This paper uses a nonperturbative scattering theory to study photoelectron angular distributions of homonuclear diatomic molecules irradiated by circularly polarized laser fields. This study shows that the nonisotropi...This paper uses a nonperturbative scattering theory to study photoelectron angular distributions of homonuclear diatomic molecules irradiated by circularly polarized laser fields. This study shows that the nonisotropic feature of photoelectron angular distributions is not due to the polarization of the laser field but the internuclear vector of the molecules. It suggests a method to measure the molecular orientation and the internuclear distance of molecules through the measurement of photoelectron angular distributions.展开更多
Measurements of zero-degree breakup fragment energy distribution fromthe Coulomb-Explosions of 1.50965 MeV HD+ ion inicro-cluster beam are reported.Mean value of the internuclear separation of HD+ is found to be 0.125...Measurements of zero-degree breakup fragment energy distribution fromthe Coulomb-Explosions of 1.50965 MeV HD+ ion inicro-cluster beam are reported.Mean value of the internuclear separation of HD+ is found to be 0.12510.003 urn. Aset of high-resolution experimental arrangement and improvement of the Van-de-Graaffaccelerator are described briefly.展开更多
The double ionization process of molecules driven by co-rotating two-color circularly polarized fields is investigated with a three-dimensional classical ensemble model. Numerical results indicate that a considerable ...The double ionization process of molecules driven by co-rotating two-color circularly polarized fields is investigated with a three-dimensional classical ensemble model. Numerical results indicate that a considerable part of the sequential double ionization(DI) events of molecules occur through internal collision double ionization(ICD), and the ICD recollision mechanism is significantly different from that in non-sequential double ionization(NSDI). By analyzing the results of internuclear distances R = 5 a.u. and 2 a.u., these two recollision mechanisms are studied in depth. It is found that the dynamic behaviors of the recollision mechanisms of NSDI and ICD are similar. For NSDI, the motion range of electrons after the ionization is relatively large, and the electrons will return to the core after a period of time. In the ICD process,electrons will rotate around the parent ion before ionization, and the distance of the electron motion is relatively small. After a period of time, the electrons will come back to the core and collide with another electron. Furthermore, the molecular internuclear distance has a significant effect on the electron dynamic behavior of the two ionization mechanisms. This study will help to understand the multi-electron ionization process of complex systems.展开更多
利用全量子方法改进且加入核核作用(PT)的修正库仑玻恩近似(MCBPT)和前人基于半经典的方法且不考虑核核作用的修正库仑玻恩近似(MCB)计算了散射平面和垂直平面内100 Me V/amu C6+单电离氦原子的全微分截面,研究了核核作用对截面的影响....利用全量子方法改进且加入核核作用(PT)的修正库仑玻恩近似(MCBPT)和前人基于半经典的方法且不考虑核核作用的修正库仑玻恩近似(MCB)计算了散射平面和垂直平面内100 Me V/amu C6+单电离氦原子的全微分截面,研究了核核作用对截面的影响.其结果与实验数据和3DW理论进行了比较.发现,对于小动量转移,MCBPT计算结果与实验符合的很好;对于大动量转移,MCB结果很好的反映了实验数据.而且,我们详细的分析了扭曲势效应对截面的影响,结果表明随着动量转移的增加扭曲势效应迅速增强.展开更多
基金supported by the National Natural Science Foundation of China (Grant No. 10774153)the National Basic Research Program of China (Grant No. 2006CD806000)the Shanghai "Phosphor" Science Foundation, China (Grant No. 08QH1402400)
文摘This paper uses a nonperturbative scattering theory to study photoelectron angular distributions of homonuclear diatomic molecules irradiated by circularly polarized laser fields. This study shows that the nonisotropic feature of photoelectron angular distributions is not due to the polarization of the laser field but the internuclear vector of the molecules. It suggests a method to measure the molecular orientation and the internuclear distance of molecules through the measurement of photoelectron angular distributions.
文摘Measurements of zero-degree breakup fragment energy distribution fromthe Coulomb-Explosions of 1.50965 MeV HD+ ion inicro-cluster beam are reported.Mean value of the internuclear separation of HD+ is found to be 0.12510.003 urn. Aset of high-resolution experimental arrangement and improvement of the Van-de-Graaffaccelerator are described briefly.
基金the National Key Research and Development Program of China (Grant No.2019YFA0307700)the National Natural Science Foundation of China (Grant Nos.12074145 and 11975012)+1 种基金Jilin Provincial Research Foundation for Basic Research,China (Grant No.20220101003JC)Jilin Provincial Education Department (Grant No.JJKH20230284KJ)。
文摘The double ionization process of molecules driven by co-rotating two-color circularly polarized fields is investigated with a three-dimensional classical ensemble model. Numerical results indicate that a considerable part of the sequential double ionization(DI) events of molecules occur through internal collision double ionization(ICD), and the ICD recollision mechanism is significantly different from that in non-sequential double ionization(NSDI). By analyzing the results of internuclear distances R = 5 a.u. and 2 a.u., these two recollision mechanisms are studied in depth. It is found that the dynamic behaviors of the recollision mechanisms of NSDI and ICD are similar. For NSDI, the motion range of electrons after the ionization is relatively large, and the electrons will return to the core after a period of time. In the ICD process,electrons will rotate around the parent ion before ionization, and the distance of the electron motion is relatively small. After a period of time, the electrons will come back to the core and collide with another electron. Furthermore, the molecular internuclear distance has a significant effect on the electron dynamic behavior of the two ionization mechanisms. This study will help to understand the multi-electron ionization process of complex systems.
文摘利用全量子方法改进且加入核核作用(PT)的修正库仑玻恩近似(MCBPT)和前人基于半经典的方法且不考虑核核作用的修正库仑玻恩近似(MCB)计算了散射平面和垂直平面内100 Me V/amu C6+单电离氦原子的全微分截面,研究了核核作用对截面的影响.其结果与实验数据和3DW理论进行了比较.发现,对于小动量转移,MCBPT计算结果与实验符合的很好;对于大动量转移,MCB结果很好的反映了实验数据.而且,我们详细的分析了扭曲势效应对截面的影响,结果表明随着动量转移的增加扭曲势效应迅速增强.
