Nuclear charge density distribution plays an important role in both nuclear and atomic physics,for which the two-parameter Fermi(2pF)model has been widely applied as one of the most frequently used models.Currently,th...Nuclear charge density distribution plays an important role in both nuclear and atomic physics,for which the two-parameter Fermi(2pF)model has been widely applied as one of the most frequently used models.Currently,the feedforward neural network has been employed to study the available 2pF model parameters for 86 nuclei,and the accuracy and precision of the parameter-learning effect are improved by introducing A^(1∕3)into the input parameter of the neural network.Furthermore,the average result of multiple predictions is more reliable than the best result of a single prediction and there is no significant difference between the average result of the density and parameter values for the average charge density distribution.In addition,the 2pF parameters of 284(near)stable nuclei are predicted in this study,which provides a reference for the experiment.展开更多
The ion density distribution in the reaction chamber was diagnosed by a Langmuir probe. The rules of the ion density distribution were obtained under the pressures of 9 Pa, 13 Pa, 27 Pa and 53 Pa in the reaction chamb...The ion density distribution in the reaction chamber was diagnosed by a Langmuir probe. The rules of the ion density distribution were obtained under the pressures of 9 Pa, 13 Pa, 27 Pa and 53 Pa in the reaction chamber, different radio-frequency powers and different positions. The result indicates that the ion density decreases as the pressure increases, and increases as the power decreases. The ion density of axial position z =0 achieves 5.8×1010 on the center of coil under the power of 200 w and pressure of 9 Pa in the reaction chamber.展开更多
The uniformity of current density distribution upon electrodes is one of the most important factors determining the lithium dendrites growth and cycling performance of lithium metal batteries(LMBs). Herein,current den...The uniformity of current density distribution upon electrodes is one of the most important factors determining the lithium dendrites growth and cycling performance of lithium metal batteries(LMBs). Herein,current density distributions of lithium metal anodes induced by various engineering factors, consisting of uneven cathode, electrolyte distribution, and different tab positions, and their effects on the electrochemical performance are investigated theoretically and experimentally in pouch cells. The deviation of current density in lithium metal anodes ranges from 2.47% to 196.18% due to the different levels of uneven cathode materials. However, the deviation is just 13.60% for different electrolyte thicknesses between cathodes and anodes, even a ten-layer separator in some positions. The maximum deviation for variational tab positions is only 0.17%. The nonuniformity in current density distribution results in severe dendrite growth issues and poor electrochemical performance of LMBs. This work not only confirms the direct correlation between the uneven current density distribution and lithium deposition behaviors, but also points out the decisive effects of cathode surface roughness on current distribution of anodes, to which more attentions should be paid in practical applications of LMBs.展开更多
In this paper,the penetration mechanism of reactive jet with non-uniform density distribution is studied.The simulations show that the density deficit occurs in the whole reactive jet,and the density increases from th...In this paper,the penetration mechanism of reactive jet with non-uniform density distribution is studied.The simulations show that the density deficit occurs in the whole reactive jet,and the density increases from the jet tip to tail.The density of jet tip is approximately 1.5 g/cm3,which is lower than that of the reactive liner materials.The X-ray experiments show similar results with the simulations.The density decreasing effect of jet tip has a significant influence on the penetration behavior when the reactive jet impacts steel plate.According to the simulation results,this paper assumes that the density gradient in the jet section has linear distribution.Then,the deflagration pressure generated by each jet element at the bottom of crater is introduced into the Bernoulli equation.Based on the virtual origin model and Szendrei-Held equation,the analytical models for penetration depth and radial cratering of reactive jet with the density reduction are obtained.Moreover,to further prove the validity of analytical models,the penetration experiments of the reactive liner shaped charge against steel plate under different standoffs are carried out.There is a convergence between the analytical crater profiles and experimental results when reactive jets penetrate steel plates under different standoffs,especially at standoff of 1.5 and 2.0charge diameters.展开更多
A two-dimensional, three-temperature radiation magneto-hydrodynamics model is applied to the investigation of evolutional trends in x-ray radiation power, energy, peak plasma temperature and density as functions of dr...A two-dimensional, three-temperature radiation magneto-hydrodynamics model is applied to the investigation of evolutional trends in x-ray radiation power, energy, peak plasma temperature and density as functions of drive current rise-time and initial load density distribution by using the typical experimental parameters of tungsten wire-array Z- pinch on the Qiangguang-I generator. The numerical results show that as the drive current rise-time is shortened, x-ray radiation peak power, energy, peak plasma density and peak ion temperature increase approximately linearly, but among them the x-ray radiation peak power increases more quickly. As the initial plasma density distribution in the radial direction becomes gradually flattened, the peak radiation power and the peak ion-temperature almost exponentially increase, while the radiation energy and the peak plasma density change only a little. The main effect of shortening drive current rise-time is to enhance compression of plasma, and the effect of flattening initial load density distribution in the radial direction is to raise the plasma temperature. Both of the approaches elevate the x-ray peak radiation power展开更多
Electron density plays an important role in determining the properties of functional materials.Revealing the electron density distribution experimentally in real space can help to tune the properties of materials.Spin...Electron density plays an important role in determining the properties of functional materials.Revealing the electron density distribution experimentally in real space can help to tune the properties of materials.Spinel Li Mn2 O4 is one of the most promising cathode candidates because of its high voltage,low cost,and non-toxicity,but suffers severe capacity fading during electrochemical cycling due to the Mn dissolution.Real-space measurement of electron distribution of Li Mn2 O4 experimentally can provide direct evaluation on the strength of Mn–O bond and give an explanation of the structure stability.Here,through high energy synchrotron powder x-ray diffraction(SPXRD),accurate electron density distribution in spinel Li Mn2 O4 has been investigated based on the multipole model.The electron accumulation between Mn and O atoms in deformation density map indicates the shared interaction of Mn–O bond.The quantitative topological analysis at bond critical points shows that the Mn–O bond is relatively weak covalent interaction due to the oxygen loss.These findings suggest that oxygen stoichiometry is the key factor for preventing the Mn dissolution and capacity fading.展开更多
We perform an experimental study of two-dimensional（2D） electron density profiles of the laser-induced plasma plumes in air by ordinarily laboratorial interferometry. The electron density distributions measured show...We perform an experimental study of two-dimensional（2D） electron density profiles of the laser-induced plasma plumes in air by ordinarily laboratorial interferometry. The electron density distributions measured show a feature of hollow core. To illustrate the feature, we present a theoretical investigation by using dynamics analysis. In the simulation, the propagation of laser pulse with the evolution of electron density is utilized to evaluate ionization of air target for the plasma-formation stage. In the plasma-expansion stage, a simple adiabatic fluid dynamics is used to calculate the evolution of plasma outward expansion. The simulations show good agreements with experimental results, and demonstrate an effective way of determining 2D density profiles of the laser-induced plasma plume in gas.展开更多
Propellant ionization in the Hall thruster discharge channel is a significant process and has strong influence on the thruster＇s efficiency. In this work, the functional relation has been established between the ioni...Propellant ionization in the Hall thruster discharge channel is a significant process and has strong influence on the thruster＇s efficiency. In this work, the functional relation has been established between the ionization density distribution and the function of the ion energy distribution through the basic equations governing the ion flow in the Hall thruster channel and the method achieved for reconstructing the ionization density distribution inside the channel by ordinary plasma diagnosis of the potential distribution and ion energy spectrum of the plasma jet. The ionization density distributions of single and double charged ions in an ATON-thruster channel have been reconstructed according to the experimental data of the potential distribution along the axis of the channel and the ion energy spectrum of the plasma jet. The agreement between the calculation and experimental results of the percentage of double charged ions proves the validity of our method achieved in this work.展开更多
The distributions of traps and electron density in the interfaces between polyimide （PI） matrix and Al2O3 nanoparticles are researched using the isothermal decay current and the small-angle x-ray scattering （SAXS）...The distributions of traps and electron density in the interfaces between polyimide （PI） matrix and Al2O3 nanoparticles are researched using the isothermal decay current and the small-angle x-ray scattering （SAXS） tests. According to the electron density distribution for quasi two-phase mixture doped by spherical nanoparticles, the electron densities in the interfaces of PI/Al2O3 nanocomposite films are evaluated. The trap level density and carrier mobility in the interface are studied. The experimental results show that the distribution and the change rate of the electron density in the three layers of interface are different, indicating different trap distributions in the interface layers. There is a maximum trap level density in the second layer, where the maximum trap level density for the nanocomposite film doped by 25 wt% is 1.054 × 10^22 eV·m^-3 at 1.324eV, resulting in the carrier mobility reducing. In addition, both the thickness and the electron density of the nanocomposite film interface increase with the addition of the doped Al2O3 contents. Through the study on the trap level distribution in the interface, it is possible to further analyze the insulation mechanism and to improve the performance of nano-dielectric materials.展开更多
In this work, a bridge density functional approximation （BDFA） （J. Chem. Phys. 112, 8079 （2000）） for a nonuniform hard-sphere fluid is extended to a non-uniform hard-core repulsive Yukawa （HCRY） fluid. It is f...In this work, a bridge density functional approximation （BDFA） （J. Chem. Phys. 112, 8079 （2000）） for a nonuniform hard-sphere fluid is extended to a non-uniform hard-core repulsive Yukawa （HCRY） fluid. It is found that the choice of a bulk bridge functional approximation is crucial for both a uniform HCRY fluid and a non-uniform HCRY fluid. A new bridge functional approximation is proposed, which can accurately predict the radial distribution function of the bulk HCRY fluid. With the new bridge functional approximation and its associated bulk second order direct correlation function as input, the BDFA can be used to well calculate the density profile of the HCRY fluid subjected to the influence of varying external fields, and the theoretical predictions are in good agreement with the corresponding simulation data. The calculated results indicate that the present BDFA captures quantitatively the phenomena such as the coexistence of solid-like high density phase and low density gas phase, and the adsorption properties of the HCRY fluid, which qualitatively differ from those of the fluids combining both hard-core repulsion and an attractive tail.展开更多
The experimental data of the isotopic distribution for projectile-like fragments are presented for the 17,18N ＋ 197Au reaction at 33 MeV/u. The width of the isotopic distributions for lSN projectile is significantly ...The experimental data of the isotopic distribution for projectile-like fragments are presented for the 17,18N ＋ 197Au reaction at 33 MeV/u. The width of the isotopic distributions for lSN projectile is significantly broader than that for 17N projectile, and the average N/Z ratio of the former shifts to higher neutron number side. As long as the realistic nucleon density distribution is used, the isotopic distribution for fragments is reproduced by the simple abrasion-ablation model calculation, which thus provides an independent way to determine the surface distribution of the nuclear matter density for neutron-rich nuclei.展开更多
The spatial distributions of different kinds of ions are usually not completely the same in the process of extracting.In order to study the reason for the different characteristics of ion extraction, a simplified simu...The spatial distributions of different kinds of ions are usually not completely the same in the process of extracting.In order to study the reason for the different characteristics of ion extraction, a simplified simulation model of Cu+ andCr+ ions extraction process was established by 2D3V (two-dimensional in space and three- dimensional in velocity space)particle-in-cell (PIC) method. The effects of different extraction voltages from 0 V to 500 V on the density distribution ofCu+ and Cr+ ions and the change of plasma emission surface were analyzed. On the basis of this model, the ion densitydistribution characteristics of Cu+ ions mixed with Li+, Mg+, K+, Fe+, Y+, Ag+, Xe+, Au+, and Pb+ ions respectivelyunder 200-V extraction voltage are further simulated, and it is revealed that the atomic mass of the ions is the key reason fordifferent ion density distributions when different kinds of ions are mixed and extracted, which provides support for furtherunderstanding of ion extraction characteristics.展开更多
The geometric structure parameters and radial density distribution of 1s2s1S excited state of the two-electron atomic system near the critical nuclear charge Z_(c)were calculated in detail under tripled Hylleraas basi...The geometric structure parameters and radial density distribution of 1s2s1S excited state of the two-electron atomic system near the critical nuclear charge Z_(c)were calculated in detail under tripled Hylleraas basis set.Contrary to the localized behavior observed in the ground and the doubly excited 2p^(23)Pe states,for this state our results identify that while the behavior of the inner electron increasingly resembles that of a hydrogen-like atomic system,the outer electron in the excited state exhibits diffused hydrogen-like character and becomes perpendicular to the inner electron as nuclear charge Z approaches Z_(c).This study provides insights into the electronic structure and stability of the two-electron system in the vicinity of the critical nuclear charge.展开更多
The density distributions related to gas electronegativity for c-C4Fs gas, including negative ion, electron number and electron energy densities in the discharge process, are derived theoretically in both plane-to-pla...The density distributions related to gas electronegativity for c-C4Fs gas, including negative ion, electron number and electron energy densities in the discharge process, are derived theoretically in both plane-to-plane and point-to-plane electrode geometries. These calculations have been performed through the Boltzmann equation in the condition of a steady-state Townsend （SST） experiment and a fluid model in the condition of both uniform and non-uniform electric fields. The electronegativity coefficients a = n-/ne of c-C4Fs and SF6 are compared to further describe the electron affinity of c-C4Fs. The result shows that c-C4Fs represents an obvious electron-attachment performance in the discharge process. However, c-C4Fs still has much weaker gas electronegativity than SF6, whose electronegativity coefficient is lower than that of SF6 by at least three orders of magnitude.展开更多
In current investigations of electric arc plasmas, experiments based on modern testing technology play an important role. To enrich the testing methods and contribute to the understanding and grasping of the inherent ...In current investigations of electric arc plasmas, experiments based on modern testing technology play an important role. To enrich the testing methods and contribute to the understanding and grasping of the inherent mechanism of air switching arcs, in this paper, a nonintrusive detecting system is described that combines the magneto-optic imaging（MOI） technique with the solution to inverse electromagnetic problems. The detecting system works in a sequence of main steps as follows： MOI of the variation of the arc flux density over a plane, magnetic field information extracted from the magneto-optic（MO） images, arc current density distribution and spatial pattern reconstruction by inverting the resulting field data. Correspondingly, in the system, an MOI set-up is designed based on the Faraday effect and the polarization properties of light, and an intelligent inversion algorithm is proposed that involves simulated annealing（SA）.Experiments were carried out for high current（2 kA RMS） discharge cases in a typical low-voltage switchgear. The results show that the MO detection system possesses the advantages of visualization, high resolution and response, and electrical insulation, which provides a novel diagnostics tool for further studies of the arc.展开更多
In this study, the Chinese fir （Cunninghamia lanceolata Hook.） specimens with different ratios of heartwood thickness to sapwood thickness （HS） were radially compressed at different compression speeds, and then ab...In this study, the Chinese fir （Cunninghamia lanceolata Hook.） specimens with different ratios of heartwood thickness to sapwood thickness （HS） were radially compressed at different compression speeds, and then absorbed amine copper quat-type D （ACQ-D） preservative solution under the negative-pressure produced by the recovery of compression deformation. The liquid uptake （Al）, the recovery rate of compression deformation （Rs） and the chemical absorption （Ac） of samples were determined, as well as the overall distribution of density and effective component of ACQ-D （i.e., copper in wood）, the mechanical properties such as surface hardness were also measured. The Al, Rs, Ac values of compressed samples including the whole heartwood ones were higher than those of uncompressed samples, showing that radial compression had an obvious positive effect on improving the liquid absorption of heartwood. Higher compression speed of 3 mm.min^-1 is preferable since the samples with that speed could reach the highest Al and Ac; in addition, more deformation fixation has been produced possibly because of the faster heat and moisture transmission at the higher compressed speed, and more bonds of hydrophobic nature were formed, leading to the higher surface hardness and density. A consistent tendency of the density distribution and the copper retentions along the thickness direction could be explained that the layers with higher density have smaller volumes of void areas, and more chemicals were absorbed and fixed, resulting in the higher copper retentions.展开更多
A three-dimensional fluid model for surface-wave plasma （SWP）, to investigate the discharge characteristics of a rectangular SWP source working in a steady state, was presented. The simulation is performed for diffe...A three-dimensional fluid model for surface-wave plasma （SWP）, to investigate the discharge characteristics of a rectangular SWP source working in a steady state, was presented. The simulation is performed for different gas pressures in argon and different deposited powers. The results showed that there is a peak of plasma density at a distance of 2 cm to 3 cm from the plasma-quartz interface whose position depends mainly on the gas pressure but not the deposited power. The spatial distributions of plasma parameters and their dependence on the gas pressure and deposited power are also presented and discussed. Using this model a good agreement between the simulation results and the available experimental data is obtained.展开更多
The electronic properties of twinned ZnS nanowires （NWs） with different diameters were investigated based on first-principles calculations. The energy band structures, projected density of states and the spatial dis...The electronic properties of twinned ZnS nanowires （NWs） with different diameters were investigated based on first-principles calculations. The energy band structures, projected density of states and the spatial distributions of the bottom of conduction band and the top of the valence band were presented. The results show that the twinned nanowires exhibit a semiconducting character and the band gap decreases with increasing nanowire diameter due to quantum confinement effects. The valence band maximum and conduction band minimum originate mainly from the S-p and Zn-s orbitals at the core of the nanowires, respectively, which was confirmed by their spatial charge density distribution. We also found that no heterostructure is formed in the twinned ZnS NWs since the valence band maximum and conduction band minimum states are distributed along the NW axis uniformly. We suggest that the hexagonal （2H） stacking inside the cubic （3C） stacking has no effect on the electronic properties of thin ZnS NWs.展开更多
The effect of plasma with toroidal rotation on the resistive wall modes in tokamaks is studied numerically. An eigenvalue method is adopted to calculate the growth rate of the modes for changing plasma resistivity and...The effect of plasma with toroidal rotation on the resistive wall modes in tokamaks is studied numerically. An eigenvalue method is adopted to calculate the growth rate of the modes for changing plasma resistivity and plasma density distribution, as well as the diffusion time of magnetic field through the resistive wall. It is found that the resistive wall mode can be suppressed by the toroidal rotation of the plasma. Also, the growth rate of the resistive wall mode decreases when the edge plasma density is the same as the core plasma density, but it only changes slightly with the plasma resistivity.展开更多
We study the electronic band structure, density distribution, and transport of a Bi2Se3 nanoribbon, We find that the density distribution of the surface states is dependent on not only the shape and size of the transv...We study the electronic band structure, density distribution, and transport of a Bi2Se3 nanoribbon, We find that the density distribution of the surface states is dependent on not only the shape and size of the transverse cross section of the nanoribbon, but also the energy of the electron. We demonstrate that a transverse electric field can eliminate the coupling between surface states on the walls of the nanoribbon, remove the gap of the surface states, and restore the quantum spin Hall effects. In addition, we study the spin-dependent transport property of the surface states transmitting from top and bottom surfaces （x-y plane） to the side surfaces （z-x plane） of a Bi2Se3 nanoribbon. We find that transverse electric fields can open two surface channels for spin-up and -down Dirac electrons, and then switch off one channel for the spin-up Dirac electron. Our results may provide a simple way for the design of a spin filter based on topological insulator nanostructures.展开更多
基金supported by the Natural Science Foundation of Jilin Province (No. 20220101017JC)the National Natural Science Foundation of China (Nos. 11675063, 11875070, and 11935001)+1 种基金Key Laboratory of Nuclear Data foundation (JCKY2020201C157)the Anhui Project (Z010118169)
文摘Nuclear charge density distribution plays an important role in both nuclear and atomic physics,for which the two-parameter Fermi(2pF)model has been widely applied as one of the most frequently used models.Currently,the feedforward neural network has been employed to study the available 2pF model parameters for 86 nuclei,and the accuracy and precision of the parameter-learning effect are improved by introducing A^(1∕3)into the input parameter of the neural network.Furthermore,the average result of multiple predictions is more reliable than the best result of a single prediction and there is no significant difference between the average result of the density and parameter values for the average charge density distribution.In addition,the 2pF parameters of 284(near)stable nuclei are predicted in this study,which provides a reference for the experiment.
基金The project supported by the Natural Science Foundation of Guangdong province (No. 000675) the Key project tackled of Guangdong province (ZKM01401G)
文摘The ion density distribution in the reaction chamber was diagnosed by a Langmuir probe. The rules of the ion density distribution were obtained under the pressures of 9 Pa, 13 Pa, 27 Pa and 53 Pa in the reaction chamber, different radio-frequency powers and different positions. The result indicates that the ion density decreases as the pressure increases, and increases as the power decreases. The ion density of axial position z =0 achieves 5.8×1010 on the center of coil under the power of 200 w and pressure of 9 Pa in the reaction chamber.
基金supported by the National Natural Science Foundation of China (22075029, 22179070, U1932220)。
文摘The uniformity of current density distribution upon electrodes is one of the most important factors determining the lithium dendrites growth and cycling performance of lithium metal batteries(LMBs). Herein,current density distributions of lithium metal anodes induced by various engineering factors, consisting of uneven cathode, electrolyte distribution, and different tab positions, and their effects on the electrochemical performance are investigated theoretically and experimentally in pouch cells. The deviation of current density in lithium metal anodes ranges from 2.47% to 196.18% due to the different levels of uneven cathode materials. However, the deviation is just 13.60% for different electrolyte thicknesses between cathodes and anodes, even a ten-layer separator in some positions. The maximum deviation for variational tab positions is only 0.17%. The nonuniformity in current density distribution results in severe dendrite growth issues and poor electrochemical performance of LMBs. This work not only confirms the direct correlation between the uneven current density distribution and lithium deposition behaviors, but also points out the decisive effects of cathode surface roughness on current distribution of anodes, to which more attentions should be paid in practical applications of LMBs.
基金supported by the National Natural Science Foundation of China(No.12002046)the China Postdoctoral Science Foundation(No.2020M680392)。
文摘In this paper,the penetration mechanism of reactive jet with non-uniform density distribution is studied.The simulations show that the density deficit occurs in the whole reactive jet,and the density increases from the jet tip to tail.The density of jet tip is approximately 1.5 g/cm3,which is lower than that of the reactive liner materials.The X-ray experiments show similar results with the simulations.The density decreasing effect of jet tip has a significant influence on the penetration behavior when the reactive jet impacts steel plate.According to the simulation results,this paper assumes that the density gradient in the jet section has linear distribution.Then,the deflagration pressure generated by each jet element at the bottom of crater is introduced into the Bernoulli equation.Based on the virtual origin model and Szendrei-Held equation,the analytical models for penetration depth and radial cratering of reactive jet with the density reduction are obtained.Moreover,to further prove the validity of analytical models,the penetration experiments of the reactive liner shaped charge against steel plate under different standoffs are carried out.There is a convergence between the analytical crater profiles and experimental results when reactive jets penetrate steel plates under different standoffs,especially at standoff of 1.5 and 2.0charge diameters.
基金Project supported by the National Natural Science Foundation of China （Grant No 10035020）.
文摘A two-dimensional, three-temperature radiation magneto-hydrodynamics model is applied to the investigation of evolutional trends in x-ray radiation power, energy, peak plasma temperature and density as functions of drive current rise-time and initial load density distribution by using the typical experimental parameters of tungsten wire-array Z- pinch on the Qiangguang-I generator. The numerical results show that as the drive current rise-time is shortened, x-ray radiation peak power, energy, peak plasma density and peak ion temperature increase approximately linearly, but among them the x-ray radiation peak power increases more quickly. As the initial plasma density distribution in the radial direction becomes gradually flattened, the peak radiation power and the peak ion-temperature almost exponentially increase, while the radiation energy and the peak plasma density change only a little. The main effect of shortening drive current rise-time is to enhance compression of plasma, and the effect of flattening initial load density distribution in the radial direction is to raise the plasma temperature. Both of the approaches elevate the x-ray peak radiation power
基金Beijing Natural Science Foundation,China(Grant No.Z190010)the National Key Research and Development Program of China(Grant No.2019YFA0308500)+2 种基金the Strategic Priority Research Program of Chinese Academy of Sciences(Grant No.XDB07030200)Key Research Projects of Frontier Science of Chinese Academy of Sciences(Grant No.QYZDB-SSW-JSC035)the National Natural Science Foundation of China(Grant Nos.51421002,51672307,51991344,52025025,and 52072400).
文摘Electron density plays an important role in determining the properties of functional materials.Revealing the electron density distribution experimentally in real space can help to tune the properties of materials.Spinel Li Mn2 O4 is one of the most promising cathode candidates because of its high voltage,low cost,and non-toxicity,but suffers severe capacity fading during electrochemical cycling due to the Mn dissolution.Real-space measurement of electron distribution of Li Mn2 O4 experimentally can provide direct evaluation on the strength of Mn–O bond and give an explanation of the structure stability.Here,through high energy synchrotron powder x-ray diffraction(SPXRD),accurate electron density distribution in spinel Li Mn2 O4 has been investigated based on the multipole model.The electron accumulation between Mn and O atoms in deformation density map indicates the shared interaction of Mn–O bond.The quantitative topological analysis at bond critical points shows that the Mn–O bond is relatively weak covalent interaction due to the oxygen loss.These findings suggest that oxygen stoichiometry is the key factor for preventing the Mn dissolution and capacity fading.
基金supported by National Natural Science Foundation of China(Nos.11264036,11465016 and 11364038)
文摘We perform an experimental study of two-dimensional（2D） electron density profiles of the laser-induced plasma plumes in air by ordinarily laboratorial interferometry. The electron density distributions measured show a feature of hollow core. To illustrate the feature, we present a theoretical investigation by using dynamics analysis. In the simulation, the propagation of laser pulse with the evolution of electron density is utilized to evaluate ionization of air target for the plasma-formation stage. In the plasma-expansion stage, a simple adiabatic fluid dynamics is used to calculate the evolution of plasma outward expansion. The simulations show good agreements with experimental results, and demonstrate an effective way of determining 2D density profiles of the laser-induced plasma plume in gas.
文摘Propellant ionization in the Hall thruster discharge channel is a significant process and has strong influence on the thruster＇s efficiency. In this work, the functional relation has been established between the ionization density distribution and the function of the ion energy distribution through the basic equations governing the ion flow in the Hall thruster channel and the method achieved for reconstructing the ionization density distribution inside the channel by ordinary plasma diagnosis of the potential distribution and ion energy spectrum of the plasma jet. The ionization density distributions of single and double charged ions in an ATON-thruster channel have been reconstructed according to the experimental data of the potential distribution along the axis of the channel and the ion energy spectrum of the plasma jet. The agreement between the calculation and experimental results of the percentage of double charged ions proves the validity of our method achieved in this work.
基金Supported by the National Natural Science Foundation of China under Grant Nos 51337002,51077028,51502063 and 51307046the Foundation of Harbin Science and Technology Bureau of Heilongjiang Province under Grant No RC2014QN017034
文摘The distributions of traps and electron density in the interfaces between polyimide （PI） matrix and Al2O3 nanoparticles are researched using the isothermal decay current and the small-angle x-ray scattering （SAXS） tests. According to the electron density distribution for quasi two-phase mixture doped by spherical nanoparticles, the electron densities in the interfaces of PI/Al2O3 nanocomposite films are evaluated. The trap level density and carrier mobility in the interface are studied. The experimental results show that the distribution and the change rate of the electron density in the three layers of interface are different, indicating different trap distributions in the interface layers. There is a maximum trap level density in the second layer, where the maximum trap level density for the nanocomposite film doped by 25 wt% is 1.054 × 10^22 eV·m^-3 at 1.324eV, resulting in the carrier mobility reducing. In addition, both the thickness and the electron density of the nanocomposite film interface increase with the addition of the doped Al2O3 contents. Through the study on the trap level distribution in the interface, it is possible to further analyze the insulation mechanism and to improve the performance of nano-dielectric materials.
基金Project supported by the National Natural Science Foundation of China (Grant No 20673150)
文摘In this work, a bridge density functional approximation （BDFA） （J. Chem. Phys. 112, 8079 （2000）） for a nonuniform hard-sphere fluid is extended to a non-uniform hard-core repulsive Yukawa （HCRY） fluid. It is found that the choice of a bulk bridge functional approximation is crucial for both a uniform HCRY fluid and a non-uniform HCRY fluid. A new bridge functional approximation is proposed, which can accurately predict the radial distribution function of the bulk HCRY fluid. With the new bridge functional approximation and its associated bulk second order direct correlation function as input, the BDFA can be used to well calculate the density profile of the HCRY fluid subjected to the influence of varying external fields, and the theoretical predictions are in good agreement with the corresponding simulation data. The calculated results indicate that the present BDFA captures quantitatively the phenomena such as the coexistence of solid-like high density phase and low density gas phase, and the adsorption properties of the HCRY fluid, which qualitatively differ from those of the fluids combining both hard-core repulsion and an attractive tail.
基金supported by National Natural Science Foundation of China (Nos. 11035001, 11175003, 10875002, 10775005)
文摘The experimental data of the isotopic distribution for projectile-like fragments are presented for the 17,18N ＋ 197Au reaction at 33 MeV/u. The width of the isotopic distributions for lSN projectile is significantly broader than that for 17N projectile, and the average N/Z ratio of the former shifts to higher neutron number side. As long as the realistic nucleon density distribution is used, the isotopic distribution for fragments is reproduced by the simple abrasion-ablation model calculation, which thus provides an independent way to determine the surface distribution of the nuclear matter density for neutron-rich nuclei.
基金the Presidential Foundation of China Academy of Engineering Physics(Grant No.YZJJZQ2022016)the National Natural Science Foun-dation of China(Grant No.52207177).
文摘The spatial distributions of different kinds of ions are usually not completely the same in the process of extracting.In order to study the reason for the different characteristics of ion extraction, a simplified simulation model of Cu+ andCr+ ions extraction process was established by 2D3V (two-dimensional in space and three- dimensional in velocity space)particle-in-cell (PIC) method. The effects of different extraction voltages from 0 V to 500 V on the density distribution ofCu+ and Cr+ ions and the change of plasma emission surface were analyzed. On the basis of this model, the ion densitydistribution characteristics of Cu+ ions mixed with Li+, Mg+, K+, Fe+, Y+, Ag+, Xe+, Au+, and Pb+ ions respectivelyunder 200-V extraction voltage are further simulated, and it is revealed that the atomic mass of the ions is the key reason fordifferent ion density distributions when different kinds of ions are mixed and extracted, which provides support for furtherunderstanding of ion extraction characteristics.
基金supported by the National Natural Science Foundation of China(Grant Nos.12074295,12304271,and 12104420).
文摘The geometric structure parameters and radial density distribution of 1s2s1S excited state of the two-electron atomic system near the critical nuclear charge Z_(c)were calculated in detail under tripled Hylleraas basis set.Contrary to the localized behavior observed in the ground and the doubly excited 2p^(23)Pe states,for this state our results identify that while the behavior of the inner electron increasingly resembles that of a hydrogen-like atomic system,the outer electron in the excited state exhibits diffused hydrogen-like character and becomes perpendicular to the inner electron as nuclear charge Z approaches Z_(c).This study provides insights into the electronic structure and stability of the two-electron system in the vicinity of the critical nuclear charge.
基金supported by National Natural Science Foundation of China (No.51337006)
文摘The density distributions related to gas electronegativity for c-C4Fs gas, including negative ion, electron number and electron energy densities in the discharge process, are derived theoretically in both plane-to-plane and point-to-plane electrode geometries. These calculations have been performed through the Boltzmann equation in the condition of a steady-state Townsend （SST） experiment and a fluid model in the condition of both uniform and non-uniform electric fields. The electronegativity coefficients a = n-/ne of c-C4Fs and SF6 are compared to further describe the electron affinity of c-C4Fs. The result shows that c-C4Fs represents an obvious electron-attachment performance in the discharge process. However, c-C4Fs still has much weaker gas electronegativity than SF6, whose electronegativity coefficient is lower than that of SF6 by at least three orders of magnitude.
基金supported by the Fundamental Research Funds for the Central Universities of China(XJJ2011019)
文摘In current investigations of electric arc plasmas, experiments based on modern testing technology play an important role. To enrich the testing methods and contribute to the understanding and grasping of the inherent mechanism of air switching arcs, in this paper, a nonintrusive detecting system is described that combines the magneto-optic imaging（MOI） technique with the solution to inverse electromagnetic problems. The detecting system works in a sequence of main steps as follows： MOI of the variation of the arc flux density over a plane, magnetic field information extracted from the magneto-optic（MO） images, arc current density distribution and spatial pattern reconstruction by inverting the resulting field data. Correspondingly, in the system, an MOI set-up is designed based on the Faraday effect and the polarization properties of light, and an intelligent inversion algorithm is proposed that involves simulated annealing（SA）.Experiments were carried out for high current（2 kA RMS） discharge cases in a typical low-voltage switchgear. The results show that the MO detection system possesses the advantages of visualization, high resolution and response, and electrical insulation, which provides a novel diagnostics tool for further studies of the arc.
文摘In this study, the Chinese fir （Cunninghamia lanceolata Hook.） specimens with different ratios of heartwood thickness to sapwood thickness （HS） were radially compressed at different compression speeds, and then absorbed amine copper quat-type D （ACQ-D） preservative solution under the negative-pressure produced by the recovery of compression deformation. The liquid uptake （Al）, the recovery rate of compression deformation （Rs） and the chemical absorption （Ac） of samples were determined, as well as the overall distribution of density and effective component of ACQ-D （i.e., copper in wood）, the mechanical properties such as surface hardness were also measured. The Al, Rs, Ac values of compressed samples including the whole heartwood ones were higher than those of uncompressed samples, showing that radial compression had an obvious positive effect on improving the liquid absorption of heartwood. Higher compression speed of 3 mm.min^-1 is preferable since the samples with that speed could reach the highest Al and Ac; in addition, more deformation fixation has been produced possibly because of the faster heat and moisture transmission at the higher compressed speed, and more bonds of hydrophobic nature were formed, leading to the higher surface hardness and density. A consistent tendency of the density distribution and the copper retentions along the thickness direction could be explained that the layers with higher density have smaller volumes of void areas, and more chemicals were absorbed and fixed, resulting in the higher copper retentions.
文摘A three-dimensional fluid model for surface-wave plasma （SWP）, to investigate the discharge characteristics of a rectangular SWP source working in a steady state, was presented. The simulation is performed for different gas pressures in argon and different deposited powers. The results showed that there is a peak of plasma density at a distance of 2 cm to 3 cm from the plasma-quartz interface whose position depends mainly on the gas pressure but not the deposited power. The spatial distributions of plasma parameters and their dependence on the gas pressure and deposited power are also presented and discussed. Using this model a good agreement between the simulation results and the available experimental data is obtained.
基金Project supported by the Special Funds of the National Natural Science Foundation of China (Grant No. 10947102)the Foundation of the Education Committee of Chongqing (Grant No. KJ090503)
文摘The electronic properties of twinned ZnS nanowires （NWs） with different diameters were investigated based on first-principles calculations. The energy band structures, projected density of states and the spatial distributions of the bottom of conduction band and the top of the valence band were presented. The results show that the twinned nanowires exhibit a semiconducting character and the band gap decreases with increasing nanowire diameter due to quantum confinement effects. The valence band maximum and conduction band minimum originate mainly from the S-p and Zn-s orbitals at the core of the nanowires, respectively, which was confirmed by their spatial charge density distribution. We also found that no heterostructure is formed in the twinned ZnS NWs since the valence band maximum and conduction band minimum states are distributed along the NW axis uniformly. We suggest that the hexagonal （2H） stacking inside the cubic （3C） stacking has no effect on the electronic properties of thin ZnS NWs.
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 11275041, 11105065, 11095015, and 10675029)the National Basic Research Program of China (Grant Nos. 2008CB717801, 2008CB787103, 2009GB105004, and 2010GB106002)
文摘The effect of plasma with toroidal rotation on the resistive wall modes in tokamaks is studied numerically. An eigenvalue method is adopted to calculate the growth rate of the modes for changing plasma resistivity and plasma density distribution, as well as the diffusion time of magnetic field through the resistive wall. It is found that the resistive wall mode can be suppressed by the toroidal rotation of the plasma. Also, the growth rate of the resistive wall mode decreases when the edge plasma density is the same as the core plasma density, but it only changes slightly with the plasma resistivity.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11547051 and 11274018)
文摘We study the electronic band structure, density distribution, and transport of a Bi2Se3 nanoribbon, We find that the density distribution of the surface states is dependent on not only the shape and size of the transverse cross section of the nanoribbon, but also the energy of the electron. We demonstrate that a transverse electric field can eliminate the coupling between surface states on the walls of the nanoribbon, remove the gap of the surface states, and restore the quantum spin Hall effects. In addition, we study the spin-dependent transport property of the surface states transmitting from top and bottom surfaces （x-y plane） to the side surfaces （z-x plane） of a Bi2Se3 nanoribbon. We find that transverse electric fields can open two surface channels for spin-up and -down Dirac electrons, and then switch off one channel for the spin-up Dirac electron. Our results may provide a simple way for the design of a spin filter based on topological insulator nanostructures.
