Solar steam generation(SSG)is widely regarded as one of the most sustainable technologies for seawater desalination.However,salt fouling severely compromises the evaporation performance and lifetime of evaporators,lim...Solar steam generation(SSG)is widely regarded as one of the most sustainable technologies for seawater desalination.However,salt fouling severely compromises the evaporation performance and lifetime of evaporators,limiting their practical applications.Herein,we propose a hierarchical salt-rejection(HSR)strategy to prevent salt precipitation during long-term evaporation while maintaining a rapid evaporation rate,even in high-salinity brine.The salt diffusion process is segmented into three steps—insulation,branching diffusion,and arterial transport—that significantly enhance the salt-resistance properties of the evaporator.Moreover,the HSR strategy overcomes the tradeoff between salt resistance and evaporation rate.Consequently,a high evaporation rate of 2.84 kg m^(-2) h^(-1),stable evaporation for 7 days cyclic tests in 20 wt%NaCl solution,and continuous operation for 170 h in natural seawater under 1 sun illumination were achieved.Compared with control evaporators,the HSR evaporator exhibited a>54%enhancement in total water evaporation mass during 24 h continuous evaporation in 20 wt%salt water.Furthermore,a water collection device equipped with the HSR evaporator realized a high water purification rate(1.1 kg m^(-2) h^(-1)),highlighting its potential for agricultural applications.展开更多
Two new AlTiN coated cemented carbide drills with Al content of 40% and 55% in weight are developed for high efficiency dry drilling of 40Cr. By studying tool durability, machined hole quality, tool wear mechanism, ch...Two new AlTiN coated cemented carbide drills with Al content of 40% and 55% in weight are developed for high efficiency dry drilling of 40Cr. By studying tool durability, machined hole quality, tool wear mechanism, chip deformation, and lubrication, the dry drilling performance of the two kinds of coated drills is analyzed. Experimental results show that the AlTiN coated drills are suitable for high efficiency dry drilling and can obtain higher quality of machined holes. The tool durability of the drill with 55% Al content is 1. 3 times of that of the drill with 40% Al content at the cutting speed of 90 m/min. The wear mechanism of two AlTiN coatings are studied in experiments. During dry drilling process, oxidative wear appears in both two kinds of drills. The oxide film is formed on the top of the coated drill containing Al content of 55%. And the oxide film helps to increase its high temperature resistance and decrease the coating flaking, thus the drill is failed because of coating subsidence. The drill with less Al content is failed due to peeling and breakage. The lubricated condition in dry drilling is improved by the high Al content coating. It helps to reduce the cutting deformation and benefits to improve the quality of machined holes. The AlTiN coating with higher Al content shows longer tool life and higher quality of machined holes in high efficiency dry drilling. Its tool life increases by 30% compared with that of the coating with less Al content.展开更多
Green manufacturing （GM） and high efficiency machining technology are inevitable trends in the field of advanced manufacturing of the 21st century. To ensure green and high-efficiency machining, a new high efficienc...Green manufacturing （GM） and high efficiency machining technology are inevitable trends in the field of advanced manufacturing of the 21st century. To ensure green and high-efficiency machining, a new high efficiency cooling technology-cryogenic pneumatic mist jet impinging cooling （CPMJI） technology is presented. For obtaining the best cooling effect, a little quantity of coolant is carried by high speed cryogenic air （-20 C ） and reaches the machining zone in the form of mist jet to enhance heat transfer. Experimental results indicate that under the conditions of 40 m/s in the jet impinging speed and 10 mm in the jet impinging distance, the critical heat flux（CHF） nearly reaches 6× 10^7 W/m^2, more than six times of the CHF of the grinding burn with a value of （8～10）×10^6 W/m^2.展开更多
The lead-free perovskite solar cells(PSCs) have drawn a great deal of research interest due to the Pb toxicity of the lead halide perovskite.CHNHSnIis a viable alternative to CHNHPbX,because it has a narrower band gap...The lead-free perovskite solar cells(PSCs) have drawn a great deal of research interest due to the Pb toxicity of the lead halide perovskite.CHNHSnIis a viable alternative to CHNHPbX,because it has a narrower band gap of 1.3 eV and a wider visible absorption spectrum than the lead halide perovskite.The progress of fabricating tin iodide PSCs with good stability has stimulated the studies of these CHNHSnIbased cells greatly.In the paper,we study the influences of various parameters on the solar cell performance through theoretical analysis and device simulation.It is found in the simulation that the solar cell performance can be improved to some extent by adjusting the doping concentration of the perovskite absorption layer and the electron affinity of the buffer and HTM,while the reduction of the defect density of the perovskite absorption layer significantly improves the cell performance.By further optimizing the parameters of the doping concentration(1.3 × 10cm~3) and the defect density(1 × 10cm~3) of perovskite absorption layer,and the electron affinity of buffer(4.0 eV) and HTM(2.6 eV),we finally obtain some encouraging results of the Jof 31.59 mA/cm~2,Vof 0.92 V,FF of 79.99%,and PCE of 23.36%.The results show that the lead-free CHNHSnIPSC is a potential environmentally friendly solar cell with high efficiency.Improving the Snstability and reducing the defect density of CHNHSnIare key issues for the future research,which can be solved by improving the fabrication and encapsulation process of the cell.展开更多
High-brightness and color-stable two-wavelength hybrid white organic light emitting diodes （HWOLEDs） with the configuration of indium tin oxide （ITO）/ N, N, N, N-tetrakis（4-methoxyphenyl）-benzidine （MeO-TPD）：...High-brightness and color-stable two-wavelength hybrid white organic light emitting diodes （HWOLEDs） with the configuration of indium tin oxide （ITO）/ N, N, N, N-tetrakis（4-methoxyphenyl）-benzidine （MeO-TPD）： tetrafluoro-tetracyanoqino dimethane （F4-TCNQ）/N,N-di（naphthalene-1-yl）-N,N-diphenyl-benzidine （NPB）/ 4,4-N,N-dicarbazolebiphenyl （CBP）： iridium （III） diazine complexes （MPPZ） 2 Ir（acac）/NPB/2-methyl-9,10-di（2-naphthyl）anthracene （MADN）： p-bis（p-N,N-di-phenyl-aminostyryl）benzene （DSA-ph）/bis（10-hydroxybenzo[h] quino-linato）beryllium complex （Bebq2）/LiF/Al have been fabricated and characterized. The optimal brightness of the device is 69932 cd/m2 at a voltage of 13 V, and the Commission Internationale de l’Eclairage （CIE） chromaticity coordinates are almost constant during a large voltage change of 6–12 V. Furthermore, a current efficiency of 15.3 cd/A at an illumination-relevant brightness of 1000 cd/m2 is obtained, which rolls off slightly to 13.0 cd/A at an ultra high brightness of 50000 cd/m2. We attribute this great performance to wisely selecting an appropriate spacer together with effectively utilizing the combinations of exciton-harvested orange-phosphorescence/blue-fluorescence in the device. Undoubtedly, this is one of the most exciting results in two-wavelength HWOLEDs up to now.展开更多
To master theoretical calculation for dust removal efficiency of high pressure atomization in an underground coal mine, the corresponding atomization characteristics and dust removal efficiency were both comprehensive...To master theoretical calculation for dust removal efficiency of high pressure atomization in an underground coal mine, the corresponding atomization characteristics and dust removal efficiency were both comprehensively studied in theory by virtue of related theories of hydromechanics and aerosol.According to actual measurements of flow coefficients and atomization angles of X-type swirl nozzle,computational formula was derived for atomized particle sizes of such a nozzle in conjunction with relevant empirical equation. Moreover, a mathematical model for applying high pressure atomization to dust removal in underground coal mine was also established to deduce theoretical computation formula of fractional efficiency. Then, Matlab was adopted to portray the relation curve between fractional efficiency and influence factors. In addition, a theoretical formula was also set up for removal efficiency of respirable dust and total coal dust based on dust size and frequency distribution equations. In the end,impacts of dust characteristic parameters on various dust removal efficiencies were analyzed.展开更多
Sodium-ion capacitors(SICs)have attracted appreciable attention in virtue of the higher energy and power densities compared with their rivals,supercapacitors and sodium-ion batteries.Due to the lack of sodium resource...Sodium-ion capacitors(SICs)have attracted appreciable attention in virtue of the higher energy and power densities compared with their rivals,supercapacitors and sodium-ion batteries.Due to the lack of sodium resources in cathode,presodiation is critical for SICs to further augment performances.However,current presodiation strategy utilizes metallic sodium as the presodiation material.In this strategy,assembling/disassembling of half-cells is required,which is dangerous and in creases the time and cost of SIC leading to the restriction of their industrialization and commercialization.Herein we present a safe,low-cost and high-efficiency presodiation strategy by first employing Na_(2)C_(2)O_(4) as the sacrificial salt applied in SICs.Na_(2)C_(2)O_(4) is environmentally friendly and possesses considerably low expenditure.No additional residues remain after sodium extraction ascribed to its"zero dead mass"property.When paired with commercial activated carb on as the cathode and commercial hard carbon as the ano de,the constructed pouch-type SICs exhibit high energy and power densities of 91.7 Wh/kg and 13.1 kW/kg,respectively.This work shows a prospect of realizing the safe and low-cost manufacturing for high-performance SICs commercially.展开更多
In this paper, we present a high-efficiency S-band gallium nitride （GaN） power amplifier （PA）. This amplifier is fabri- cated based on a self-developed GaN high-electron-mobility transistor （HEMT） with 10 mm gat...In this paper, we present a high-efficiency S-band gallium nitride （GaN） power amplifier （PA）. This amplifier is fabri- cated based on a self-developed GaN high-electron-mobility transistor （HEMT） with 10 mm gate width on SiC substrate. Harmonic manipulation circuits are presented in the amplifier. The matching networks consist of microstrip lines and discrete components. Open-circuited stub lines in both input and output are used to tune the 2rid harmonic wave and match the GaN HEMT to the highest efficiency condition. The developed amplifier delivers an output power of 48.5 dBm （70 W） with a power-added efficiency （PAE） of 72.2% at 2 GHz in pulse condition. When operating at 1.8-2.2 GHz （20% relative bandwidth）, the amplifier provides an output power higher than 48 dBm （,-~ 65 W）, with a PAE over 70% and a power gain above 15 dB. When operating in continuous-wave （CW） operating conditions, the amplifier gives an output power over 46 dBm （40 W） with PAE beyond 60% over the whole operation frequency range.展开更多
We propose a controllable high-efficiency electrostatic surface trap for cold polar molecules on a chip by using two insulator-embedded charged rings and a grounded conductor plate. We calculate Stark energy structure...We propose a controllable high-efficiency electrostatic surface trap for cold polar molecules on a chip by using two insulator-embedded charged rings and a grounded conductor plate. We calculate Stark energy structure pattern of ND3 molecules in an external electric field using the method of matrix diagonalization. We analyze how the voltages that are applied to the ring electrodes affect the depth of the efficient well and the controllability of the distance between the trap center and the surface of the chip. To obtain a better understanding, we simulate the dynamical loading and trapping processes of ND3 molecules in a ｜J, KM = ｜1,-1 state by using classical Monte–Carlo method. Our study shows that the loading efficiency of our trap can reach ～ 88%. Finally, we study the adiabatic cooling of cold molecules in our surface trap by linearly lowering the potential-well depth（i.e., lowering the trapping voltage）, and find that the temperature of the trapped ND3 molecules can be adiabatically cooled from 34.5 m K to ～ 5.8 m K when the trapping voltage is reduced from-35 k V to-3 k V.展开更多
The paper describes recent trends to carry forward the automation in welding process in Japanese industries.The present situation on the introduction of computer integrated manufacturing is surveyed and its concept an...The paper describes recent trends to carry forward the automation in welding process in Japanese industries.The present situation on the introduction of computer integrated manufacturing is surveyed and its concept and relation among the constituent subsystems are shown.Also recent developments of arc welding processes and related tools are reviewed.They are as follows.1) Schematic image of the structure of computer integrated manufacturing system (CIM).2) Short descriptions for the trend of introducing CIM system.An example of multi-robot welding system in shipyard,virtual factory,network monitoring of welding quality,clarification of welder’s skill.3) Development of high efficiency welding processes.Copper-less wire electrode,tandem large fillet welding,tandem pulse GMA welding,digital wire feeder with new!push-pull system,overhead horizontal tandem GMA welding for ship bottom shell,one-sided fillet groove GMA welding for construction machinery,ultra-NGW hot wire GTA process,Al-alloy sheet welding with laser assisted AC pulsed MIG process.展开更多
A newly designed grating used in terahertz region is proposed, which is composed of the trapezoidal elements repeated successively along one dimension of the substrate, and uniform interval （the grating period） repe...A newly designed grating used in terahertz region is proposed, which is composed of the trapezoidal elements repeated successively along one dimension of the substrate, and uniform interval （the grating period） repeated along the other dimension. The transmission of the grating owns a designable trapezoidal profile dependent on the geometric dimensions of the element. The far-field diffraction patterns of a designed grating at incident broadband terahertz frequencies, with element dimensions of upper, lower side and period of 50, 250, and 300 μm, respectively, are simulated by the scalar diffraction theory. The simulation results indicate that the terahertz grating exhibits a property of single-order diffraction, and the diffraction efficiency of the first order reaches 6.6%, exceeding that of a traditional sinusoidal amplitude grating with identical period and duty cycle. Owing to the regular architecture and the high single-order diffraction efficiency, the grating is easy to fabricate and shows great potential applications in single-shot spectral measurements of weak broadband terahertz pulse.展开更多
A spectrum-splitting and beam-concentrating （SSBC） diffractive optical element （DOE） for three-junction pho- tovoltaics （PV） system is designed and fabricated by five-circ/e micro-fabrication. The incident solar...A spectrum-splitting and beam-concentrating （SSBC） diffractive optical element （DOE） for three-junction pho- tovoltaics （PV） system is designed and fabricated by five-circ/e micro-fabrication. The incident solar light is efficiently split into three sub-spectrum ranges and strongly concentrated on the focal plane, which can be di- rectly utilized by suitable spectrum-matching solar cells. The system concentration factor reaches 12x. Moreover, the designed wavelengths （450nm, 550nm and 65Onto） are spatially distributed on the focal plane, in good agree- ment with the theoretical results. The average optical effic/ency of all the cells over the three designed wavelengths is 60.07%. The SSBC DOE with a high concentration factor and a high optical efficiency provides a cost-effective approach to achieve higher PV conversion efficieneies.展开更多
The relationship between infrared light （IR） and vacuum ultraviolet （VUV） emission in shadow mask plasma display panels （SMPDP） at high xenon content and high voltage is investigated. The respective ratios of VI...The relationship between infrared light （IR） and vacuum ultraviolet （VUV） emission in shadow mask plasma display panels （SMPDP） at high xenon content and high voltage is investigated. The respective ratios of VIS/IR-823 am, VIS/IR-828 nm and of efficacy/VIS/IR-823 nm, efficacy/VIS/IR-823 nm are calculated to determine the behavior of the xenon excitation efficiency and the electron excitation efficiency as a function of the driving voltage and xenon content. It is found that the xenon excitation efficiency is almost independent of the driving voltage, and increases approximately linearly with the xenon content. The values for efficacy/VIS/IR-828 nm increase rapidly with the xenon content, but saturate at a xenon ratio of about 30% while, on the other hand, the efficacy/VIS/IR-823 nm values decrease continuously with the xenon content.展开更多
The versatility and flexibility of organic photoelectric materials endow organic photovoltaic cells fine function modulation and huge commercial potential. In this work, a new noncovalent fused-ring small molecule acc...The versatility and flexibility of organic photoelectric materials endow organic photovoltaic cells fine function modulation and huge commercial potential. In this work, a new noncovalent fused-ring small molecule acceptor(SMA) BID-4 F has been synthesized for high-efficient organic solar cells(OSCs). BID-4 F consists of a diflurobenzothiadiazole(DFBT) core, ladder-like indacenodithiophene(IDT) spacers, and dicyanoindanone electron-withdrawing end groups, which are supposed to be conformationally interlocked by noncovalent interactions, leading to good molecular planarity. In addition, compact solid state stacking was revealed by UV–vis–NIR absorption spectrum. The optimized PM6:BID-4 F based device delivers an eminent power conversion efficiency(PCE) of 12.30% with a high open-circuit voltage(Voc) of 0.92 V and a high fill factor(FF) of 74.3%. Most importantly, the PCE and FF are among one of the highest values reported for the OSCs based on the unfused-ring SMAs. Overall, our work demonstrates that the unfused ring central framework with high molecular planarity through noncovalent interactions provides a good strategy to construct highly efficient SMAs.展开更多
Diffractive lenses(DLs)can realize high-resolution imaging with light weight and compact size.Conventional DLs suffer large chromatic and off-axis aberrations,which significantly limits their practical applications.Al...Diffractive lenses(DLs)can realize high-resolution imaging with light weight and compact size.Conventional DLs suffer large chromatic and off-axis aberrations,which significantly limits their practical applications.Although many achromatic methods have been proposed,most of them are used for designing small aperture DLs,which have low diffraction efficiencies.In the designing of diffractive achromatic lenses,increasing the aperture and improving the diffraction efficiency have become two of the most important design issues.Here,a novel phase-coded diffractive lens(PCDL)for achromatic imaging with a large aperture and high efficiency is proposed and demonstrated experimentally,and it also possesses wide field-of-view(FOV)imaging at the same time.The phase distribution of the conventional phase-type diffractive lens(DL)is coded with a cubic function to expand both the working bandwidth and the FOV of conventional DL.The proposed phase-type DL is fabricated by using the laser direct writing of grey-scale patterns for a PCDL of a diameter of 10 mm,a focal length of 100 mm,and a cubic phase coding parameter of 30π.Experimental results show that the working bandwidth and the FOV of the PCDL respectively reach 50 nm and 16°with over 8%focusing efficiency,which are in significant contrast to the counterparts of conventional DL and in good agreement with the theoretical predictions.This work provides a novel way for implementing the achromatic,wide FOV,and high-efficiency imaging with large aperture DL.展开更多
Nucleophile oxidation reaction(NOR), represented by ethanol oxidation reaction(EOR), is a promising pathway to replace oxygen evolution reaction(OER). EOR can effectively reduce the driving voltage of hydrogen product...Nucleophile oxidation reaction(NOR), represented by ethanol oxidation reaction(EOR), is a promising pathway to replace oxygen evolution reaction(OER). EOR can effectively reduce the driving voltage of hydrogen production in direct water splitting. In this work, large current and high efficiency of EOR on a Ni, Fe layered double hydroxide(NiFe-LDH) catalyst were simultaneously achieved by a facile fluorination strategy. F in NiFe-LDH can reduce the activation energy of the dehydrogenation reaction, thus promoting the deprotonation process of NiFe-LDH to achieve a lower EOR onset potential. It also weakens the absorption of OH-and nucleophile electrooxidation products on the surface of NiFe-LDH at a higher potential, achieving a high current density and EOR selectivity, according to density functional theory calculations. Based on our experiment results, the optimized fluorinated NiFe-LDH catalyst achieves a low potential of 1.386 V to deliver a 10 mA cm^(-2)EOR. Moreover, the Faraday efficiency is greater than 95%, with a current density ranging from 10 to 250 mA cm^(-2). This work provides a promising pathway for an efficient and cost-effective NOR catalyst design for economic hydrogen production.展开更多
All-inorganic CsPbIBr2perovskite solar cells(PSCs)have attracted considerable research attention in recent years due to their excellent thermal stability.However,their power conversion efficiencies(PCEs)are relatively...All-inorganic CsPbIBr2perovskite solar cells(PSCs)have attracted considerable research attention in recent years due to their excellent thermal stability.However,their power conversion efficiencies(PCEs)are relatively low and still far below the theoretical limit.Here,we report the use of an organic dye molecule(namely VG1-C8)as a bifunctional interlayer between perovskite and the hole-transport layer in CsPbIBr2PSCs.Combined experimental and theoretical calculation results disclose that the multiple Lewis base sites in VG1-C8 can effectively passivate the trap states on the perovskite films.Meanwhile,theπ-conjugated dye molecule significantly accelerates the hole extraction from the perovskite absorber as evidenced by the photoluminescence analysis.Consequently,the VG1-C8 treatment simultaneously boosts the photovoltage and photocurrent density values from 1.26 V and 10.80 mA cm^(-2) to 1.31 V and 12.44 m A cm^(-2),respectively.This leads to a significant enhancement of PCE from 9.20%to12.10%under one sun irradiation(AM 1.5G).To our knowledge,this is the record efficiency reported so far for CsPbIBr_(2) PSCs.Thus,the present work demonstrates an effective interfacial passivation strategy for the development of highly efficient PSCs.展开更多
High efficiency, stable organic light-emitting diodes （OLEDs） based on 2-pheyl-4＇-carbazole-9-H-Thioxanthen-9- one-10, 10-dioxide （TXO-PhCz） with different doping concentration are constructed. The stability of t...High efficiency, stable organic light-emitting diodes （OLEDs） based on 2-pheyl-4＇-carbazole-9-H-Thioxanthen-9- one-10, 10-dioxide （TXO-PhCz） with different doping concentration are constructed. The stability of the encap- sulated devices are investigated in detail. The devices with the 10 wt% doped TXO-PhCz emitter layer （EML） show the best performance with a current efficiency of 52.1 cd/A, a power efficiency of 32.71re^W, and an external quantum efficiency （EQE） of 17.7%. The devices based on the lOwt%-doped TXO-PhCz EML show the best operational stability with a half-life time （LTSO） of 8Oh, which is 8 h longer than that of the reference devices based on fac-tris（2-phenylpyridinato）iridium（ Ⅲ） （Ir（ppy）a）. These indicate excellent stability of TXO-PhCz for redox and oxidation processes under electrical excitation and TXO-PhCz can be potentially used as the emitters for OLEDs with high efficiency and excellent stability. The high-performance device based on TXO-PhCz with high stability can be further improved by the optimization of the encapsulation technology and the development of a new host for TXO-PhCz.展开更多
This paper presents a novel coupled receiver-transmitter metasurface(MS)which is used to realize a high-aperture-efficiency Fabry-Perot resonator antenna.The unit cell of the MS adopts a slot-coupling procedure to rea...This paper presents a novel coupled receiver-transmitter metasurface(MS)which is used to realize a high-aperture-efficiency Fabry-Perot resonator antenna.The unit cell of the MS adopts a slot-coupling procedure to realize energy transmission from the receiver patch to the radiator patch.This approach makes it easier to independently control the transmission magnitude and phase.Based on this characteristic,the transmission coefficients of different unit cells on the MS can be optimized by a genetic algorithm.Then,nearly uniform electric amplitude and phase distribution across the aperture field of the antenna are achieved.Therefore,the gain and aperture efficiency of the antenna are improved.A prototype of the optimized antenna is fabricated and measured to validate the design.The measured gain of the fabricated antenna reaches 17.3 dBi with an aperture efficiency of 94.5%.A higher aperture efficiency is obtained with the proposed antenna which has a low profile and simple structure.展开更多
High Efficiency Video Coding (HEVC) is the latest international video coding standard, which can provide the similar quality with about half bandwidth compared with its predecessor, H.264/MPEG?4 AVC. To meet the requi...High Efficiency Video Coding (HEVC) is the latest international video coding standard, which can provide the similar quality with about half bandwidth compared with its predecessor, H.264/MPEG?4 AVC. To meet the requirement of higher bit depth coding and more chroma sampling formats, range extensions of HEVC were developed. This paper introduces the coding tools in HEVC range extensions and provides experimental results to compare HEVC range extensions with previous video coding standards. Ex?perimental results show that HEVC range extensions improve coding efficiency much over H.264/MPEG?4 AVC High Predictive profile, especially for 4K sequences.展开更多
基金support provided by the Shenzhen-Hong Kong Science and Technology Innovation Cooperation Zone Shenzhen Park Project(HZQB-KCZYB-2020030)the Research Grants Council of Hong Kong(Project No:AoE/M-402/20.)+1 种基金the Open Project of Yunnan Precious Metals Laboratory Co.,Ltd(YPML-2023050248)the Hong Kong Innovation and Technology Commission via the Hong Kong Branch of National Precious Metals Material Engineering Research Center.
文摘Solar steam generation(SSG)is widely regarded as one of the most sustainable technologies for seawater desalination.However,salt fouling severely compromises the evaporation performance and lifetime of evaporators,limiting their practical applications.Herein,we propose a hierarchical salt-rejection(HSR)strategy to prevent salt precipitation during long-term evaporation while maintaining a rapid evaporation rate,even in high-salinity brine.The salt diffusion process is segmented into three steps—insulation,branching diffusion,and arterial transport—that significantly enhance the salt-resistance properties of the evaporator.Moreover,the HSR strategy overcomes the tradeoff between salt resistance and evaporation rate.Consequently,a high evaporation rate of 2.84 kg m^(-2) h^(-1),stable evaporation for 7 days cyclic tests in 20 wt%NaCl solution,and continuous operation for 170 h in natural seawater under 1 sun illumination were achieved.Compared with control evaporators,the HSR evaporator exhibited a>54%enhancement in total water evaporation mass during 24 h continuous evaporation in 20 wt%salt water.Furthermore,a water collection device equipped with the HSR evaporator realized a high water purification rate(1.1 kg m^(-2) h^(-1)),highlighting its potential for agricultural applications.
文摘Two new AlTiN coated cemented carbide drills with Al content of 40% and 55% in weight are developed for high efficiency dry drilling of 40Cr. By studying tool durability, machined hole quality, tool wear mechanism, chip deformation, and lubrication, the dry drilling performance of the two kinds of coated drills is analyzed. Experimental results show that the AlTiN coated drills are suitable for high efficiency dry drilling and can obtain higher quality of machined holes. The tool durability of the drill with 55% Al content is 1. 3 times of that of the drill with 40% Al content at the cutting speed of 90 m/min. The wear mechanism of two AlTiN coatings are studied in experiments. During dry drilling process, oxidative wear appears in both two kinds of drills. The oxide film is formed on the top of the coated drill containing Al content of 55%. And the oxide film helps to increase its high temperature resistance and decrease the coating flaking, thus the drill is failed because of coating subsidence. The drill with less Al content is failed due to peeling and breakage. The lubricated condition in dry drilling is improved by the high Al content coating. It helps to reduce the cutting deformation and benefits to improve the quality of machined holes. The AlTiN coating with higher Al content shows longer tool life and higher quality of machined holes in high efficiency dry drilling. Its tool life increases by 30% compared with that of the coating with less Al content.
文摘Green manufacturing （GM） and high efficiency machining technology are inevitable trends in the field of advanced manufacturing of the 21st century. To ensure green and high-efficiency machining, a new high efficiency cooling technology-cryogenic pneumatic mist jet impinging cooling （CPMJI） technology is presented. For obtaining the best cooling effect, a little quantity of coolant is carried by high speed cryogenic air （-20 C ） and reaches the machining zone in the form of mist jet to enhance heat transfer. Experimental results indicate that under the conditions of 40 m/s in the jet impinging speed and 10 mm in the jet impinging distance, the critical heat flux（CHF） nearly reaches 6× 10^7 W/m^2, more than six times of the CHF of the grinding burn with a value of （8～10）×10^6 W/m^2.
基金supported by the Graduate Student Education Teaching Reform Project,China(Grant No.JG201512)the Young Teachers Research Project of Yanshan University,China(Grant No.13LGB028)
文摘The lead-free perovskite solar cells(PSCs) have drawn a great deal of research interest due to the Pb toxicity of the lead halide perovskite.CHNHSnIis a viable alternative to CHNHPbX,because it has a narrower band gap of 1.3 eV and a wider visible absorption spectrum than the lead halide perovskite.The progress of fabricating tin iodide PSCs with good stability has stimulated the studies of these CHNHSnIbased cells greatly.In the paper,we study the influences of various parameters on the solar cell performance through theoretical analysis and device simulation.It is found in the simulation that the solar cell performance can be improved to some extent by adjusting the doping concentration of the perovskite absorption layer and the electron affinity of the buffer and HTM,while the reduction of the defect density of the perovskite absorption layer significantly improves the cell performance.By further optimizing the parameters of the doping concentration(1.3 × 10cm~3) and the defect density(1 × 10cm~3) of perovskite absorption layer,and the electron affinity of buffer(4.0 eV) and HTM(2.6 eV),we finally obtain some encouraging results of the Jof 31.59 mA/cm~2,Vof 0.92 V,FF of 79.99%,and PCE of 23.36%.The results show that the lead-free CHNHSnIPSC is a potential environmentally friendly solar cell with high efficiency.Improving the Snstability and reducing the defect density of CHNHSnIare key issues for the future research,which can be solved by improving the fabrication and encapsulation process of the cell.
基金the National Basic Research Program of China(Grant No.2009CB623604)the National Natural Science Foundation of China(Grant Nos.61204087,51173049,U0634003,61036007,and 60937001)+1 种基金the Fundamental Research Funds for the Central Universities,China(Grant Nos.2011ZB0002 and 2011ZM0009)China Postdoctoral Science Foundation
文摘High-brightness and color-stable two-wavelength hybrid white organic light emitting diodes （HWOLEDs） with the configuration of indium tin oxide （ITO）/ N, N, N, N-tetrakis（4-methoxyphenyl）-benzidine （MeO-TPD）： tetrafluoro-tetracyanoqino dimethane （F4-TCNQ）/N,N-di（naphthalene-1-yl）-N,N-diphenyl-benzidine （NPB）/ 4,4-N,N-dicarbazolebiphenyl （CBP）： iridium （III） diazine complexes （MPPZ） 2 Ir（acac）/NPB/2-methyl-9,10-di（2-naphthyl）anthracene （MADN）： p-bis（p-N,N-di-phenyl-aminostyryl）benzene （DSA-ph）/bis（10-hydroxybenzo[h] quino-linato）beryllium complex （Bebq2）/LiF/Al have been fabricated and characterized. The optimal brightness of the device is 69932 cd/m2 at a voltage of 13 V, and the Commission Internationale de l’Eclairage （CIE） chromaticity coordinates are almost constant during a large voltage change of 6–12 V. Furthermore, a current efficiency of 15.3 cd/A at an illumination-relevant brightness of 1000 cd/m2 is obtained, which rolls off slightly to 13.0 cd/A at an ultra high brightness of 50000 cd/m2. We attribute this great performance to wisely selecting an appropriate spacer together with effectively utilizing the combinations of exciton-harvested orange-phosphorescence/blue-fluorescence in the device. Undoubtedly, this is one of the most exciting results in two-wavelength HWOLEDs up to now.
基金Financial provided by the National Natural Science Foundation of China (Nos. 51574123 and U1361118)the China Postdoctoral Science Foundation (No. 2015M 582118)
文摘To master theoretical calculation for dust removal efficiency of high pressure atomization in an underground coal mine, the corresponding atomization characteristics and dust removal efficiency were both comprehensively studied in theory by virtue of related theories of hydromechanics and aerosol.According to actual measurements of flow coefficients and atomization angles of X-type swirl nozzle,computational formula was derived for atomized particle sizes of such a nozzle in conjunction with relevant empirical equation. Moreover, a mathematical model for applying high pressure atomization to dust removal in underground coal mine was also established to deduce theoretical computation formula of fractional efficiency. Then, Matlab was adopted to portray the relation curve between fractional efficiency and influence factors. In addition, a theoretical formula was also set up for removal efficiency of respirable dust and total coal dust based on dust size and frequency distribution equations. In the end,impacts of dust characteristic parameters on various dust removal efficiencies were analyzed.
基金supported by the National Science Foundation of China(No.51907193,51822706 and 51777200)the Beijing Natural Science foundation(JQ19012)+2 种基金the Key Research Program of Frontier Sciences,CAS(No.ZDBS-LY-JSC047)the Youth Innovation Promotion Association,CAS(No.2020145)the Dalian National Laboratory for Clean Energy Cooperation Fund,the CAS(Nos.DNL201912,DNL201915).
文摘Sodium-ion capacitors(SICs)have attracted appreciable attention in virtue of the higher energy and power densities compared with their rivals,supercapacitors and sodium-ion batteries.Due to the lack of sodium resources in cathode,presodiation is critical for SICs to further augment performances.However,current presodiation strategy utilizes metallic sodium as the presodiation material.In this strategy,assembling/disassembling of half-cells is required,which is dangerous and in creases the time and cost of SIC leading to the restriction of their industrialization and commercialization.Herein we present a safe,low-cost and high-efficiency presodiation strategy by first employing Na_(2)C_(2)O_(4) as the sacrificial salt applied in SICs.Na_(2)C_(2)O_(4) is environmentally friendly and possesses considerably low expenditure.No additional residues remain after sodium extraction ascribed to its"zero dead mass"property.When paired with commercial activated carb on as the cathode and commercial hard carbon as the ano de,the constructed pouch-type SICs exhibit high energy and power densities of 91.7 Wh/kg and 13.1 kW/kg,respectively.This work shows a prospect of realizing the safe and low-cost manufacturing for high-performance SICs commercially.
基金Project supported by the National Natural Science Foundation of China(Grant No.61203211)the Natural Science Foundation of Jiangsu Higher Education Institutions of China(Grant No.13KJB140006)the Foundation for Outstanding Young Teachers of Nanjing University of Information Science&Technology,China(Grant No.20110423)
文摘In this paper, we present a high-efficiency S-band gallium nitride （GaN） power amplifier （PA）. This amplifier is fabri- cated based on a self-developed GaN high-electron-mobility transistor （HEMT） with 10 mm gate width on SiC substrate. Harmonic manipulation circuits are presented in the amplifier. The matching networks consist of microstrip lines and discrete components. Open-circuited stub lines in both input and output are used to tune the 2rid harmonic wave and match the GaN HEMT to the highest efficiency condition. The developed amplifier delivers an output power of 48.5 dBm （70 W） with a power-added efficiency （PAE） of 72.2% at 2 GHz in pulse condition. When operating at 1.8-2.2 GHz （20% relative bandwidth）, the amplifier provides an output power higher than 48 dBm （,-~ 65 W）, with a PAE over 70% and a power gain above 15 dB. When operating in continuous-wave （CW） operating conditions, the amplifier gives an output power over 46 dBm （40 W） with PAE beyond 60% over the whole operation frequency range.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.10674047,10804031,10904037,10904060,10974055,11034002,and61205198)the National Key Basic Research and Development Program of China(Grant Nos.2006CB921604 and 2011CB921602)+2 种基金the Basic Key Program of Shanghai Municipality,China(Grant No.07JC14017)the Fundamental Research Funds for the Central Universitiesthe Shanghai Leading Academic Discipline Project,China(Grant No.B408)
文摘We propose a controllable high-efficiency electrostatic surface trap for cold polar molecules on a chip by using two insulator-embedded charged rings and a grounded conductor plate. We calculate Stark energy structure pattern of ND3 molecules in an external electric field using the method of matrix diagonalization. We analyze how the voltages that are applied to the ring electrodes affect the depth of the efficient well and the controllability of the distance between the trap center and the surface of the chip. To obtain a better understanding, we simulate the dynamical loading and trapping processes of ND3 molecules in a ｜J, KM = ｜1,-1 state by using classical Monte–Carlo method. Our study shows that the loading efficiency of our trap can reach ～ 88%. Finally, we study the adiabatic cooling of cold molecules in our surface trap by linearly lowering the potential-well depth（i.e., lowering the trapping voltage）, and find that the temperature of the trapped ND3 molecules can be adiabatically cooled from 34.5 m K to ～ 5.8 m K when the trapping voltage is reduced from-35 k V to-3 k V.
文摘The paper describes recent trends to carry forward the automation in welding process in Japanese industries.The present situation on the introduction of computer integrated manufacturing is surveyed and its concept and relation among the constituent subsystems are shown.Also recent developments of arc welding processes and related tools are reviewed.They are as follows.1) Schematic image of the structure of computer integrated manufacturing system (CIM).2) Short descriptions for the trend of introducing CIM system.An example of multi-robot welding system in shipyard,virtual factory,network monitoring of welding quality,clarification of welder’s skill.3) Development of high efficiency welding processes.Copper-less wire electrode,tandem large fillet welding,tandem pulse GMA welding,digital wire feeder with new!push-pull system,overhead horizontal tandem GMA welding for ship bottom shell,one-sided fillet groove GMA welding for construction machinery,ultra-NGW hot wire GTA process,Al-alloy sheet welding with laser assisted AC pulsed MIG process.
基金Project supported by the National Key Research and Development Program of China(Grant No.2017YFB05033)the National Science Instruments Major Project of China(Grant No.2012YQ130125)
文摘A newly designed grating used in terahertz region is proposed, which is composed of the trapezoidal elements repeated successively along one dimension of the substrate, and uniform interval （the grating period） repeated along the other dimension. The transmission of the grating owns a designable trapezoidal profile dependent on the geometric dimensions of the element. The far-field diffraction patterns of a designed grating at incident broadband terahertz frequencies, with element dimensions of upper, lower side and period of 50, 250, and 300 μm, respectively, are simulated by the scalar diffraction theory. The simulation results indicate that the terahertz grating exhibits a property of single-order diffraction, and the diffraction efficiency of the first order reaches 6.6%, exceeding that of a traditional sinusoidal amplitude grating with identical period and duty cycle. Owing to the regular architecture and the high single-order diffraction efficiency, the grating is easy to fabricate and shows great potential applications in single-shot spectral measurements of weak broadband terahertz pulse.
基金Supported by the National Natural Science Foundation of China under Grant Nos 91233202,91433205 and 51421002the Chinese Academy of Sciences
文摘A spectrum-splitting and beam-concentrating （SSBC） diffractive optical element （DOE） for three-junction pho- tovoltaics （PV） system is designed and fabricated by five-circ/e micro-fabrication. The incident solar light is efficiently split into three sub-spectrum ranges and strongly concentrated on the focal plane, which can be di- rectly utilized by suitable spectrum-matching solar cells. The system concentration factor reaches 12x. Moreover, the designed wavelengths （450nm, 550nm and 65Onto） are spatially distributed on the focal plane, in good agree- ment with the theoretical results. The average optical effic/ency of all the cells over the three designed wavelengths is 60.07%. The SSBC DOE with a high concentration factor and a high optical efficiency provides a cost-effective approach to achieve higher PV conversion efficieneies.
基金supported by National Natural Science Foundation of China (No. 60571033)the National Hi'Tech projects of China (No. 2008AA03A308)Programme of Introducing Talents of Discipline to Universities of China (B07027)
文摘The relationship between infrared light （IR） and vacuum ultraviolet （VUV） emission in shadow mask plasma display panels （SMPDP） at high xenon content and high voltage is investigated. The respective ratios of VIS/IR-823 am, VIS/IR-828 nm and of efficacy/VIS/IR-823 nm, efficacy/VIS/IR-823 nm are calculated to determine the behavior of the xenon excitation efficiency and the electron excitation efficiency as a function of the driving voltage and xenon content. It is found that the xenon excitation efficiency is almost independent of the driving voltage, and increases approximately linearly with the xenon content. The values for efficacy/VIS/IR-828 nm increase rapidly with the xenon content, but saturate at a xenon ratio of about 30% while, on the other hand, the efficacy/VIS/IR-823 nm values decrease continuously with the xenon content.
基金supported by the National Key Research and Development Program of China (2017YFA0206600)the National Natural Science Foundation of China (21875286)the Science Fund for Distinguished Young Scholars of Hunan Province (2017JJ1029)。
文摘The versatility and flexibility of organic photoelectric materials endow organic photovoltaic cells fine function modulation and huge commercial potential. In this work, a new noncovalent fused-ring small molecule acceptor(SMA) BID-4 F has been synthesized for high-efficient organic solar cells(OSCs). BID-4 F consists of a diflurobenzothiadiazole(DFBT) core, ladder-like indacenodithiophene(IDT) spacers, and dicyanoindanone electron-withdrawing end groups, which are supposed to be conformationally interlocked by noncovalent interactions, leading to good molecular planarity. In addition, compact solid state stacking was revealed by UV–vis–NIR absorption spectrum. The optimized PM6:BID-4 F based device delivers an eminent power conversion efficiency(PCE) of 12.30% with a high open-circuit voltage(Voc) of 0.92 V and a high fill factor(FF) of 74.3%. Most importantly, the PCE and FF are among one of the highest values reported for the OSCs based on the unfused-ring SMAs. Overall, our work demonstrates that the unfused ring central framework with high molecular planarity through noncovalent interactions provides a good strategy to construct highly efficient SMAs.
基金the National Natural Science Foundation of China(Grant No.61775154)the Natural Science Foundation of the Jiangsu Higher Education Institutions,China(Grant No.18KJB140015)+1 种基金the Priority Academic Program Development of Jiangsu Higher Education Institutions,Chinathe Open Research Fund of CAS Key Laboratory of Space Precision Measurement Technology,China(Grant No.SPMT2021001)。
文摘Diffractive lenses(DLs)can realize high-resolution imaging with light weight and compact size.Conventional DLs suffer large chromatic and off-axis aberrations,which significantly limits their practical applications.Although many achromatic methods have been proposed,most of them are used for designing small aperture DLs,which have low diffraction efficiencies.In the designing of diffractive achromatic lenses,increasing the aperture and improving the diffraction efficiency have become two of the most important design issues.Here,a novel phase-coded diffractive lens(PCDL)for achromatic imaging with a large aperture and high efficiency is proposed and demonstrated experimentally,and it also possesses wide field-of-view(FOV)imaging at the same time.The phase distribution of the conventional phase-type diffractive lens(DL)is coded with a cubic function to expand both the working bandwidth and the FOV of conventional DL.The proposed phase-type DL is fabricated by using the laser direct writing of grey-scale patterns for a PCDL of a diameter of 10 mm,a focal length of 100 mm,and a cubic phase coding parameter of 30π.Experimental results show that the working bandwidth and the FOV of the PCDL respectively reach 50 nm and 16°with over 8%focusing efficiency,which are in significant contrast to the counterparts of conventional DL and in good agreement with the theoretical predictions.This work provides a novel way for implementing the achromatic,wide FOV,and high-efficiency imaging with large aperture DL.
基金the financial support from the National Natural Science Foundation of China (22197121)Knowledge Innovation Program of Wuhan-Basic Research (2022010801010202)Research Fund Program of Guangdong Provincial Key Laboratory of Fuel Cell Technology (FC202201)。
文摘Nucleophile oxidation reaction(NOR), represented by ethanol oxidation reaction(EOR), is a promising pathway to replace oxygen evolution reaction(OER). EOR can effectively reduce the driving voltage of hydrogen production in direct water splitting. In this work, large current and high efficiency of EOR on a Ni, Fe layered double hydroxide(NiFe-LDH) catalyst were simultaneously achieved by a facile fluorination strategy. F in NiFe-LDH can reduce the activation energy of the dehydrogenation reaction, thus promoting the deprotonation process of NiFe-LDH to achieve a lower EOR onset potential. It also weakens the absorption of OH-and nucleophile electrooxidation products on the surface of NiFe-LDH at a higher potential, achieving a high current density and EOR selectivity, according to density functional theory calculations. Based on our experiment results, the optimized fluorinated NiFe-LDH catalyst achieves a low potential of 1.386 V to deliver a 10 mA cm^(-2)EOR. Moreover, the Faraday efficiency is greater than 95%, with a current density ranging from 10 to 250 mA cm^(-2). This work provides a promising pathway for an efficient and cost-effective NOR catalyst design for economic hydrogen production.
基金the financial support by the National Natural Science Foundation of China(52161145408 and21975038)the Fundamental Research Funds for the Central Universities(DUT20RC(3)085)。
文摘All-inorganic CsPbIBr2perovskite solar cells(PSCs)have attracted considerable research attention in recent years due to their excellent thermal stability.However,their power conversion efficiencies(PCEs)are relatively low and still far below the theoretical limit.Here,we report the use of an organic dye molecule(namely VG1-C8)as a bifunctional interlayer between perovskite and the hole-transport layer in CsPbIBr2PSCs.Combined experimental and theoretical calculation results disclose that the multiple Lewis base sites in VG1-C8 can effectively passivate the trap states on the perovskite films.Meanwhile,theπ-conjugated dye molecule significantly accelerates the hole extraction from the perovskite absorber as evidenced by the photoluminescence analysis.Consequently,the VG1-C8 treatment simultaneously boosts the photovoltage and photocurrent density values from 1.26 V and 10.80 mA cm^(-2) to 1.31 V and 12.44 m A cm^(-2),respectively.This leads to a significant enhancement of PCE from 9.20%to12.10%under one sun irradiation(AM 1.5G).To our knowledge,this is the record efficiency reported so far for CsPbIBr_(2) PSCs.Thus,the present work demonstrates an effective interfacial passivation strategy for the development of highly efficient PSCs.
基金Supported by the National Natural Science Foundation of China under Grant Nos 61420106002,51373189,61178061,and 61227008the Hundred Talents Program of the Chinese Academy of Sciences,the National Basic Research Program of China under Grant No 2014CB932600the Start-Up Fund of the Technical Institute of Physics and Chemistry of the Chinese Academy of Sciences
文摘High efficiency, stable organic light-emitting diodes （OLEDs） based on 2-pheyl-4＇-carbazole-9-H-Thioxanthen-9- one-10, 10-dioxide （TXO-PhCz） with different doping concentration are constructed. The stability of the encap- sulated devices are investigated in detail. The devices with the 10 wt% doped TXO-PhCz emitter layer （EML） show the best performance with a current efficiency of 52.1 cd/A, a power efficiency of 32.71re^W, and an external quantum efficiency （EQE） of 17.7%. The devices based on the lOwt%-doped TXO-PhCz EML show the best operational stability with a half-life time （LTSO） of 8Oh, which is 8 h longer than that of the reference devices based on fac-tris（2-phenylpyridinato）iridium（ Ⅲ） （Ir（ppy）a）. These indicate excellent stability of TXO-PhCz for redox and oxidation processes under electrical excitation and TXO-PhCz can be potentially used as the emitters for OLEDs with high efficiency and excellent stability. The high-performance device based on TXO-PhCz with high stability can be further improved by the optimization of the encapsulation technology and the development of a new host for TXO-PhCz.
基金Project supported by the National Natural Science Foundation of China(Grant No.61871394)Natural Science Foundation of Shanxi Province,China(Grant No.2020JQ-482).
文摘This paper presents a novel coupled receiver-transmitter metasurface(MS)which is used to realize a high-aperture-efficiency Fabry-Perot resonator antenna.The unit cell of the MS adopts a slot-coupling procedure to realize energy transmission from the receiver patch to the radiator patch.This approach makes it easier to independently control the transmission magnitude and phase.Based on this characteristic,the transmission coefficients of different unit cells on the MS can be optimized by a genetic algorithm.Then,nearly uniform electric amplitude and phase distribution across the aperture field of the antenna are achieved.Therefore,the gain and aperture efficiency of the antenna are improved.A prototype of the optimized antenna is fabricated and measured to validate the design.The measured gain of the fabricated antenna reaches 17.3 dBi with an aperture efficiency of 94.5%.A higher aperture efficiency is obtained with the proposed antenna which has a low profile and simple structure.
文摘High Efficiency Video Coding (HEVC) is the latest international video coding standard, which can provide the similar quality with about half bandwidth compared with its predecessor, H.264/MPEG?4 AVC. To meet the requirement of higher bit depth coding and more chroma sampling formats, range extensions of HEVC were developed. This paper introduces the coding tools in HEVC range extensions and provides experimental results to compare HEVC range extensions with previous video coding standards. Ex?perimental results show that HEVC range extensions improve coding efficiency much over H.264/MPEG?4 AVC High Predictive profile, especially for 4K sequences.
