieves an obvious performance gain versus the traditional MADRL;2)the proposed VDDN algorithm can handle an extremely large action space and quickly converge with a low computational complexity.展开更多
Perovskite-based solar cell technology has advanced significantly and the power conversion efficiencies are nowadays on par with commercialized photovoltaic technologies. To realize the potential of perovskite solar c...Perovskite-based solar cell technology has advanced significantly and the power conversion efficiencies are nowadays on par with commercialized photovoltaic technologies. To realize the potential of perovskite solar cells, the focus is now shifting to scalable fabrication technologies that will enable low-cost solution processing of perovskite solar cells over large areas and with high yields. This review article discusses the fundamental concerns that arise when transitioning from laboratory to large area solution coating, available scalable coating technologies, and their applicability to the fabrication of high-performance perovskite solar cells. We find that a significant amount of work has been done to test scalable coating technologies, but also that often the methods that led to highest-performing cells in the laboratory （e.g. antisolvent processing） show limited compatibility with scalable coating methods. To achieve a high-yield and low-cost process, development must emphasize a high degree of control provided by sequential conversion of perovskite films and engineering of additives that fine-tune coating properties of perovskite precursor inks.展开更多
We develop a design of a hybrid quantum interface for quantum information transfer （QIT）, adopting a nanome- chanical resonator as the intermedium, which is magnetically coupled with individual nitrogen-vacancy cent...We develop a design of a hybrid quantum interface for quantum information transfer （QIT）, adopting a nanome- chanical resonator as the intermedium, which is magnetically coupled with individual nitrogen-vacancy centers as the solid qubits, while eapacitively coupled with a coplanar waveguide resonator as the quantum data bus. We describe the Hamiltonian of the model, and analytically demonstrate the QIT for both the resonant interaction and large detuning cases. The hybrid quantum interface allows for QIT between arbitrarily selected individual nitrogen-vacancy centers, and has advantages of the sealability and controllability. Our methods open an alter- native perspective for implementing QIT, which is important during quantum storing or processing procedures in quantum computing.展开更多
A layered compression algorithm is presented which delivers spatial scalable encoded bit streams for remote video monitoring system. The complexity of the algorithm is modest and is well suited to real time implementa...A layered compression algorithm is presented which delivers spatial scalable encoded bit streams for remote video monitoring system. The complexity of the algorithm is modest and is well suited to real time implementation. Based on the layered compression algorithm, a codec system model is established. High-speed video compression can be realized with parallel data compression in this codec system. For image reconstruction, a prediction method using two nearest pix points is presented.展开更多
The emerging new services in the sixth generation(6G)communication system impose increasingly stringent requirements and challenges on video transmission.Semantic communications are envisioned as a promising solution ...The emerging new services in the sixth generation(6G)communication system impose increasingly stringent requirements and challenges on video transmission.Semantic communications are envisioned as a promising solution to these challenges.This paper provides a highly-efficient solution to video transmission by proposing a scalable semantic transmission algorithm,named scalable semantic transmission framework for video(SST-V),which jointly considers the semantic importance and channel conditions.Specifically,a semantic importance evaluation module is designed to extract more informative semantic features according to the estimated importance level,facilitating high-efficiency semantic coding.By further considering the channel condition,a cascaded learning based scalable joint semanticchannel coding algorithm is proposed,which autonomously adapts the semantic coding and channel coding strategies to the specific signalto-noise ratio(SNR).Simulation results show that SST-V achieves better video reconstruction performance,while significantly reducing the transmission overhead.展开更多
To achieve an optimal trade-off between video quality and energy efficiency in the uplink streaming of multi-user Scalable Video Coding (SVC) videos in relay-based Orthogonal Frequency Division Multiple Access (OFDMA)...To achieve an optimal trade-off between video quality and energy efficiency in the uplink streaming of multi-user Scalable Video Coding (SVC) videos in relay-based Orthogonal Frequency Division Multiple Access (OFDMA) cellular networks, a cross-layer design framework that jointly selects the Transmission Policy (TP) for SVC video frames, assigns OFDMA subcarriers, and allocates power for each subcarrier is proposed. We apply the dual decomposition method to the problem, and obtain a TP selection subproblem for each SVC video adaptation and a resource allocation subproblem of Joint Subcarrier, Relay and Power Allocation (JSRPA). A second level of dual decomposition is used to divide the JSRPA problem into independent subcarrier subproblems. The proposed Crosslayer Trade-off Optimization (CTO) algorithm is sub-distributed with significantly low complexity. A performance evaluation with typical SVC video traces demonstrates that the proposed algorithm is able to converge and efficiently achieve the optimal trade-off between the video quality and energy consumption at the MSs for uplink SVC streaming.展开更多
Electronic skins(e-skins) with an excellent sensing performance have been widely developed over the last few decades.However,wearability,biocompatibility,environmental friendliness and scalability have become new limi...Electronic skins(e-skins) with an excellent sensing performance have been widely developed over the last few decades.However,wearability,biocompatibility,environmental friendliness and scalability have become new limitations. Self-healing ability can improve the long-term robustness and reliability of e-skins. However,self-healing ability and integration are hardly balanced in classical structures of self-healable devices. Here,cellulose nanofiber/poly(vinyl alcohol)(CNF/PVA),a biocompatible moisture-inspired self-healable composite,was applied both as the binder in functional layers and the substrate. Various functional layers comprising particular carbon materials and CNF/PVA were patterned on the substrate. A planar structure was beneficial for integration,and the active self-healing ability of the functional layers endowed self-healed e-skins with a higher toughness. Water served as both the only solvent throughout the fabrication process and the trigger of the self-healing process,which avoids the pollution and bioincompatibility caused by the application of noxious additives. Our e-skins could achieve real-time monitoring of whole-body physiological signals and environmental temperature and humidity. Cross-interference between di erent external stimuli was suppressed through reasonable material selection and structural design. Combined with conventional electronics,data could be transmitted to a nearby smartphone for post-processing. This work provides a previously unexplored strategy for multifunctional e-skins with an excellent practicality.展开更多
Dynamic Controller Provisioning Problem(DCPP) is a key problem for scalable SDN. Previously, the solution to this problem focused on adapting the number of controllers and their locations with changing network conditi...Dynamic Controller Provisioning Problem(DCPP) is a key problem for scalable SDN. Previously, the solution to this problem focused on adapting the number of controllers and their locations with changing network conditions, but ignored balancing control loads via switch migration. In this paper, we study a scalable control mechanism to decide which switch and where it should be migrated for more balanced control plane, and we define it as Switch Migration Problem(SMP). The main contributions of this paper are as follows. First, we define a SDN model to describe the relation between controllers and switches from the view of loads. Based on this model, we form SMP as a Network Utility Maximization(NUM) problem with the objective of serving more requests under available control resources. Second, we design a synthesizing distributed algorithm for SMP--- Distributed Hopping Algorithm(DHA), by approximating our optimal objective via Log-Sum-Exp function. In DHA, individual controller performs algorithmic procedure independently. With the solution space F, we prove that the optimal gap caused by approximation is at most 1/βlog|F|, and DHA procedure is equal to implementation of a time-reversible Markov Chain process. Finally, the results are corroborated by several numerical simulations.展开更多
Network Functions Virtualization(NFV) is an attempt to help operators more effectively manage their networks by implementing traditional network functions embedded in specialized hardware platforms in term of virtuali...Network Functions Virtualization(NFV) is an attempt to help operators more effectively manage their networks by implementing traditional network functions embedded in specialized hardware platforms in term of virtualized software instances. But, existing novel network appliances designed for NFV infrastructure are always architected on a general-purpose x86 server, which makes the performance of network functions limited by the hosted single server. To address this challenge, we propose ApplianceB ricks, a novel NFV-enable network appliance architecture that is used to explore the way of consolidating multiple physical network functions into a clustered network appliance, which is able to improve the processing capability of NFV-enabled network appliances.展开更多
In a software-defined network, a powerful central controller provides a flexible platform for defining network traffic through the use of software. When SDN is used in a large-scale network, the logical central contro...In a software-defined network, a powerful central controller provides a flexible platform for defining network traffic through the use of software. When SDN is used in a large-scale network, the logical central controller comprises multiple physical servers, and multiple controllers must act as one to provide transparent control logic to network applications and devices. The challenge is to minimize the cost of network state distribution. To this end, we propose Distributed ZTE Elastic Network Intelligent Controller （DZENIC）, a network-control platform that supports distributed deployment and linear scale-out. A dedicated component in the DZENIC controller provides a global view of the network topology as well as the distribution of host information. The evaluation shows that balance complexity with scalability, the network state distribution needs to be strictly classified.展开更多
In recent years,perovskite solar cells(PSCs)have garnered significant attention as a potential mainstream technology in the future photovol-taic(PV)market.This is primarily attributed to their salient advantages inclu...In recent years,perovskite solar cells(PSCs)have garnered significant attention as a potential mainstream technology in the future photovol-taic(PV)market.This is primarily attributed to their salient advantages including high efficiency,low cost,and ease of preparation.Nota-bly,the power conversion efficiency(PCE)of PSCs has experienced a remarkable increase from 3.8%in 2009 to over 26%at present.Conse-quently,the adoption of roll-to-roll(R2R)technology for PSCs is considered a crucial step towards their successful commercialization.This arti-de reviews the diverse substrates,scalable deposition techniques(such as solution-based knife-coating and spraying technology),and optimiza.tion procedures employed in recent years to enhance device performance within the R2R process.Additionally,novel perspectives are presented to enrich the existing knowledge in this field.展开更多
Herein,ionomer-free amorphous iridium oxide(IrO_(x))thin electrodes are first developed as highly active anodes for proton exchange membrane electrolyzer cells(PEMECs)via low-cost,environmentally friendly,and easily s...Herein,ionomer-free amorphous iridium oxide(IrO_(x))thin electrodes are first developed as highly active anodes for proton exchange membrane electrolyzer cells(PEMECs)via low-cost,environmentally friendly,and easily scalable electrodeposition at room temperature.Combined with a Nafion 117 membrane,the IrO_(x)-integrated electrode with an ultralow loading of 0.075 mg cm^(-2)delivers a high cell efficiency of about 90%,achieving more than 96%catalyst savings and 42-fold higher catalyst utilization compared to commercial catalyst-coated membrane(2 mg cm^(-2)).Additionally,the IrO_(x)electrode demonstrates superior performance,higher catalyst utilization and significantly simplified fabrication with easy scalability compared with the most previously reported anodes.Notably,the remarkable performance could be mainly due to the amorphous phase property,sufficient Ir^(3+)content,and rich surface hydroxide groups in catalysts.Overall,due to the high activity,high cell efficiency,an economical,greatly simplified and easily scalable fabrication process,and ultrahigh material utilization,the IrO_(x)electrode shows great potential to be applied in industry and accelerates the commercialization of PEMECs and renewable energy evolution.展开更多
Composite solid electrolytes(CSEs)have emerged as promising candidates for safe and high-energy–density solid-state lithium metal batteries(SSLMBs).However,concurrently achieving exceptional ionic conductivity and in...Composite solid electrolytes(CSEs)have emerged as promising candidates for safe and high-energy–density solid-state lithium metal batteries(SSLMBs).However,concurrently achieving exceptional ionic conductivity and interface compatibility between the electrolyte and electrode presents a significant challenge in the development of high-performance CSEs for SSLMBs.To overcome these challenges,we present a method involving the in-situ polymerization of a monomer within a self-supported porous Li_(6.4)La_(3)Zr_(1.4)Ta_(0.6)O_(12)(LLZT)to produce the CSE.The synergy of the continuous conductive LLZT network,well-organized polymer,and their interface can enhance the ionic conductivity of the CSE at room temperature.Furthermore,the in-situ polymerization process can also con-struct the integration and compatibility of the solid electrolyte–solid electrode interface.The synthesized CSE exhibited a high ionic conductivity of 1.117 mS cm^(-1),a significant lithium transference number of 0.627,and exhibited electrochemical stability up to 5.06 V vs.Li/Li+at 30℃.Moreover,the Li|CSE|LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2) cell delivered a discharge capacity of 105.1 mAh g^(-1) after 400 cycles at 0.5 C and 30℃,corresponding to a capacity retention of 61%.This methodology could be extended to a variety of ceramic,polymer electrolytes,or battery systems,thereby offering a viable strategy to improve the electrochemical properties of CSEs for high-energy–density SSLMBs.展开更多
Metal-free defective carbon materials with abundant active sites have been widely studied as low-cost and efficient oxygen reduction reaction(ORR)electrocatalysts in metal-air batteries.However,the active sites in def...Metal-free defective carbon materials with abundant active sites have been widely studied as low-cost and efficient oxygen reduction reaction(ORR)electrocatalysts in metal-air batteries.However,the active sites in defective carbon are easily subjected to serious oxidation or hydroxylation during ORR or storage,leading to rapid degradation of activity.Herein,we design a van der Waals heterostructure comprised of vitamin C(VC)and defective carbon(DC)to not only boost the activity but also enhance the durability and storage stability of the DC-VC electrocatalyst.The formation of VC van der Waals between DC and VC is demonstrated to be an effective strategy to protect the defect active sites from oxidation and hydroxylation degradation,thus significantly enhancing the electrochemical durability and storage anti-aging performance.Moreover,the DC-VC van der Waals can reduce the reaction energy barrier to facilitate the ORR.These findings are also confirmed by operando Fourier transform infrared spectroscopy and density functional theory calculations.It is necessary to mention that the preparation of this DC-VC electrocatalyst can be scaled up,and the ORR performance of the largely produced electrocatalyst is demonstrated to be very consistent.Furthermore,the DC-VC-based aluminum-air batteries display very competitive power density with good performance maintenance.展开更多
Scaling up spin qubits in silicon-based quantum dots is one of the pivotal challenges in achieving large-scale semiconductor quantum computation.To satisfy the connectivity requirements and reduce the lithographic com...Scaling up spin qubits in silicon-based quantum dots is one of the pivotal challenges in achieving large-scale semiconductor quantum computation.To satisfy the connectivity requirements and reduce the lithographic complexity,utilizing the qubit array structure and the circuit quantum electrodynamics(cQED)architecture together is expected to be a feasible scaling scheme.A triple-quantum dot(TQD)coupled with a superconducting resonator is regarded as a basic cell to demonstrate this extension scheme.In this article,we investigate a system consisting of a silicon TQD and a high-impedance TiN coplanar waveguide(CPW)resonator.The TQD can couple to the resonator via the right double-quantum dot(RDQD),which reaches the strong coupling regime with a charge–photon coupling strength of g0/(2p)=175 MHz.Moreover,we illustrate the high tunability of the TQD through the characterization of stability diagrams,quadruple points(QPs),and the quantum cellular automata(QCA)process.Our results contribute to fostering the exploration of silicon-based qubit integration.展开更多
In this theoretical work,we describe a mechanism for the coupling between a plane structure consisting of four quantum dots and a resonator.We systematically study the dependence of the quadruple coupling strength and...In this theoretical work,we describe a mechanism for the coupling between a plane structure consisting of four quantum dots and a resonator.We systematically study the dependence of the quadruple coupling strength and the qubit decoherence rate and point out the optimized operating position of the hybrid system.According to the transmission given by the input-output theory,the signatures in the resonator spectrum are predicted.Furthermore,based on the parameters already achieved in previous works,we prove that the device described in this paper can achieve the strong coupling limit,i.e.,this approach can be used for system extension under the existing technical conditions.Our results show an effective and promotable approach to couple quantum dot structures in plane with the resonator and propose a meaningful extension method.展开更多
A physical model for scaling and optimizing InGaAs/InP double heterojunction bipolar transistors（DHBTs） based on hydrodynamic simulation is developed.The model is based on the hydrodynamic equation,which can accurat...A physical model for scaling and optimizing InGaAs/InP double heterojunction bipolar transistors（DHBTs） based on hydrodynamic simulation is developed.The model is based on the hydrodynamic equation,which can accurately describe non-equilibrium conditions such as quasi-ballistic transport in the thin base and the velocity overshoot effect in the depleted collector.In addition,the model accounts for several physical effects such as bandgap narrowing,variable effective mass,and doping-dependent mobility at high fields.Good agreement between the measured and simulated values of cutoff frequency,f t,and maximum oscillation frequency,f max,are achieved for lateral and vertical device scalings.It is shown that the model in this paper is appropriate for downscaling and designing InGaAs/InP DHBTs.展开更多
基金the National Key R&D Program of China(2022YFA1203304)the Natural Science Foundation of Jiangsu Province(BK20220288)+1 种基金Suzhou Institute of Nano-Tech and Nano-Bionics,Chinese Academy of Sciences(Start-up grant E1552102)the China Postdoctoral Science Foundation(No.2023M732553).
文摘The poor interfacial stability not only deteriorates fibre lithium-ion batteries(FLBs)performance but also impacts their scalable applications.To efficiently address these challenges,Prof.Huisheng Peng team proposed a generalized channel structures strategy with optimized in situ polymerization technology in their recent study.The resultant FLBs can be woven into different-sized powering textiles,providing a high energy density output of 128 Wh kg^(-1) and simultaneously demonstrating good durability even under harsh conditions.Such a promising strategy expands the horizon in developing FLB with particular polymer gel electrolytes,and significantly ever-deepening understanding of the scaled wearable energy textile system toward a sustainable future.
基金financially supported by the National Key Research and Development Project funding from the Ministry of Science and Technology of China(2021YFB3800104)the National Natural Science Foundation of China(51822203,52002140,U20A20252,51861145404,62105293,62205187)+4 种基金the Young Elite Scientists Sponsorship Program by CAST,the Self-determined and Innovative Research Funds of HUST(2020KFYXJJS008)the Natural Science Foundation of Hubei Province(ZRJQ2022000408)the Shenzhen Science and Technology Innovation Committee(JCYJ20180507182257563)Fundamental Research Program of Shanxi Province(202103021223032)the Innovation Project of Optics Valley Laboratory of China(OVL2021BG008)。
文摘Over the last decade,remarkable progress has been made in metal halide perovskite solar cells(PSCs),which have been a focus of emerging photovoltaic techniques and show great potential for commercialization.However,the upscaling of small-area PSCs to large-area solar modules to meet the demands of practical applications remains a significant challenge.The scalable production of high-quality perovskite films by a simple,reproducible process is crucial for resolving this issue.Furthermore,the crystallization behavior in the solution-processed fabrication of perovskite films can be strongly influenced by the physicochemical properties of the precursor inks,which are significantly affected by the employed solvents and their interactions with the solutes.Thus,a comprehensive understanding of solvent engineering for fabricating perovskite films over large areas is urgently required.In this paper,we first analyze the role of solvents in the solution-processed fabrication of large-area perovskite films based on the classical crystal nucleation and growth mechanism.Recent efforts in solvent engineering to improve the quality of perovskite films for solar modules are discussed.Finally,the basic principles and future challenges of solvent system design for scalable fabrication of high-quality perovskite films for efficient solar modules are proposed.
基金supported by the National Key Research and Development Program of China(Nos.2019YFA0707003 and 2019YFE0114100)the National Natural Science Foundation of China(NSFC 51872007)Beijing Municipal Natural Science Foundation(No.7202094).
文摘Perovskite solar cells have reached a power-conversion efficiency(PCE) of 25.6%,showing great potential with reliable moisture and heat stability.Most results are achieved on small-area devices,using conventional thin-film processing technologies like spin-coating method.However,such approaches may not be upscaled for large-area substrates.Thus,strategies and materials need to be developed for manufacturing processing routes to realize future commercial photovoltaic fabrications.Notable results have been achieved on large-area perovskite solar cells.In this review,similarities and differences of large-area perovskite fabrication mechanisms between the various pathways are investigated,especially on the parameters affecting the nucleation and crystal growth kinetics.Moreover,the methods for large-area transporting layers and electrodes are discussed,and some key issues from cells to modules.Challenges and opportunities are proposed to pave the way of high-efficiency perovskite solar modules.
基金supported by the National Natural Science Foundation of China under Grant No.61801119。
文摘Scalable video coding(SVC)has been widely used in video-on-demand(VOD)service,to efficiently satisfy users’different video quality requirements and dynamically adjust video stream to timevariant wireless channels.Under the 5G network structure,we consider a cooperative caching scheme inside each cluster with SVC to economically utilize the limited caching storage.A novel multi-agent deep reinforcement learning(MADRL)framework is proposed to jointly optimize the video access delay and users’satisfaction,where an aggregation node is introduced helping individual agents to achieve global observations and overall system rewards.Moreover,to cope with the large action space caused by the large number of videos and users,a dimension decomposition method is embedded into the neural network in each agent,which greatly reduce the computational complexity and memory cost of the reinforcement learning.Experimental results show that:1)the proposed value-decomposed dimensional network(VDDN)algorithm achieves an obvious performance gain versus the traditional MADRL;2)the proposed VDDN algorithm can handle an extremely large action space and quickly converge with a low computational complexity.
基金supported by funding from the Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate Universitythe OIST R&D Cluster Research Program+1 种基金the OIST Proof of Concept(POC)ProgramJSPS KAKENHI Grant Number 15K17925
文摘Perovskite-based solar cell technology has advanced significantly and the power conversion efficiencies are nowadays on par with commercialized photovoltaic technologies. To realize the potential of perovskite solar cells, the focus is now shifting to scalable fabrication technologies that will enable low-cost solution processing of perovskite solar cells over large areas and with high yields. This review article discusses the fundamental concerns that arise when transitioning from laboratory to large area solution coating, available scalable coating technologies, and their applicability to the fabrication of high-performance perovskite solar cells. We find that a significant amount of work has been done to test scalable coating technologies, but also that often the methods that led to highest-performing cells in the laboratory （e.g. antisolvent processing） show limited compatibility with scalable coating methods. To achieve a high-yield and low-cost process, development must emphasize a high degree of control provided by sequential conversion of perovskite films and engineering of additives that fine-tune coating properties of perovskite precursor inks.
基金Supported by the National Natural Science Foundation of China under Grant No 11305021the Fundamental Research Funds for the Central Universities of China under Grants Nos 3132014229 and 3132014328
文摘We develop a design of a hybrid quantum interface for quantum information transfer （QIT）, adopting a nanome- chanical resonator as the intermedium, which is magnetically coupled with individual nitrogen-vacancy centers as the solid qubits, while eapacitively coupled with a coplanar waveguide resonator as the quantum data bus. We describe the Hamiltonian of the model, and analytically demonstrate the QIT for both the resonant interaction and large detuning cases. The hybrid quantum interface allows for QIT between arbitrarily selected individual nitrogen-vacancy centers, and has advantages of the sealability and controllability. Our methods open an alter- native perspective for implementing QIT, which is important during quantum storing or processing procedures in quantum computing.
文摘A layered compression algorithm is presented which delivers spatial scalable encoded bit streams for remote video monitoring system. The complexity of the algorithm is modest and is well suited to real time implementation. Based on the layered compression algorithm, a codec system model is established. High-speed video compression can be realized with parallel data compression in this codec system. For image reconstruction, a prediction method using two nearest pix points is presented.
基金supported in part by the National Natural Science Founda⁃tion of China under Grant No.62293485the Fundamental Research Funds for the Central Universities under Grant No.2022RC18.
文摘The emerging new services in the sixth generation(6G)communication system impose increasingly stringent requirements and challenges on video transmission.Semantic communications are envisioned as a promising solution to these challenges.This paper provides a highly-efficient solution to video transmission by proposing a scalable semantic transmission algorithm,named scalable semantic transmission framework for video(SST-V),which jointly considers the semantic importance and channel conditions.Specifically,a semantic importance evaluation module is designed to extract more informative semantic features according to the estimated importance level,facilitating high-efficiency semantic coding.By further considering the channel condition,a cascaded learning based scalable joint semanticchannel coding algorithm is proposed,which autonomously adapts the semantic coding and channel coding strategies to the specific signalto-noise ratio(SNR).Simulation results show that SST-V achieves better video reconstruction performance,while significantly reducing the transmission overhead.
基金partially supported by the National Natural Science Foundation of China under Grants No. 610202380, No. 60932007Major Program of National Natural Science Foundation of China under Grant No. 60932007+2 种基金Tianjin Research Program of Application Foundation and Advanced Technology under Grant No. 12JCQNJC00300Research Fund for the Doctoral Program of Higher Education of China under Grant No. 20110032120029the Innovation Foundation of Tianjin University
文摘To achieve an optimal trade-off between video quality and energy efficiency in the uplink streaming of multi-user Scalable Video Coding (SVC) videos in relay-based Orthogonal Frequency Division Multiple Access (OFDMA) cellular networks, a cross-layer design framework that jointly selects the Transmission Policy (TP) for SVC video frames, assigns OFDMA subcarriers, and allocates power for each subcarrier is proposed. We apply the dual decomposition method to the problem, and obtain a TP selection subproblem for each SVC video adaptation and a resource allocation subproblem of Joint Subcarrier, Relay and Power Allocation (JSRPA). A second level of dual decomposition is used to divide the JSRPA problem into independent subcarrier subproblems. The proposed Crosslayer Trade-off Optimization (CTO) algorithm is sub-distributed with significantly low complexity. A performance evaluation with typical SVC video traces demonstrates that the proposed algorithm is able to converge and efficiently achieve the optimal trade-off between the video quality and energy consumption at the MSs for uplink SVC streaming.
基金supported by the Natural Science Foundation Committee (NSFC,No. 61903150)the Science and Technology Development Program of Jilin Province (20200401079GX)Research Funding Scheme for Ph.D. Graduate Interdisciplinary Studies,Jilin University (419100200835)。
文摘Electronic skins(e-skins) with an excellent sensing performance have been widely developed over the last few decades.However,wearability,biocompatibility,environmental friendliness and scalability have become new limitations. Self-healing ability can improve the long-term robustness and reliability of e-skins. However,self-healing ability and integration are hardly balanced in classical structures of self-healable devices. Here,cellulose nanofiber/poly(vinyl alcohol)(CNF/PVA),a biocompatible moisture-inspired self-healable composite,was applied both as the binder in functional layers and the substrate. Various functional layers comprising particular carbon materials and CNF/PVA were patterned on the substrate. A planar structure was beneficial for integration,and the active self-healing ability of the functional layers endowed self-healed e-skins with a higher toughness. Water served as both the only solvent throughout the fabrication process and the trigger of the self-healing process,which avoids the pollution and bioincompatibility caused by the application of noxious additives. Our e-skins could achieve real-time monitoring of whole-body physiological signals and environmental temperature and humidity. Cross-interference between di erent external stimuli was suppressed through reasonable material selection and structural design. Combined with conventional electronics,data could be transmitted to a nearby smartphone for post-processing. This work provides a previously unexplored strategy for multifunctional e-skins with an excellent practicality.
基金supported by the Foundation for Innovative Research Groups of the National Natural Science Foundation of China (Grant No. 2016YFB0800100, No. 2016YFB0800101)the National Natural Science Foundation of China (Grant No. 61521003)the National Key R&D Program of China (Grant No. 61309020)
文摘Dynamic Controller Provisioning Problem(DCPP) is a key problem for scalable SDN. Previously, the solution to this problem focused on adapting the number of controllers and their locations with changing network conditions, but ignored balancing control loads via switch migration. In this paper, we study a scalable control mechanism to decide which switch and where it should be migrated for more balanced control plane, and we define it as Switch Migration Problem(SMP). The main contributions of this paper are as follows. First, we define a SDN model to describe the relation between controllers and switches from the view of loads. Based on this model, we form SMP as a Network Utility Maximization(NUM) problem with the objective of serving more requests under available control resources. Second, we design a synthesizing distributed algorithm for SMP--- Distributed Hopping Algorithm(DHA), by approximating our optimal objective via Log-Sum-Exp function. In DHA, individual controller performs algorithmic procedure independently. With the solution space F, we prove that the optimal gap caused by approximation is at most 1/βlog|F|, and DHA procedure is equal to implementation of a time-reversible Markov Chain process. Finally, the results are corroborated by several numerical simulations.
基金supported by Program for National Basic Research Program of China (973 Program) "Reconfigurable Network Emulation Testbed for Basic Network Communication"
文摘Network Functions Virtualization(NFV) is an attempt to help operators more effectively manage their networks by implementing traditional network functions embedded in specialized hardware platforms in term of virtualized software instances. But, existing novel network appliances designed for NFV infrastructure are always architected on a general-purpose x86 server, which makes the performance of network functions limited by the hosted single server. To address this challenge, we propose ApplianceB ricks, a novel NFV-enable network appliance architecture that is used to explore the way of consolidating multiple physical network functions into a clustered network appliance, which is able to improve the processing capability of NFV-enabled network appliances.
文摘In a software-defined network, a powerful central controller provides a flexible platform for defining network traffic through the use of software. When SDN is used in a large-scale network, the logical central controller comprises multiple physical servers, and multiple controllers must act as one to provide transparent control logic to network applications and devices. The challenge is to minimize the cost of network state distribution. To this end, we propose Distributed ZTE Elastic Network Intelligent Controller （DZENIC）, a network-control platform that supports distributed deployment and linear scale-out. A dedicated component in the DZENIC controller provides a global view of the network topology as well as the distribution of host information. The evaluation shows that balance complexity with scalability, the network state distribution needs to be strictly classified.
文摘In recent years,perovskite solar cells(PSCs)have garnered significant attention as a potential mainstream technology in the future photovol-taic(PV)market.This is primarily attributed to their salient advantages including high efficiency,low cost,and ease of preparation.Nota-bly,the power conversion efficiency(PCE)of PSCs has experienced a remarkable increase from 3.8%in 2009 to over 26%at present.Conse-quently,the adoption of roll-to-roll(R2R)technology for PSCs is considered a crucial step towards their successful commercialization.This arti-de reviews the diverse substrates,scalable deposition techniques(such as solution-based knife-coating and spraying technology),and optimiza.tion procedures employed in recent years to enhance device performance within the R2R process.Additionally,novel perspectives are presented to enrich the existing knowledge in this field.
基金the support from the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy (EERE) under the Hydrogen and Fuel Cell Technologies Office Awards DE-EE0008426 and DE-EE0008423National Energy Technology Laboratory under Award DEFE0011585.
文摘Herein,ionomer-free amorphous iridium oxide(IrO_(x))thin electrodes are first developed as highly active anodes for proton exchange membrane electrolyzer cells(PEMECs)via low-cost,environmentally friendly,and easily scalable electrodeposition at room temperature.Combined with a Nafion 117 membrane,the IrO_(x)-integrated electrode with an ultralow loading of 0.075 mg cm^(-2)delivers a high cell efficiency of about 90%,achieving more than 96%catalyst savings and 42-fold higher catalyst utilization compared to commercial catalyst-coated membrane(2 mg cm^(-2)).Additionally,the IrO_(x)electrode demonstrates superior performance,higher catalyst utilization and significantly simplified fabrication with easy scalability compared with the most previously reported anodes.Notably,the remarkable performance could be mainly due to the amorphous phase property,sufficient Ir^(3+)content,and rich surface hydroxide groups in catalysts.Overall,due to the high activity,high cell efficiency,an economical,greatly simplified and easily scalable fabrication process,and ultrahigh material utilization,the IrO_(x)electrode shows great potential to be applied in industry and accelerates the commercialization of PEMECs and renewable energy evolution.
基金supported by the National Research Foundation of Korea (NRF) grant funded by the MSIT,Korea (No. 2018R1A5A1025224 and No. 2019R1A2C1084020)this research received funding support from a grant from the Korea Planning&Evaluation Institute of Industrial Technology (KEIT),funded by the MOTIE of Korea (No. 10077287)。
文摘Composite solid electrolytes(CSEs)have emerged as promising candidates for safe and high-energy–density solid-state lithium metal batteries(SSLMBs).However,concurrently achieving exceptional ionic conductivity and interface compatibility between the electrolyte and electrode presents a significant challenge in the development of high-performance CSEs for SSLMBs.To overcome these challenges,we present a method involving the in-situ polymerization of a monomer within a self-supported porous Li_(6.4)La_(3)Zr_(1.4)Ta_(0.6)O_(12)(LLZT)to produce the CSE.The synergy of the continuous conductive LLZT network,well-organized polymer,and their interface can enhance the ionic conductivity of the CSE at room temperature.Furthermore,the in-situ polymerization process can also con-struct the integration and compatibility of the solid electrolyte–solid electrode interface.The synthesized CSE exhibited a high ionic conductivity of 1.117 mS cm^(-1),a significant lithium transference number of 0.627,and exhibited electrochemical stability up to 5.06 V vs.Li/Li+at 30℃.Moreover,the Li|CSE|LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2) cell delivered a discharge capacity of 105.1 mAh g^(-1) after 400 cycles at 0.5 C and 30℃,corresponding to a capacity retention of 61%.This methodology could be extended to a variety of ceramic,polymer electrolytes,or battery systems,thereby offering a viable strategy to improve the electrochemical properties of CSEs for high-energy–density SSLMBs.
基金financially supported by the National Natural Science Foundation of China (51874197)the Natural Science Foundation of Shanghai (21ZR1429400,22ZR1429700)。
文摘Metal-free defective carbon materials with abundant active sites have been widely studied as low-cost and efficient oxygen reduction reaction(ORR)electrocatalysts in metal-air batteries.However,the active sites in defective carbon are easily subjected to serious oxidation or hydroxylation during ORR or storage,leading to rapid degradation of activity.Herein,we design a van der Waals heterostructure comprised of vitamin C(VC)and defective carbon(DC)to not only boost the activity but also enhance the durability and storage stability of the DC-VC electrocatalyst.The formation of VC van der Waals between DC and VC is demonstrated to be an effective strategy to protect the defect active sites from oxidation and hydroxylation degradation,thus significantly enhancing the electrochemical durability and storage anti-aging performance.Moreover,the DC-VC van der Waals can reduce the reaction energy barrier to facilitate the ORR.These findings are also confirmed by operando Fourier transform infrared spectroscopy and density functional theory calculations.It is necessary to mention that the preparation of this DC-VC electrocatalyst can be scaled up,and the ORR performance of the largely produced electrocatalyst is demonstrated to be very consistent.Furthermore,the DC-VC-based aluminum-air batteries display very competitive power density with good performance maintenance.
基金the National Natural Science Foun-dation of China(Grant Nos.92265113,12074368,12304560,and 12034018)China Postdoctoral Science Foundation(Grant Nos.BX20220281 and 2023M733408).
文摘Scaling up spin qubits in silicon-based quantum dots is one of the pivotal challenges in achieving large-scale semiconductor quantum computation.To satisfy the connectivity requirements and reduce the lithographic complexity,utilizing the qubit array structure and the circuit quantum electrodynamics(cQED)architecture together is expected to be a feasible scaling scheme.A triple-quantum dot(TQD)coupled with a superconducting resonator is regarded as a basic cell to demonstrate this extension scheme.In this article,we investigate a system consisting of a silicon TQD and a high-impedance TiN coplanar waveguide(CPW)resonator.The TQD can couple to the resonator via the right double-quantum dot(RDQD),which reaches the strong coupling regime with a charge–photon coupling strength of g0/(2p)=175 MHz.Moreover,we illustrate the high tunability of the TQD through the characterization of stability diagrams,quadruple points(QPs),and the quantum cellular automata(QCA)process.Our results contribute to fostering the exploration of silicon-based qubit integration.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.92265113,12074368,and 12034018).
文摘In this theoretical work,we describe a mechanism for the coupling between a plane structure consisting of four quantum dots and a resonator.We systematically study the dependence of the quadruple coupling strength and the qubit decoherence rate and point out the optimized operating position of the hybrid system.According to the transmission given by the input-output theory,the signatures in the resonator spectrum are predicted.Furthermore,based on the parameters already achieved in previous works,we prove that the device described in this paper can achieve the strong coupling limit,i.e.,this approach can be used for system extension under the existing technical conditions.Our results show an effective and promotable approach to couple quantum dot structures in plane with the resonator and propose a meaningful extension method.
基金Project supported by the National Basic Research Program of China (Grant No. 2010CB327502)
文摘A physical model for scaling and optimizing InGaAs/InP double heterojunction bipolar transistors（DHBTs） based on hydrodynamic simulation is developed.The model is based on the hydrodynamic equation,which can accurately describe non-equilibrium conditions such as quasi-ballistic transport in the thin base and the velocity overshoot effect in the depleted collector.In addition,the model accounts for several physical effects such as bandgap narrowing,variable effective mass,and doping-dependent mobility at high fields.Good agreement between the measured and simulated values of cutoff frequency,f t,and maximum oscillation frequency,f max,are achieved for lateral and vertical device scalings.It is shown that the model in this paper is appropriate for downscaling and designing InGaAs/InP DHBTs.
