We perform a theoretical investigation on the control over the atomic excitation of Rydberg states with shaped intense ultrashort laser pulses. By numerically solving the time-dependent Schr?dinger equation(TDSE), w...We perform a theoretical investigation on the control over the atomic excitation of Rydberg states with shaped intense ultrashort laser pulses. By numerically solving the time-dependent Schr?dinger equation(TDSE), we systematically study the dependence of the population of the Rydberg states on the π phase step position in the frequency spectra of the laser pulse for different intensities, central wavelengths and pulse durations. Our results show that the Rydberg excitation process can be effectively modulated using shaped intense laser pulses with the laser intensity as high as 1 × 1014 W/cm2. Our work also have benefit to the future investigation to find out the dominant mechanism behind the excitation of Rydberg states in strong laser fields.展开更多
We present a parallel numerical method of simulating the interaction of atoms with a strong laser field by solving the time-depending Schr?dinger equation(TDSE) in spherical coordinates. This method is realized by com...We present a parallel numerical method of simulating the interaction of atoms with a strong laser field by solving the time-depending Schr?dinger equation(TDSE) in spherical coordinates. This method is realized by combining constructing block diagonal matrices through using the real space product formula(RSPF) with splitting out diagonal sub-matrices for short iterative Lanczos(SIL) propagator. The numerical implementation of the solver guarantees efficient parallel computing for the simulation of real physical problems such as high harmonic generation(HHG) in these interaction systems.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant No.11874246)
文摘We perform a theoretical investigation on the control over the atomic excitation of Rydberg states with shaped intense ultrashort laser pulses. By numerically solving the time-dependent Schr?dinger equation(TDSE), we systematically study the dependence of the population of the Rydberg states on the π phase step position in the frequency spectra of the laser pulse for different intensities, central wavelengths and pulse durations. Our results show that the Rydberg excitation process can be effectively modulated using shaped intense laser pulses with the laser intensity as high as 1 × 1014 W/cm2. Our work also have benefit to the future investigation to find out the dominant mechanism behind the excitation of Rydberg states in strong laser fields.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11534004,11627807,11774131,and 11774130)the Scientific and Technological Project of Jilin Provincial Education Department in the Thirteenth Five-Year Plan,China(Grant No.JJKH20170538KJ)
文摘We present a parallel numerical method of simulating the interaction of atoms with a strong laser field by solving the time-depending Schr?dinger equation(TDSE) in spherical coordinates. This method is realized by combining constructing block diagonal matrices through using the real space product formula(RSPF) with splitting out diagonal sub-matrices for short iterative Lanczos(SIL) propagator. The numerical implementation of the solver guarantees efficient parallel computing for the simulation of real physical problems such as high harmonic generation(HHG) in these interaction systems.