The alteration in surface color of metallic glasses(MGs)holds great significance in the context of microstructuredesign and commercial utility.It is essential to accurately describe the structures that are formed duri...The alteration in surface color of metallic glasses(MGs)holds great significance in the context of microstructuredesign and commercial utility.It is essential to accurately describe the structures that are formed during the laser and colorseparation processes in order to develop practical laser coloring applications.Due to the high oxidation sensitivity of Labasedmetallic glass,it can broaden the color range but make it more complex.Structure coloring by laser processing on thesurface of La-based metallic glass can be conducted after thermoplastic forming.It is particularly important to clarify therole of structure and composition in the surface coloring process.The aim is to study the relationship between amorphoussurface structural color,surface geometry,and oxide formation by laser processing in metallic glasses.The findings revealedthat the periodic structure primarily determines the surface color at laser energy densities below 1.0 J/mm^(2).In contrast,thesurface color predominantly depends on the proportion of oxides that are formed when energy densities exceed 1.0 J/mm^(2).Consequently,this study provides a novel concept for the fundamental investigation of laser coloring and establishes a newavenue for practical application.展开更多
As an intense picosecond laser pulse irradiates a hydrocarbon target,the protons therein can be accelerated by the radiation pressure as well as the sheath field behind the target.We investigate the effect of the lase...As an intense picosecond laser pulse irradiates a hydrocarbon target,the protons therein can be accelerated by the radiation pressure as well as the sheath field behind the target.We investigate the effect of the laser and hydrocarbon target parameters on proton acceleration with two/threedimensional particle-in-cell simulations.It is found that the resulting two-ion species plasma can generate a multiple peaked charge-separation field that accelerates the protons.In particular,a smaller carbon-to-hydrogen ratio,as well as the thinner and/or lower density of the target,leads to a larger sheath field and thus proton beams with a larger cutoff energy and smoother energy spectrum.These results may be useful in achieving high-flux quasi-monoenergetic proton beams by properly designing the hydrocarbon target.展开更多
Pulse-burst 1064-nm picosecond azimuthal polarization beam amplification up to an average power of 16.32 W using side-pumped Nd: YAG amplifiers has been demonstrated. The maximum envelop energy as much as 16.32 mJ, co...Pulse-burst 1064-nm picosecond azimuthal polarization beam amplification up to an average power of 16.32 W using side-pumped Nd: YAG amplifiers has been demonstrated. The maximum envelop energy as much as 16.32 mJ, corresponding to a power amplification factor of 299.5%. A simple criterion was defined to help estimate the amount of depolarization in Nd:YAG amplifier stages. The degree of depolarization of the beam was 7.1% and the beam quality was measured to be M2= 3.69. The reason for the azimuthal polarization depolarization and beam quality degradation were explained theoretically and experimentally during the amplification process.展开更多
Picosecond optical parametric generation and amplification in the near-infrared region within 1.361-1.656 μm and the mid-infrared region within 2.976-4.875 μm is constructed on the basis of bulk MgO：LiNbO 3 crystal...Picosecond optical parametric generation and amplification in the near-infrared region within 1.361-1.656 μm and the mid-infrared region within 2.976-4.875 μm is constructed on the basis of bulk MgO：LiNbO 3 crystals pumped at 1.064 μm.The maximum pulse energy reaches 1.3 mJ at 1.464 μm and 0.47 mJ at 3.894 μm,corresponding to a pumpto-idler photon conversion efficiency of 25%.By seeding the hard-to-measure mid-infrared radiation as the idler in the optical parametric amplification and measuring the amplified and frequency up-converted signal in the near-infrared or even visible region,one can measure very week mid-infrared radiation with ordinary detectors,which are insensitive to mid-infrared radiation,with a very high gain.A maximum gain factor of about 7 脳 10 7 is achieved at the mid-infrared wavelength of 3.374 μm and the corresponding energy detection limit is as low as about 390 aJ per pulse.展开更多
Picosecond pulse radiolysis of neat tetrahydrofuran (THF) shows a fast decay of the solvated electron within 2.5ns.The decay of the solvated electron observed at 790nm is because of spur reaction.A numerical simulatio...Picosecond pulse radiolysis of neat tetrahydrofuran (THF) shows a fast decay of the solvated electron within 2.5ns.The decay of the solvated electron observed at 790nm is because of spur reaction.A numerical simulation using time dependent Smoluchowski equation containing a sink term with a distance dependent reaction rate is used to fit the pulse-probe data and shows that the geminate reaction can proceed at long distance in this low polar solvent.展开更多
We present a cascaded nonlinear spectral broadening scheme for Nd-doped lasers,featuring with long pulse duration and high average power.This scheme is based on two multi-pass cells(MPCs)and one multiple-plate superco...We present a cascaded nonlinear spectral broadening scheme for Nd-doped lasers,featuring with long pulse duration and high average power.This scheme is based on two multi-pass cells(MPCs)and one multiple-plate supercontinuum generation(MPSG),and the numerical investigation is driven by a home-made Nd-doped fiber laser with 12 ps pulse duration,50 kHz repetition rate and 100 W average power.The MPC-based first two stages allow us to broaden the pulse spectrum to 4 nm and 43 nm respectively,and subsequently,the MPSG-based third stage allows us to reach 235 nm spectral bandwidth.This broadened spectrum can support a Fourier-transfer-limited pulse duration of 9.8 fs,which is shorter than three optical cycles.To the best of our knowledge,it is the first time to demonstrate the possibility of few-cycle pulses generation based on the 10 ps level Nd-doped lasers.Such few-cycle and high average power laser sources should be attractive and prospective,benefiting from the characteristics of structure compact,low-cost and flexibility.展开更多
基金supported by the National Natural Science Foundation of China(Grant Nos.52071222 and 52471180)Guangdong Major Project of Basic and Applied Basic Research,China(Grant No.2019B030302010)+2 种基金Guangdong Basic and Applied Basic Research,China(Grant No.2020B1515130007)the National Key Research and Development Program of China(Grant No.2021YFA0716302)the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB30000000).
文摘The alteration in surface color of metallic glasses(MGs)holds great significance in the context of microstructuredesign and commercial utility.It is essential to accurately describe the structures that are formed during the laser and colorseparation processes in order to develop practical laser coloring applications.Due to the high oxidation sensitivity of Labasedmetallic glass,it can broaden the color range but make it more complex.Structure coloring by laser processing on thesurface of La-based metallic glass can be conducted after thermoplastic forming.It is particularly important to clarify therole of structure and composition in the surface coloring process.The aim is to study the relationship between amorphoussurface structural color,surface geometry,and oxide formation by laser processing in metallic glasses.The findings revealedthat the periodic structure primarily determines the surface color at laser energy densities below 1.0 J/mm^(2).In contrast,thesurface color predominantly depends on the proportion of oxides that are formed when energy densities exceed 1.0 J/mm^(2).Consequently,this study provides a novel concept for the fundamental investigation of laser coloring and establishes a newavenue for practical application.
基金the National Key R&D Program of China(No.2016YFA0401100)National Natural Science Foundation of China(Nos.12175154,11875092,and 12005149)+1 种基金the Natural Science Foundation of Top Talent of SZTU(Nos.2019010801001 and 2019020801001)The EPOCH code is used under UK EPSRC contract(EP/G055165/1 and EP/G056803/1).
文摘As an intense picosecond laser pulse irradiates a hydrocarbon target,the protons therein can be accelerated by the radiation pressure as well as the sheath field behind the target.We investigate the effect of the laser and hydrocarbon target parameters on proton acceleration with two/threedimensional particle-in-cell simulations.It is found that the resulting two-ion species plasma can generate a multiple peaked charge-separation field that accelerates the protons.In particular,a smaller carbon-to-hydrogen ratio,as well as the thinner and/or lower density of the target,leads to a larger sheath field and thus proton beams with a larger cutoff energy and smoother energy spectrum.These results may be useful in achieving high-flux quasi-monoenergetic proton beams by properly designing the hydrocarbon target.
基金Project supported by the National Natural Science Foundation of China(Grant No.U1631240)the Education Commission Program of BeijingBeijing Natural Science Foundation(Grant No.KZ201510005001)
文摘Pulse-burst 1064-nm picosecond azimuthal polarization beam amplification up to an average power of 16.32 W using side-pumped Nd: YAG amplifiers has been demonstrated. The maximum envelop energy as much as 16.32 mJ, corresponding to a power amplification factor of 299.5%. A simple criterion was defined to help estimate the amount of depolarization in Nd:YAG amplifier stages. The degree of depolarization of the beam was 7.1% and the beam quality was measured to be M2= 3.69. The reason for the azimuthal polarization depolarization and beam quality degradation were explained theoretically and experimentally during the amplification process.
基金Project supported by the National Natural Science Foundation of China (Grant No. 61078005)the National Basic ResearchProgram of China (Grant No. 2007CB613205)the China Postdoctoral Science Foundation
文摘Picosecond optical parametric generation and amplification in the near-infrared region within 1.361-1.656 μm and the mid-infrared region within 2.976-4.875 μm is constructed on the basis of bulk MgO：LiNbO 3 crystals pumped at 1.064 μm.The maximum pulse energy reaches 1.3 mJ at 1.464 μm and 0.47 mJ at 3.894 μm,corresponding to a pumpto-idler photon conversion efficiency of 25%.By seeding the hard-to-measure mid-infrared radiation as the idler in the optical parametric amplification and measuring the amplified and frequency up-converted signal in the near-infrared or even visible region,one can measure very week mid-infrared radiation with ordinary detectors,which are insensitive to mid-infrared radiation,with a very high gain.A maximum gain factor of about 7 脳 10 7 is achieved at the mid-infrared wavelength of 3.374 μm and the corresponding energy detection limit is as low as about 390 aJ per pulse.
文摘Picosecond pulse radiolysis of neat tetrahydrofuran (THF) shows a fast decay of the solvated electron within 2.5ns.The decay of the solvated electron observed at 790nm is because of spur reaction.A numerical simulation using time dependent Smoluchowski equation containing a sink term with a distance dependent reaction rate is used to fit the pulse-probe data and shows that the geminate reaction can proceed at long distance in this low polar solvent.
基金Project supported by the National Natural Science Foundation of China(Grant No.61925507)the National Key R&D Program of China(Grant No.2017YFE0123700)+5 种基金the Strategic Priority Research Program of Chinese Academic Sciences(Grant No.XDB1603)the Shanghai Municipal Science and Technology Major Project(Grant No.2017SHZDZX02)the Shanghai Natural ScienceFoundation(Grant No.20ZR1464600)the Program of Shanghai Academic/Technology Research Leader(Grant No.18XD1404200)the Shanghai Sailing Program(Grant No.21YF1453800)Youth Innovation Promotion Association of Chinese Academic Sciences(Grant No.Y202059).
文摘We present a cascaded nonlinear spectral broadening scheme for Nd-doped lasers,featuring with long pulse duration and high average power.This scheme is based on two multi-pass cells(MPCs)and one multiple-plate supercontinuum generation(MPSG),and the numerical investigation is driven by a home-made Nd-doped fiber laser with 12 ps pulse duration,50 kHz repetition rate and 100 W average power.The MPC-based first two stages allow us to broaden the pulse spectrum to 4 nm and 43 nm respectively,and subsequently,the MPSG-based third stage allows us to reach 235 nm spectral bandwidth.This broadened spectrum can support a Fourier-transfer-limited pulse duration of 9.8 fs,which is shorter than three optical cycles.To the best of our knowledge,it is the first time to demonstrate the possibility of few-cycle pulses generation based on the 10 ps level Nd-doped lasers.Such few-cycle and high average power laser sources should be attractive and prospective,benefiting from the characteristics of structure compact,low-cost and flexibility.
基金Supported by National Natural Science Foundation of China(6127514261308042+2 种基金51321091)National Key Scientific Instrument and Equipment Development Project(2011YQ030127)China Postdoctoral Science Foundation(014T70633)
