The controlled assembly of nanomaterials has demon-strated significant potential in advancing technological devices.However,achieving highly efficient and low-loss assembly technique for nanomate-rials,enabling the cr...The controlled assembly of nanomaterials has demon-strated significant potential in advancing technological devices.However,achieving highly efficient and low-loss assembly technique for nanomate-rials,enabling the creation of hierarchical structures with distinctive func-tionalities,remains a formidable challenge.Here,we present a method for nanomaterial assembly enhanced by ionic liquids,which enables the fabrication of highly stable,flexible,and transparent electrodes featuring an organized layered structure.The utilization of hydrophobic and non-volatile ionic liquids facilitates the production of stable interfaces with water,effectively preventing the sedimentation of 1D/2D nanomaterials assembled at the interface.Furthermore,the interfacially assembled nanomaterial monolayer exhibits an alternate self-climbing behavior,enabling layer-by-layer transfer and the formation of a well-ordered MXene-wrapped silver nanowire network film.The resulting composite film not only demonstrates exceptional photoelectric performance with a sheet resistance of 9.4Ωsq^(-1) and 93%transmittance,but also showcases remarkable environmental stability and mechanical flexibility.Particularly noteworthy is its application in transparent electromagnetic interference shielding materials and triboelectric nanogenerator devices.This research introduces an innovative approach to manufacture and tailor functional devices based on ordered nanomaterials.展开更多
The quality and aroma of strong-flavor Baijiu are mainly dependent on Daqu,pit mud(PM),and the interaction of both.However,little is known about how their combination patterns affect the microbiome and metabolome of Z...The quality and aroma of strong-flavor Baijiu are mainly dependent on Daqu,pit mud(PM),and the interaction of both.However,little is known about how their combination patterns affect the microbiome and metabolome of Zaopei,especially the metabolic function of rare taxa.Here,an experiment on industrial size was designed to assess the effects of 6 combinations(3 kinds of Daqu×2 kinds of PM)on the composition and assembly of different taxa,as well as the flavor profile.The results showed that Zaopei's microbiota was composed of a few abundant taxa and enormous rare taxa,and rare bacterial and abundant fungal subcommunities were significantly affected by combination patterns.The assembly processes of abundant/rare taxa and bacterial/fungal communities were distinct,and environmental changes mediated the balance between stochastic and deterministic processes in rare bacteria assembly.Furthermore,specific combination patterns improved the flavor quality of Zaopei by enhancing the interspecies interaction,which was closely related to rare taxa,especially rare bacteria.These findings highlighted that rare bacteria might be the keystone in involving community interaction and maintaining metabolic function,which provided a scientific foundation for better understanding and regulating the brewing microbiota from the viewpoint of microbial ecology.展开更多
The computer numerical control（CNC） system is suited to control varied types of flexible fixtures in aircraft component manufacturing and assembly. The mechanisms and control requirements of flexible fixtures are pr...The computer numerical control（CNC） system is suited to control varied types of flexible fixtures in aircraft component manufacturing and assembly. The mechanisms and control requirements of flexible fixtures are presented and analyzed. The hardware and software architecture and implementation of CNC system are pro- posed. The flexible fixture mechanism is described using configuration parameters. According to the parameters, the CNC system automatically generates the control feature and the human machine interface （HMI） operation function. The CNC system is implemented in a flexible fixture for skin-strlnger assembly, and results show the effectiveness of the system.展开更多
Taking a microwave product as an example, a system of integrated assembly structure design is presented. Getting design constraints from the upstream design section through product data management(PDM), the system gen...Taking a microwave product as an example, a system of integrated assembly structure design is presented. Getting design constraints from the upstream design section through product data management(PDM), the system generates the assembly scheme using the case? based method, then assigns the design requirements into each component of the assembly. The detail design for each component can be performed under these design constraints. In order to practise concurrent design, the system sends the final design result to the upstream section and downstream section through PDM to achieve information sharing and integration.展开更多
The parametric part assembly generation method is presented. Based on the parametric part generated by means of constructive-element, through interactively inputting the relationships of the location and the assembly,...The parametric part assembly generation method is presented. Based on the parametric part generated by means of constructive-element, through interactively inputting the relationships of the location and the assembly, and by compiling operations like movement and rotation, the assembly drawing is created so as to implement the occurrence of the parameterizations of the assembly and the part drawing. The data structure of the assembly part and the key technologies of hidden line removal in the implementation of assembly process, etc. , are described in detail.展开更多
Nanocarbon-based materials, such as carbon nanotubes(CNTs) and graphene have been attached much attention by scientific and industrial community. As two representative nanocarbon materials, one-dimensional CNTs and tw...Nanocarbon-based materials, such as carbon nanotubes(CNTs) and graphene have been attached much attention by scientific and industrial community. As two representative nanocarbon materials, one-dimensional CNTs and twodimensional graphene both possess remarkable mechanical properties. In the past years, a large amount of work have been done by using CNTs or graphene as building blocks for constructing novel, macroscopic, mechanically strong fibrous materials. In this review, we summarize the assembly approaches of CNT-based fibers and graphene-based fibers in chronological order, respectively. The mechanical performances of these fibrous materials are compared, and the critical influences on the mechanical properties are discussed. Personal perspectives on the fabrication methods of CNT-and graphene-based fibers are further presented.展开更多
EAST （HT-7U） is a large fusion experimental device. It is a full superconducting tokamak with 1 MA of plasma current, 1000 s of plasma duration, high elongation and triangularity. It mainly consists of superconducti...EAST （HT-7U） is a large fusion experimental device. It is a full superconducting tokamak with 1 MA of plasma current, 1000 s of plasma duration, high elongation and triangularity. It mainly consists of superconducting magnets of poloidal and toroidal field （PF ＆ TF）, vacuum vessel （VV）, thermal radiation shield （TRS） and cryostat vessel （CV）. The significant difficulty for assembly of EAST is tight installation tolerances, which are in the order of several tenth of a millimeter. In particular, the alignment of plasma facing components to the magnetic axis of the device is less than ±0.5 mm. At present, a reasonable assembly process of EAST has been defined, and based on it, the alignment method for EAST, including the survey control network, the location of the main components in different directions, the magnetic axis determination and the accurate positioning of the plasma facing components inside of the vacuum vessel and so on, has been defined by using the sophisticated optical metrology system （SOMS）. This paper describes the assembly procedure of EAST and the installation tolerances associated with the main components. Meanwhile, how to establish the assembly survey control network, magnetic axis determination methods, are introduced in detail.展开更多
Nanowires and nanotubes of diverse material compositions,properties and/or functions have been produced or fabricated through various bottom-up or top-down approaches.These nanowires or nanotubes have also been utiliz...Nanowires and nanotubes of diverse material compositions,properties and/or functions have been produced or fabricated through various bottom-up or top-down approaches.These nanowires or nanotubes have also been utilized as potential building blocks for functional nanodevices.The key for the integration of those nanowire or nanotube based devices is to assemble these one dimensional nanomaterials to specific locations using techniques that are highly controllable and scalable.Ideally such techniques should enable assembly of highly uniform nanowire/nanotube arrays with precise control of density,location,dimension or even material types of nanowires/nanotubes.Numerous assembly techniques are being developed that can quickly align and assemble large quantities of one type or multiple types of nanowires through parallel processes,including flow-assisted alignment,Langmuir-Blodgett assembly,bubble-blown technique,electric/magnetic-field directed assembly,contact/roll printing,knocking-down,etc..With these assembling techniques,applications of nanowire/nanotube based devices such as flexible electronics and sensors have been demonstrated.This paper delivers an overall review of directed nanowire/nanotube assembling approaches and analyzes advantages and limitations of each method.The future research directions have also been discussed.展开更多
Two-dimensional(2D) transition metal carbides, carbonitrides and nitrides, known as MXenes, are emerging quickly at the frontiers of 2D materials world. Their exotic properties such as the highest electrical conductiv...Two-dimensional(2D) transition metal carbides, carbonitrides and nitrides, known as MXenes, are emerging quickly at the frontiers of 2D materials world. Their exotic properties such as the highest electrical conductivity among all solution-processed 2 D materials, the best electromagnetic interference shielding performance outperforming that of copper or aluminum at a nanoscale thickness, as well as the highest volumetric capacitance for pseudocapacitors, have been attracting extensive fundamental research and applications. Their unique surface chemistries, that is, hydrophilic groups terminated on the surface of MXenes after etching and delamination, enable plenty of opportunities for assembling into MXene building blocks. Particularly, assembling at liquid–liquid, liquid–solid, liquid–air, and solid–solid interfaces allows the efficient fabrication of various structures, including MXene surfactants, MXene heterostructures, MXene transparent films. Interfacial assembly of MXenes is of significance in unveiling more versatilities of MXenes as well as impacts on novel MXene-based architectures, based on which enhanced performance of devices is achieved. As such, this review focuses on the interfacial assembly of MXenes, explaining mechanisms behind various assembling and providing classical examples for corresponding interfacial assembling techniques. Applications of these as-assembled architectures are also discussed in brief. We believe this review may shed light on the interfacial chemistry of MXenes, thus guiding more efficient fabrication of MXene-based functional films/coatings/electrodes/devices.展开更多
To fulfill the demands for higher quality,efficiency and flexibility in aviation industry,a multi-functional end effector is designed to automate the drilling and riveting processes in assembling carbon fiber reinforc...To fulfill the demands for higher quality,efficiency and flexibility in aviation industry,a multi-functional end effector is designed to automate the drilling and riveting processes in assembling carbon fiber reinforced polymer(CFRP)and aluminum components for a robotic aircraft assembly system.To meet the specific functional requirements for blind rivet installation on CFRP and aluminum materials,additional modules are incorporated on the end effector aside of the basic processing modules for drilling.And all of these processing modules allow for a onestep-drilling-countersinking process,hole inspection,automatic rivet feed,rivet geometry check,sealant application,rivet insertion and installation.Besides,to guarantee the better quality of the hole drilled and joints riveted,several online detection and adjustment measures are applied to this end effector,including the reference detection and perpendicular calibration,which could effectively ensure the positioning precision and perpendicular accuracy as demanded.Finally,the test result shows that this end effector is capable of producing each hole to a positioning precision within ±0.5 mm,aperpendicular accuracy within 0.3°,a diameter tolerance of H8,and a countersink depth tolerance of±0.01 mm.Moreover,it could drill and rivet up to three joints per minute,with acceptable shearing and tensile strength.展开更多
The key realization techniques of virtual assembly process planning （VAPP） system are analyzed, including virtual assembly model, real-time collision detection, automatic constraint recognition algorithm, cable harn...The key realization techniques of virtual assembly process planning （VAPP） system are analyzed, including virtual assembly model, real-time collision detection, automatic constraint recognition algorithm, cable harness assembly process planning and visual assembly process plan at the workshop. A virtual assembly model based on hierarchical assembly task list （HATL） is put forward, in which assembly tasks are defined to express component assembling operations and are sequentially and hierarchically organized according to different subassemblies, which can perfectly model the construction process of product, And a multi-layer automatic geometry constraint recognition algorithm of how to identify assmbly constraint relations in the virtual environment is proposed, then a four-layer collision detection algorithm is discussed. A VAPP system is built and some simple mechanical assemblies are used to illustrate the feasibility of the proposed method and algorithms.展开更多
To obtain the performance characteristics of hydrodynamic tractor-retarder assembly under traction work condition,a numerical simulation model of flow channel was established and tetrahedron unstructured grids were ad...To obtain the performance characteristics of hydrodynamic tractor-retarder assembly under traction work condition,a numerical simulation model of flow channel was established and tetrahedron unstructured grids were adopted in the meshing stage.The racing rotating speed of the brake wheels was calculated by computational fluid dynamics（CFD） calculation and interpolation,and then accurate boundary condition was applied to the CFD simulation to study the pressure and velocity distribution of internal flow field in hydrodynamic tractor-retarder assembly.Finally,the original characteristics were calculated by CFD post-processing analysis.Comparison of experimental data and flow field analysis results showed that the calculation tolerance of the torque ratio K and the efficiency η was less than 5%,and the calculation tolerance of the pump torque coefficient λ was less than 10%.展开更多
Synthesis and applications of three-dimensional(3 D)porous graphene frameworks(GFs)have attracted extensive interest owing to their intriguing advantages of high specific surface area,enriched porosity,excellent elect...Synthesis and applications of three-dimensional(3 D)porous graphene frameworks(GFs)have attracted extensive interest owing to their intriguing advantages of high specific surface area,enriched porosity,excellent electrical conductivity,exceptional compressibility and processability.However,it is still challenging for economically viable,fast and scalable assembly of 3 D GFs at room-temperature.Herein,we reported a one-step scalable strategy for fast self-assembly of graphene oxide into 3 D macroscopically porous GFs,with assistance of polyoxometalates(POM)as functional cross-linker and hydrazine hydrate as reductant at room-temperature.The resulting 3 D interconnected macroporous POM-GFs uniformly decorated with ultrasmall POM nanoclusters were directly processed into binder-/additive-free film compact electrodes(1.68 g cm^(-3))with highly aligned,layer-stacked structure and electrically conductivity(622 S m-1)for high-performance supercapacitors,showing an impressive gravimetric capacitance of205 F g-1,volumetric capacitance of 334 F cm^(-3) at 1 mV s^(-1),and remarkable cycling stability with capacitance retention of 83%after 10,000 cycles,outperforming the most reported GFs.Further,the solid-state supercapacitors offered excellent gravimetric capacitance of 157 F g-1 exceptionally volumetric capacitance of 115 F cm^(-3) at 2 mV s^(-1) based on single electrode,and volumetric energy density of2.6 mWh cm^(-3).Therefore,this work will open novel opportunities to room-temperature fast assembly of 3 D porous graphene architectures for high-energy-density supercapacitors.展开更多
Jet pulse assembly is one of the main components of jet hydraulic oscillator.The pressure wave characteristics produced by jet pulse assembly have an important influence on the performance of the tool.In this paper,th...Jet pulse assembly is one of the main components of jet hydraulic oscillator.The pressure wave characteristics produced by jet pulse assembly have an important influence on the performance of the tool.In this paper,the structure and working principle of jet pulse assembly are studied,the mechanical analysis model of piston rod is established,the dynamic resistance ratio formula of jet pulse assembly is deduced,and the numerical simulation test of 89-mm jet pulse assembly structure parameters is carried out.The results show that the piston rod downward stroke is driven by both the jet element driving force and the throttle plate load driving force,and can stably descend.The driving force of the piston rod upward stroke jet element is opposite to the load acting force of the throttle disc,and the jet driving force needs to be greater than the load resistance of the throttle disc to stably ascend.The dynamic resistance ratio formula is deduced.When the area of the end of the piston rod is reduced,the resistance of the throttle disc is reduced and the jet power is increased,thus solving the problem of insufficient power of the piston rod in the upstroke and ensuring the normal operation of the tool.Ten groups of numerical simulation tests were carried out,and it was found that the pressure amplitude and pressure drop of the tool decreased significantly with the increase of the tool size,and the error between the numerical simulation value and the theoretical calculation value was less than 9%,which verified the correctness of the theory.It is suggested to select tools on site according to the drilling construction situation to ensure the drilling effect.展开更多
Due to the complexity of strong metal interference and multiple occlusions in aircraft assembly workshop,the random "drift"phenomenon often happens in the ultra wide band (UWB)based positioning system.To sol...Due to the complexity of strong metal interference and multiple occlusions in aircraft assembly workshop,the random "drift"phenomenon often happens in the ultra wide band (UWB)based positioning system.To solve this,a fusion positioning optimization algorithm is proposed based on median filtering,hidden Markov model (HMM)a nd Kalman filtering.Firstly,based on the three-dimensional (3D) median filtering,aqueue optimization method with weights is introduced to smooth the measurement data and eliminate the abnormal value.Secondly,taking Singer model as a reference,a single-dimension acceleration distribution model is designed.In order to further consider the spatial motion characteristics of objects in workshop,the distribution is extended from 1D to 3D,and discretized into the state quantity of HMM.Subsequently,the data obtained by the two methods are fused by taking Kalman filter as an iterator,and then the optimized location solution is obtained based on dynamic weights.Finally,an experiment is conducted in an aircraft assembly workshop.Results show that 99.3% of dynamic positioning errors are less than 15 cm after using the proposed algorithm.Even in the situation with large signal-fluctuation,there are 71.6% of positioning data whose errors are reduced.The random "drift"is greatly decreased.展开更多
Complex multiscale assemblies of metal-organic frameworks are essential in the construction of largescale optical platforms but often restricted by their bulk nature and conventional techniques.The integration of nano...Complex multiscale assemblies of metal-organic frameworks are essential in the construction of largescale optical platforms but often restricted by their bulk nature and conventional techniques.The integration of nanomaterials and 3D printing technologies allows the fabrication of multiscale functional architectures.Our study reports a unique method of controlled 3D assembly purely relying on the post-printing treatment of printed constructs.By immersing a 3D-printed patterned construct consisting of organic ligand in a solution of lanthanide ions,in situ growth of lanthanide metal-organic frameworks(LnMOFs)can rapidly occur,resulting in macroscopic assemblies and tunable fluorescence properties.This phenomenon,caused by coordination and chelation of lanthanide ions,also renders a sub-millimeter resolution and high shape fidelity.As a proof of concept,a type of 3D assembled LnMOFsbased optical sensing platform has demonstrated the feasibility in response to small molecules such as acetone.It is anticipated that the facile printing and design approach developed in this work can be applied to fabricate bespoke multiscale architectures of functional materials with controlled assembly,bringing a realistic and economic prospect.展开更多
Stimuli-triggered drug delivery systems hold vast promise in local infection treatment for the site-specific targeting and shuttling of drugs.Herein,chitosan conjugates(SPCS)installed with sialic acid(SA)and phenylbor...Stimuli-triggered drug delivery systems hold vast promise in local infection treatment for the site-specific targeting and shuttling of drugs.Herein,chitosan conjugates(SPCS)installed with sialic acid(SA)and phenylboronic acid(PBA)were synthesized,of which SA served as targeting ligand for coccidium and reversible-binding bridge for PBA.The enhanced drug-loading capacity of SPCS micelles was attributed to a combination assembly from hydrophobicity-driving and reversible borate bridges.The drug-loaded SPCS micelles shared superior biostability in upper gastrointestinal tract.After reaching the lesions,the borate bridges were snipped by carbohydrates under a higher pH followed by accelerated drug release,while SA exposure on micellar surface facilitated drug cellular internalization to eliminate parasites inside.The drugmicelles revealed an enhanced anti-coccidial capacity with a higher index of 185.72 compared with commercial preparation.The dual-responsive combination of physicochemical assembly could provide an efficient strategy for the exploitation of stable,safe and flexible anti-infectious drug delivery systems.展开更多
基金This work was supported by the National Natural Science Foundation of China(nos.21988102,and 22305026)the China Postdoctoral Science Foundation(2019M650433).
文摘The controlled assembly of nanomaterials has demon-strated significant potential in advancing technological devices.However,achieving highly efficient and low-loss assembly technique for nanomate-rials,enabling the creation of hierarchical structures with distinctive func-tionalities,remains a formidable challenge.Here,we present a method for nanomaterial assembly enhanced by ionic liquids,which enables the fabrication of highly stable,flexible,and transparent electrodes featuring an organized layered structure.The utilization of hydrophobic and non-volatile ionic liquids facilitates the production of stable interfaces with water,effectively preventing the sedimentation of 1D/2D nanomaterials assembled at the interface.Furthermore,the interfacially assembled nanomaterial monolayer exhibits an alternate self-climbing behavior,enabling layer-by-layer transfer and the formation of a well-ordered MXene-wrapped silver nanowire network film.The resulting composite film not only demonstrates exceptional photoelectric performance with a sheet resistance of 9.4Ωsq^(-1) and 93%transmittance,but also showcases remarkable environmental stability and mechanical flexibility.Particularly noteworthy is its application in transparent electromagnetic interference shielding materials and triboelectric nanogenerator devices.This research introduces an innovative approach to manufacture and tailor functional devices based on ordered nanomaterials.
基金supported by the Cooperation Project of Luzhou Laojiao Co.,Ltd.Sichuan University (21H0997)。
文摘The quality and aroma of strong-flavor Baijiu are mainly dependent on Daqu,pit mud(PM),and the interaction of both.However,little is known about how their combination patterns affect the microbiome and metabolome of Zaopei,especially the metabolic function of rare taxa.Here,an experiment on industrial size was designed to assess the effects of 6 combinations(3 kinds of Daqu×2 kinds of PM)on the composition and assembly of different taxa,as well as the flavor profile.The results showed that Zaopei's microbiota was composed of a few abundant taxa and enormous rare taxa,and rare bacterial and abundant fungal subcommunities were significantly affected by combination patterns.The assembly processes of abundant/rare taxa and bacterial/fungal communities were distinct,and environmental changes mediated the balance between stochastic and deterministic processes in rare bacteria assembly.Furthermore,specific combination patterns improved the flavor quality of Zaopei by enhancing the interspecies interaction,which was closely related to rare taxa,especially rare bacteria.These findings highlighted that rare bacteria might be the keystone in involving community interaction and maintaining metabolic function,which provided a scientific foundation for better understanding and regulating the brewing microbiota from the viewpoint of microbial ecology.
文摘The computer numerical control（CNC） system is suited to control varied types of flexible fixtures in aircraft component manufacturing and assembly. The mechanisms and control requirements of flexible fixtures are presented and analyzed. The hardware and software architecture and implementation of CNC system are pro- posed. The flexible fixture mechanism is described using configuration parameters. According to the parameters, the CNC system automatically generates the control feature and the human machine interface （HMI） operation function. The CNC system is implemented in a flexible fixture for skin-strlnger assembly, and results show the effectiveness of the system.
文摘Taking a microwave product as an example, a system of integrated assembly structure design is presented. Getting design constraints from the upstream design section through product data management(PDM), the system generates the assembly scheme using the case? based method, then assigns the design requirements into each component of the assembly. The detail design for each component can be performed under these design constraints. In order to practise concurrent design, the system sends the final design result to the upstream section and downstream section through PDM to achieve information sharing and integration.
文摘The parametric part assembly generation method is presented. Based on the parametric part generated by means of constructive-element, through interactively inputting the relationships of the location and the assembly, and by compiling operations like movement and rotation, the assembly drawing is created so as to implement the occurrence of the parameterizations of the assembly and the part drawing. The data structure of the assembly part and the key technologies of hidden line removal in the implementation of assembly process, etc. , are described in detail.
基金supported by the National Natural Science Foundation of China (Nos. 21325417, 51533008)the MOST National Key Research and Development Plan (2016YFA0200200)+1 种基金the National Postdoctoral Program for Innovative Talents (No. BX201700209)the State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Donghua University (No. LK1403)
文摘Nanocarbon-based materials, such as carbon nanotubes(CNTs) and graphene have been attached much attention by scientific and industrial community. As two representative nanocarbon materials, one-dimensional CNTs and twodimensional graphene both possess remarkable mechanical properties. In the past years, a large amount of work have been done by using CNTs or graphene as building blocks for constructing novel, macroscopic, mechanically strong fibrous materials. In this review, we summarize the assembly approaches of CNT-based fibers and graphene-based fibers in chronological order, respectively. The mechanical performances of these fibrous materials are compared, and the critical influences on the mechanical properties are discussed. Personal perspectives on the fabrication methods of CNT-and graphene-based fibers are further presented.
基金The project supported by National Meg-science Engineering Project of the Chinese Government
文摘EAST （HT-7U） is a large fusion experimental device. It is a full superconducting tokamak with 1 MA of plasma current, 1000 s of plasma duration, high elongation and triangularity. It mainly consists of superconducting magnets of poloidal and toroidal field （PF ＆ TF）, vacuum vessel （VV）, thermal radiation shield （TRS） and cryostat vessel （CV）. The significant difficulty for assembly of EAST is tight installation tolerances, which are in the order of several tenth of a millimeter. In particular, the alignment of plasma facing components to the magnetic axis of the device is less than ±0.5 mm. At present, a reasonable assembly process of EAST has been defined, and based on it, the alignment method for EAST, including the survey control network, the location of the main components in different directions, the magnetic axis determination and the accurate positioning of the plasma facing components inside of the vacuum vessel and so on, has been defined by using the sophisticated optical metrology system （SOMS）. This paper describes the assembly procedure of EAST and the installation tolerances associated with the main components. Meanwhile, how to establish the assembly survey control network, magnetic axis determination methods, are introduced in detail.
基金the financial support from Natural Science and Engineering Research Council of Canada (NSERC)funding from Science and Technology Commission of Shanghai Municipality (No.11PJ1403500)+1 种基金the Open Project Program of State Key Laboratory of Industrial Control Technology (No.ICT1113)Innovation Program of Shanghai Municipal Education Commission (No.12YZ022)
文摘Nanowires and nanotubes of diverse material compositions,properties and/or functions have been produced or fabricated through various bottom-up or top-down approaches.These nanowires or nanotubes have also been utilized as potential building blocks for functional nanodevices.The key for the integration of those nanowire or nanotube based devices is to assemble these one dimensional nanomaterials to specific locations using techniques that are highly controllable and scalable.Ideally such techniques should enable assembly of highly uniform nanowire/nanotube arrays with precise control of density,location,dimension or even material types of nanowires/nanotubes.Numerous assembly techniques are being developed that can quickly align and assemble large quantities of one type or multiple types of nanowires through parallel processes,including flow-assisted alignment,Langmuir-Blodgett assembly,bubble-blown technique,electric/magnetic-field directed assembly,contact/roll printing,knocking-down,etc..With these assembling techniques,applications of nanowire/nanotube based devices such as flexible electronics and sensors have been demonstrated.This paper delivers an overall review of directed nanowire/nanotube assembling approaches and analyzes advantages and limitations of each method.The future research directions have also been discussed.
文摘Two-dimensional(2D) transition metal carbides, carbonitrides and nitrides, known as MXenes, are emerging quickly at the frontiers of 2D materials world. Their exotic properties such as the highest electrical conductivity among all solution-processed 2 D materials, the best electromagnetic interference shielding performance outperforming that of copper or aluminum at a nanoscale thickness, as well as the highest volumetric capacitance for pseudocapacitors, have been attracting extensive fundamental research and applications. Their unique surface chemistries, that is, hydrophilic groups terminated on the surface of MXenes after etching and delamination, enable plenty of opportunities for assembling into MXene building blocks. Particularly, assembling at liquid–liquid, liquid–solid, liquid–air, and solid–solid interfaces allows the efficient fabrication of various structures, including MXene surfactants, MXene heterostructures, MXene transparent films. Interfacial assembly of MXenes is of significance in unveiling more versatilities of MXenes as well as impacts on novel MXene-based architectures, based on which enhanced performance of devices is achieved. As such, this review focuses on the interfacial assembly of MXenes, explaining mechanisms behind various assembling and providing classical examples for corresponding interfacial assembling techniques. Applications of these as-assembled architectures are also discussed in brief. We believe this review may shed light on the interfacial chemistry of MXenes, thus guiding more efficient fabrication of MXene-based functional films/coatings/electrodes/devices.
基金supported by the National Natural Science Foundations of China(Nos.5157051626,51475225)
文摘To fulfill the demands for higher quality,efficiency and flexibility in aviation industry,a multi-functional end effector is designed to automate the drilling and riveting processes in assembling carbon fiber reinforced polymer(CFRP)and aluminum components for a robotic aircraft assembly system.To meet the specific functional requirements for blind rivet installation on CFRP and aluminum materials,additional modules are incorporated on the end effector aside of the basic processing modules for drilling.And all of these processing modules allow for a onestep-drilling-countersinking process,hole inspection,automatic rivet feed,rivet geometry check,sealant application,rivet insertion and installation.Besides,to guarantee the better quality of the hole drilled and joints riveted,several online detection and adjustment measures are applied to this end effector,including the reference detection and perpendicular calibration,which could effectively ensure the positioning precision and perpendicular accuracy as demanded.Finally,the test result shows that this end effector is capable of producing each hole to a positioning precision within ±0.5 mm,aperpendicular accuracy within 0.3°,a diameter tolerance of H8,and a countersink depth tolerance of±0.01 mm.Moreover,it could drill and rivet up to three joints per minute,with acceptable shearing and tensile strength.
文摘The key realization techniques of virtual assembly process planning （VAPP） system are analyzed, including virtual assembly model, real-time collision detection, automatic constraint recognition algorithm, cable harness assembly process planning and visual assembly process plan at the workshop. A virtual assembly model based on hierarchical assembly task list （HATL） is put forward, in which assembly tasks are defined to express component assembling operations and are sequentially and hierarchically organized according to different subassemblies, which can perfectly model the construction process of product, And a multi-layer automatic geometry constraint recognition algorithm of how to identify assmbly constraint relations in the virtual environment is proposed, then a four-layer collision detection algorithm is discussed. A VAPP system is built and some simple mechanical assemblies are used to illustrate the feasibility of the proposed method and algorithms.
基金Supported by the National Key Laboratory of Vehicular Transmission (9140C3405020905)the National Natural Science Foundation of China(50905016)
文摘To obtain the performance characteristics of hydrodynamic tractor-retarder assembly under traction work condition,a numerical simulation model of flow channel was established and tetrahedron unstructured grids were adopted in the meshing stage.The racing rotating speed of the brake wheels was calculated by computational fluid dynamics（CFD） calculation and interpolation,and then accurate boundary condition was applied to the CFD simulation to study the pressure and velocity distribution of internal flow field in hydrodynamic tractor-retarder assembly.Finally,the original characteristics were calculated by CFD post-processing analysis.Comparison of experimental data and flow field analysis results showed that the calculation tolerance of the torque ratio K and the efficiency η was less than 5%,and the calculation tolerance of the pump torque coefficient λ was less than 10%.
基金financially supported by the National Key R@D Program of China(Grants 2016YFB0100100,2016YFA0200200)the National Natural Science Foundation of China(Grant Nos.51872283,22075279,21805273,22005297,22005298)+7 种基金the Liao Ning Revitalization Talents Program(Grant XLYC1807153)the Natural Science Foundation of Liaoning ProvinceJoint Research Fund Liaoning-Shenyang National Laboratory for Materials Science(Grant 20180510038)Dalian Innovation Support Plan for High Level Talents(2019RT09)the Dalian National Laboratory For Clean Energy(DNL),CASDNL Cooperation Fund,CAS(DNL180310,DNL180308,DNL201912,and DNL201915)DICP(DICP ZZBS201708,DICP ZZBS201802,DICP I2020032)the China Postdoctoral Science Foundation(2019M661141,2020M680995)。
文摘Synthesis and applications of three-dimensional(3 D)porous graphene frameworks(GFs)have attracted extensive interest owing to their intriguing advantages of high specific surface area,enriched porosity,excellent electrical conductivity,exceptional compressibility and processability.However,it is still challenging for economically viable,fast and scalable assembly of 3 D GFs at room-temperature.Herein,we reported a one-step scalable strategy for fast self-assembly of graphene oxide into 3 D macroscopically porous GFs,with assistance of polyoxometalates(POM)as functional cross-linker and hydrazine hydrate as reductant at room-temperature.The resulting 3 D interconnected macroporous POM-GFs uniformly decorated with ultrasmall POM nanoclusters were directly processed into binder-/additive-free film compact electrodes(1.68 g cm^(-3))with highly aligned,layer-stacked structure and electrically conductivity(622 S m-1)for high-performance supercapacitors,showing an impressive gravimetric capacitance of205 F g-1,volumetric capacitance of 334 F cm^(-3) at 1 mV s^(-1),and remarkable cycling stability with capacitance retention of 83%after 10,000 cycles,outperforming the most reported GFs.Further,the solid-state supercapacitors offered excellent gravimetric capacitance of 157 F g-1 exceptionally volumetric capacitance of 115 F cm^(-3) at 2 mV s^(-1) based on single electrode,and volumetric energy density of2.6 mWh cm^(-3).Therefore,this work will open novel opportunities to room-temperature fast assembly of 3 D porous graphene architectures for high-energy-density supercapacitors.
文摘Jet pulse assembly is one of the main components of jet hydraulic oscillator.The pressure wave characteristics produced by jet pulse assembly have an important influence on the performance of the tool.In this paper,the structure and working principle of jet pulse assembly are studied,the mechanical analysis model of piston rod is established,the dynamic resistance ratio formula of jet pulse assembly is deduced,and the numerical simulation test of 89-mm jet pulse assembly structure parameters is carried out.The results show that the piston rod downward stroke is driven by both the jet element driving force and the throttle plate load driving force,and can stably descend.The driving force of the piston rod upward stroke jet element is opposite to the load acting force of the throttle disc,and the jet driving force needs to be greater than the load resistance of the throttle disc to stably ascend.The dynamic resistance ratio formula is deduced.When the area of the end of the piston rod is reduced,the resistance of the throttle disc is reduced and the jet power is increased,thus solving the problem of insufficient power of the piston rod in the upstroke and ensuring the normal operation of the tool.Ten groups of numerical simulation tests were carried out,and it was found that the pressure amplitude and pressure drop of the tool decreased significantly with the increase of the tool size,and the error between the numerical simulation value and the theoretical calculation value was less than 9%,which verified the correctness of the theory.It is suggested to select tools on site according to the drilling construction situation to ensure the drilling effect.
基金supported in part by the National Natural Science Foundation of China(No.51575274)the National Defense Basic Scientific Research of China(No.JCKY2016605B006)the Jiangxi Provincial Key R&D Program Project(No.20161ACE50004)
文摘Due to the complexity of strong metal interference and multiple occlusions in aircraft assembly workshop,the random "drift"phenomenon often happens in the ultra wide band (UWB)based positioning system.To solve this,a fusion positioning optimization algorithm is proposed based on median filtering,hidden Markov model (HMM)a nd Kalman filtering.Firstly,based on the three-dimensional (3D) median filtering,aqueue optimization method with weights is introduced to smooth the measurement data and eliminate the abnormal value.Secondly,taking Singer model as a reference,a single-dimension acceleration distribution model is designed.In order to further consider the spatial motion characteristics of objects in workshop,the distribution is extended from 1D to 3D,and discretized into the state quantity of HMM.Subsequently,the data obtained by the two methods are fused by taking Kalman filter as an iterator,and then the optimized location solution is obtained based on dynamic weights.Finally,an experiment is conducted in an aircraft assembly workshop.Results show that 99.3% of dynamic positioning errors are less than 15 cm after using the proposed algorithm.Even in the situation with large signal-fluctuation,there are 71.6% of positioning data whose errors are reduced.The random "drift"is greatly decreased.
基金the financial support from the National Science Foundation of China(NSFC)(No.51733003).
文摘Complex multiscale assemblies of metal-organic frameworks are essential in the construction of largescale optical platforms but often restricted by their bulk nature and conventional techniques.The integration of nanomaterials and 3D printing technologies allows the fabrication of multiscale functional architectures.Our study reports a unique method of controlled 3D assembly purely relying on the post-printing treatment of printed constructs.By immersing a 3D-printed patterned construct consisting of organic ligand in a solution of lanthanide ions,in situ growth of lanthanide metal-organic frameworks(LnMOFs)can rapidly occur,resulting in macroscopic assemblies and tunable fluorescence properties.This phenomenon,caused by coordination and chelation of lanthanide ions,also renders a sub-millimeter resolution and high shape fidelity.As a proof of concept,a type of 3D assembled LnMOFsbased optical sensing platform has demonstrated the feasibility in response to small molecules such as acetone.It is anticipated that the facile printing and design approach developed in this work can be applied to fabricate bespoke multiscale architectures of functional materials with controlled assembly,bringing a realistic and economic prospect.
基金financial support from National Key Research and Development Program(2017YFD0501403)National Natural Science Foundation of China(Nos.81872819)+4 种基金Natural Science Foundation of Jiangsu Province(No.BK20171390)supported by Double First-Rate construction plan of China Pharmaceutical University(CPU2018GY26)the Project of State Key Laboratory of Natural Medicines,China Pharmaceutical University(No.SKLNMZZCX201816)the National Science and Technology Major Project(2017ZX09101001)the financial support from Development Funds for Priority Academic Programs in Jiangsu Higher Education Institutions-Young Talent Program。
文摘Stimuli-triggered drug delivery systems hold vast promise in local infection treatment for the site-specific targeting and shuttling of drugs.Herein,chitosan conjugates(SPCS)installed with sialic acid(SA)and phenylboronic acid(PBA)were synthesized,of which SA served as targeting ligand for coccidium and reversible-binding bridge for PBA.The enhanced drug-loading capacity of SPCS micelles was attributed to a combination assembly from hydrophobicity-driving and reversible borate bridges.The drug-loaded SPCS micelles shared superior biostability in upper gastrointestinal tract.After reaching the lesions,the borate bridges were snipped by carbohydrates under a higher pH followed by accelerated drug release,while SA exposure on micellar surface facilitated drug cellular internalization to eliminate parasites inside.The drugmicelles revealed an enhanced anti-coccidial capacity with a higher index of 185.72 compared with commercial preparation.The dual-responsive combination of physicochemical assembly could provide an efficient strategy for the exploitation of stable,safe and flexible anti-infectious drug delivery systems.
